Design of pH‐universal electrocatalysts for hydrogen evolution reaction
Source abstract
Abstract
Abstract The path to searching for sustainable energy has never stopped since the depletion of fossil fuels can lead to serious environmental pollution and energy shortages. Using water electrolysis to produce hydrogen has been proven to be a prioritized approach for green resource production. It is highly crucial to explore inexpensive and high‐performance electrocatalysts for accelerating hydrogen evolution reaction (HER) and apply them to industrial cases on a large scale. Here, we summarize the different mechanisms of HER in different pH settings and review recent advances in non‐noble‐metal‐based electrocatalysts. Then, based on the previous efforts, we discuss several universal strategies for designing pH‐independent catalysts and show directions for the future design of pH‐universal catalysts.
Source: crossref · Quality: baseline
Research context
OpenAlex topics: Electrocatalysts for Energy Conversion · Advanced battery technologies research · Fuel Cells and Related Materials
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
State Key Laboratory of Silicon and Advanced Semiconductor Materials, School of Materials Science and Engineering Zhejiang University Hangzhou China
Institute of Wenzhou Zhejiang University Wenzhou China
Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering Zhejiang University Hangzhou China
References (100+)
Show source-provided references
1. 10.1038/nature1147510.1038/nature11475 ↗
2. 10.1126/science.120885910.1126/science.1208859 ↗
3. 10.1073/pnas.060339510310.1073/pnas.0603395103 ↗
4. 10.1039/D1CS00800E10.1039/D1CS00800E ↗
5. 10.1016/j.rser.2011.01.00710.1016/j.rser.2011.01.007 ↗
6. 10.1021/cs500923c10.1021/cs500923c ↗
7. 10.1039/C4CS00470A10.1039/C4CS00470A ↗
8. 10.1088/2515-7655/acab2d10.1088/2515-7655/acab2d ↗
9. Water electrolysis based on renewable energy for hydrogen production, Chinese
10. 10.1007/s42864-023-00202-810.1007/s42864-023-00202-8 ↗
11. 10.1039/C4CS00448E10.1039/C4CS00448E ↗
12. 10.1016/j.jcat.2014.12.03310.1016/j.jcat.2014.12.033 ↗
13. 10.1021/jp104888710.1021/jp1048887 ↗
14. 10.1016/j.gee.2020.10.01310.1016/j.gee.2020.10.013 ↗
15. 10.1021/cr100246c10.1021/cr100246c ↗
16. 10.1021/acsnano.2c0282010.1021/acsnano.2c02820 ↗
17. 10.1016/j.cej.2020.12701310.1016/j.cej.2020.127013 ↗
18. 10.1021/acsmaterialslett.0c0053610.1021/acsmaterialslett.0c00536 ↗
19. 10.1016/B978-044452745-5.00315-410.1016/B978-044452745-5.00315-4 ↗
20. 10.1016/j.ijhydene.2013.01.15110.1016/j.ijhydene.2013.01.151 ↗
21. 10.1038/s41560-020-0577-x10.1038/s41560-020-0577-x ↗
22. 10.1016/j.electacta.2018.04.15410.1016/j.electacta.2018.04.154 ↗
23. 10.1002/anie.20191391010.1002/anie.201913910 ↗
24. 10.1002/smll.20190305710.1002/smll.201903057 ↗
25. 10.1016/j.cclet.2023.10873710.1016/j.cclet.2023.108737 ↗
26. 10.1021/acsenergylett.9b0004710.1021/acsenergylett.9b00047 ↗
27. 10.1038/s41467-020-14462-210.1038/s41467-020-14462-2 ↗
28. 10.1002/aenm.20170353810.1002/aenm.201703538 ↗
29. 10.1016/j.nanoen.2017.03.02410.1016/j.nanoen.2017.03.024 ↗
30. 10.1021/jacs.7b0633710.1021/jacs.7b06337 ↗
31. 10.1038/ncomms1227210.1038/ncomms12272 ↗
32. 10.1038/nmat473810.1038/nmat4738 ↗
33. 10.1002/anie.20130809910.1002/anie.201308099 ↗
34. 10.1002/adma.20180632610.1002/adma.201806326 ↗
35. 10.1002/advs.20170046410.1002/advs.201700464 ↗
36. 10.1186/s40580-021-00254-x10.1186/s40580-021-00254-x ↗
37. 10.1021/acssuschemeng.7b0417310.1021/acssuschemeng.7b04173 ↗
38. 10.1038/s41467-019-12773-710.1038/s41467-019-12773-7 ↗
39. 10.1038/s41467-023-39963-810.1038/s41467-023-39963-8 ↗
