journal article·2024-03-01Open access

Persistence of atoms in molecules: there is room beyond electron densities

María Menéndez-Herrero, Ángel Martín Pendás

IUCrJ· Volume 11· Issue 2

Abstract

Evidence that the electronic structure of atoms persists in molecules to a much greater extent than has been usually admitted is presented. This is achieved by resorting to N-electron real-space descriptors instead of one- or at most two-particle projections like the electron or exchange-correlation densities. Here, the 3N-dimensional maxima of the square of the wavefunction, the so-called Born maxima, are used. Since this technique is relatively unknown to the crystallographic community, a case-based approach is taken, revisiting first the Born maxima of atoms in their ground state and then some of their excited states. It is shown how they survive in molecules and that, beyond any doubt, the distribution of electrons around an atom in a molecule can be recognized as that of its isolated, in many cases excited, counterpart, relating this fact with the concept of energetic promotion. Several other cases that exemplify the applicability of the technique to solve chemical bonding conflicts and to introduce predictability in real-space analyses are also examined.
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Research context

OpenAlex topics: Advanced Chemical Physics Studies · Crystallography and molecular interactions · Spectroscopy and Quantum Chemical Studies

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