journal article·2019-12-23Open access

Theoretical Investigation of All Optical Switching by Intersystem Crossing

Yuhao Zou, Haiwei Wang, Haozhe Huang, Zhihao Zeng, Kai Wang, Sicong Wang, Xiangping Li, Changsheng Xie

Applied Sciences· Volume 10· Issue 1

Abstract

The dynamics of spin flips induced by the femtosecond laser are theoretically investigated in this article. The spin flips in this scenario are attributed to the intersystem crossing (ISC) described within the frame of the Rabi model. This new explanation is a step attempting to explain the mechanism of the all-optical magnetic orientation switching in the perspective of the conservation of the angular momentum and breaks of the selection rule, which is ignored in the Raman scattering related explanations. The final spin states discussed herein are closely related to the intensity of the incident laser and the ISC decay rate. The quantitative analysis of the relation between decay rate, temperature and the intensity of the laser is discussed.
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Research context

OpenAlex topics: Laser-Matter Interactions and Applications · Quantum optics and atomic interactions · Spectroscopy and Quantum Chemical Studies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Wuhan National Laboratory of Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, China

School of Physics, Huazhong University of Science and Technology, Wuhan 430074, China

Guangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications, Institute of Photonics Technology, Jinan University, Guangzhou 510632, China

Funding

National Natural Science Foundation of China · Science Technology Support Program of Hubei Province

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