40. 10.1038/s41467-023-40972-w10.1038/s41467-023-40972-w ↗
41. Direct seawater electrolysis by adjusting the local reaction environment of a catalyst
42. 10.1038/nchem.157410.1038/nchem.1574 ↗
43. 10.1039/D0EE01856B10.1039/D0EE01856B ↗
44. 10.1038/s41563-020-0788-310.1038/s41563-020-0788-3 ↗
45. 10.1021/acscatal.7b0368410.1021/acscatal.7b03684 ↗
46. 10.1002/cssc.20160158310.1002/cssc.201601583 ↗
47. 10.1007/s12274-022-4265-y10.1007/s12274-022-4265-y ↗
48. 10.1007/s12274-022-4869-210.1007/s12274-022-4869-2 ↗
49. 10.1002/aenm.20230143810.1002/aenm.202301438 ↗
50. 10.1021/acsenergylett.9b0022010.1021/acsenergylett.9b00220 ↗
51. 10.1007/BF0061248110.1007/BF00612481 ↗
52. 10.1126/science.aad499810.1126/science.aad4998 ↗
53. 10.1039/tf958540105310.1039/tf9585401053 ↗
54. 10.1149/1.185698810.1149/1.1856988 ↗
55. 10.1016/j.cattod.2013.07.00610.1016/j.cattod.2013.07.006 ↗
56. Rooij D · 2003 · 856
57. 10.1038/srep1380110.1038/srep13801 ↗
58. 10.1016/j.apcatb.2021.12071210.1016/j.apcatb.2021.120712 ↗
59. 10.1016/S0022-0728(84)80324-110.1016/S0022-0728(84)80324-1 ↗
60. 10.1038/s41467-018-04888-010.1038/s41467-018-04888-0 ↗
61. 10.1021/ja407115p10.1021/ja407115p ↗
62. 10.1021/ja510442p10.1021/ja510442p ↗
63. SchalenbachM.Impedance Spectroscopy and Cyclic Voltammetry to Determine Double Layer Capacitances and Electrochemically Active Surface Areas.ECSarXiv;2018. Preprint.https://www.researchgate.net/publication/330030949_Impedance_Spectroscopy_and_Cyclic_Voltammetry_to_Determine_Double_Layer_Capacitances_and_Electrochemically_Active_Surface_Areas10.1149/osf.io/gyexd ↗
64. 10.1016/S0013-4686(97)00112-610.1016/S0013-4686(97)00112-6 ↗
65. 10.1051/epjap:200717610.1051/epjap:2007176 ↗
66. 10.1006/jcis.1994.123610.1006/jcis.1994.1236 ↗
67. 10.1021/acssuschemeng.8b0402910.1021/acssuschemeng.8b04029 ↗
68. 10.1002/adma.20180713410.1002/adma.201807134 ↗
69. 10.1002/aenm.20170159210.1002/aenm.201701592 ↗
70. 10.1002/anie.20170642610.1002/anie.201706426 ↗
71. 10.1002/aenm.20170325910.1002/aenm.201703259 ↗
72. 10.1126/science.114148310.1126/science.1141483 ↗
73. 10.1021/ja201269b10.1021/ja201269b ↗
74. 10.1016/j.ijhydene.2015.09.07610.1016/j.ijhydene.2015.09.076 ↗
75. 10.1021/ja404523s10.1021/ja404523s ↗
76. 10.1038/s41467-018-07792-910.1038/s41467-018-07792-9 ↗
77. 10.1016/j.nanoen.2019.02.00610.1016/j.nanoen.2019.02.006 ↗
78. 10.1021/acsaem.9b0148610.1021/acsaem.9b01486 ↗
79. 10.1016/j.ijhydene.2022.09.18910.1016/j.ijhydene.2022.09.189 ↗
80. 10.1039/D0NR02939D10.1039/D0NR02939D ↗
81. 10.1002/celc.20190044810.1002/celc.201900448 ↗
82. 10.1016/j.jcis.2018.09.01810.1016/j.jcis.2018.09.018 ↗
83. 10.1016/j.apcatb.2021.12099310.1016/j.apcatb.2021.120993 ↗
84. 10.1016/j.electacta.2020.13659810.1016/j.electacta.2020.136598 ↗
85. 10.1016/j.ijhydene.2019.12.21210.1016/j.ijhydene.2019.12.212 ↗
86. 10.1002/adma.20170074810.1002/adma.201700748 ↗
87. 10.1021/acssuschemeng.1c0617810.1021/acssuschemeng.1c06178 ↗
88. 10.1007/s12274-018-2040-x10.1007/s12274-018-2040-x ↗
89. 10.1002/aenm.20200208210.1002/aenm.202002082 ↗
90. 10.1002/smll.20190179610.1002/smll.201901796 ↗
91. 10.1039/c3cc43107j10.1039/c3cc43107j ↗
92. 10.1021/ja403440e10.1021/ja403440e ↗
93. 10.1039/C5CS00434A10.1039/C5CS00434A ↗
94. 10.1021/acs.chemmater.5b0128410.1021/acs.chemmater.5b01284 ↗
95. 10.1039/C4EE00957F10.1039/C4EE00957F ↗
96. 10.1016/j.mtsust.2021.10007410.1016/j.mtsust.2021.100074 ↗
97. 10.1002/adma.20160550210.1002/adma.201605502 ↗
98. 10.1039/D0TA09644J10.1039/D0TA09644J ↗
99. 10.1016/j.mattod.2017.03.01910.1016/j.mattod.2017.03.019 ↗
100. 10.1002/advs.20150028610.1002/advs.201500286 ↗