Electrochemical strain microscopy of local electrochemical processes in solids: mechanism of imaging and spectroscopy in the diffusion limit
Source abstract
Abstract
Changes in ionic concentration and electrochemical processes in solids are invariably associated with changes in molar volume. Correspondingly, materials with mobile ions develop strain in response to applied electric bias. This electromechanical coupling mediated by mobile ions lays the foundation for the electrochemical strain microscopy (ESM) of energy storage and conversion materials. Here, we analyze the imaging and spectroscopic mechanism in ESM in the diffusion limit and discuss the similarities between ESM and macroscopic current-based electrochemical measurements. The theoretical challenges in ESM are formulated.
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Research context
OpenAlex topics: Force Microscopy Techniques and Applications · Electrochemical Analysis and Applications · Analytical Chemistry and Sensors
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