journal article·2020-05-29Open access

High-Efficient Micro Reacting Pipe with 3D Internal Structure: Design, Flow Simulation, and Metal Additive Manufacturing

Xiaomin Chen, Di Wang, Jingming Mai, Xiaojun Chen, Wenhao Dou

Applied Sciences· Volume 10· Issue 11

Abstract

The micro reacting pipe with 3D internal structure, which is a micromixer with the shape of the pipe, has shown great advantages regarding mass transfer and heat transfer. Since the fluid flow is mostly laminar at the micro-scale, which is unfavorable to the diffusion of reactants, it is important to understand the influence of the geometry of the microchannel on the fluid flow for improving the diffusion of the reactants and mixing efficiency. On the other hand, it is a convenient method to manufacture a micro reacting pipe in one piece through metal additive manufacturing without many post-processing processes. In this paper, a basis for the design of a micromixer model was provided by combining the metal additive manufacturing process constraints with computational fluid dynamics (CFD) simulation. The effects of microchannel structures on fluid flow and mixing efficiency were studied by CFD simulation whose results showed that the internal micro-structure had a significantly positive effect on the mixing efficiency. Based on the simulation results, the splitting-collision mechanism was discussed, and several design rules were obtained. Two different materials were selected for manufacturing with the laser powder bed fusion (L-PBF) technology. After applying pressure tests to evaluate the quality of the formed parts and comparing the corrosion-resistance of the two materials, one material was picked out for the industrial application. Additionally, the chemical experiment was conducted to evaluate the accuracy of the simulation. The experimental results showed that the mixing efficiency of the micro reacting pipe increased by 56.6%, and the optimal determining size of the micro reacting pipe was 0.2 mm. The study can be widely used in the design and manufacture of a micromixer, which can improve efficiency and reacting stability in this field.
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Research context

OpenAlex topics: Innovative Microfluidic and Catalytic Techniques Innovation · Additive Manufacturing and 3D Printing Technologies · Additive Manufacturing Materials and Processes

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

School of Mechanical and Automotive Engineering, South China University of Technology, Guangzhou 510640, China

Department of Electrical Engineering and Information Technology, Karlsruhe Institute of Technology, 76131 Karlsruhe, Germany

Funding

National Natural Science Foundation of China · Science and Technology Planning Project of Guangdong Province · High-level Personnel Special Support Plan of Guang-dong Province · Guangzhou Pearl River New Talent Project · Fundamental Research Funds for the Central Universities

References (39)

Show source-provided references
1. Post-column reaction with a 3D-printed two-stage microreactor and flame ionization detection for carbon compound independent response in fast gas chromatography10.1016/j.chroma.2019.460460 ↗
2. Lin, W. (2016). Design and Application of Microreactor: Mixing of microfluidics, Chemical Industry Press. [1st ed.].
3. Applications of microreactor in chemistry and chemical engineering
4. Microreactor Chemical Bath Deposition of Laterally Graded Cd1−xZnxS Thin Films: A Route to High-Throughput Optimization for Photovoltaic Buffer Layers10.1021/cm3023506 ↗
5. Recent Advances in Micro Reaction Technology10.1039/c1cc00089f ↗
6. Mixing intensification under turbulent conditions in a high pressure microreactor10.1016/j.cej.2019.122859 ↗
7. Design and simulation of passive mixing in microfluidic systems with geometric variations10.1016/j.cej.2009.05.035 ↗
8. A high-efficiency planar micromixer with convection and diffusion mixing over a wide Reynolds number range10.1007/s10404-007-0238-4 ↗
9. Shi, H., Nie, K., Dong, B., Chao, L., Gao, F., Ma, M., Long, M., and Liu, Z. (2020). Mixing enhancement via a serpentine micromixer for real-time activation of carboxyl. Chem. Eng. J., 392.10.1016/j.cej.2019.123642 ↗
10. Three-Dimensional Passive Micromixer Fabricated by Two-Photon Polymerization
11. Schirmer, M., Uhlemann, J., Rebenklau, L., Bauer, T., and Wolter, K.J. (2008, January 7–11). 3D-microfluidic reactor in LTCC. Proceedings of the 2008 31st International Spring Seminar on Electronics Technology, Budapest, Hungary.10.1109/ISSE.2008.5276614 ↗
12. Hydrodynamic, Mass Transfer and RTD Studies of Fluid Flow in a Spiral Microreactor10.1007/s40034-019-00143-3 ↗
13. Effect of micro-channel geometry on fluid flow and mixing10.1016/j.simpat.2010.12.008 ↗
14. A novel passive micromixer based on unbalanced splits and collisions of fluid streams10.1088/0960-1317/20/5/055007 ↗
15. A novel design for 3D passive micromixer based on Cantor fractal structure
16. A novel passive micromixer designed by applying an optimization algorithm to the zigzag microchannel10.1016/j.cej.2016.11.052 ↗
17. Metal Additive Manufacturing: A Review10.1007/s11665-014-0958-z ↗
18. Wong, K.V., and Hernandez, A. (2012). A Review of Additive Manufacturing. ISRN Mech. Eng., 1–10.10.5402/2012/208760 ↗
19. Laser additive manufacturing of metallic components: Materials, processes and mechanisms10.1179/1743280411Y.0000000014 ↗
20. Advanced reactor engineering with 3D printing for the continuous-flow synthesis of silver nanoparticles10.1039/C6RE00210B ↗
21. Integrated 3D printed heaters for microfluidic applications: Ammonium analysis within environmental water10.1016/j.aca.2019.11.025 ↗
22. Replication and characterization of 316L stainless steel micro-mixer by micro powder injection molding10.1016/j.jallcom.2010.01.147 ↗
23. Fabrication of porous metal by selective laser melting as catalyst support for hydrogen production microreactor10.1016/j.ijhydene.2019.10.173 ↗
24. Experimental Investigation of Numerically Optimized Wavy Microchannels Created Through Additive Manufacturing10.1115/1.4038180 ↗
25. Computational methodology for the development of microdevices and microreactors with ANSYS CFX10.1016/j.mex.2019.12.006 ↗
26. Build Direction Effects on Microchannel Tolerance and Surface Roughness10.1115/1.4031071 ↗
27. (2016). Investigation of crystal growth mechanism during selective laser melting and mechanical property characterization of 316L stainless steel parts. Mater. Des., 100, 291–299.10.1016/j.matdes.2016.03.111 ↗
28. Study on the designing rules and processability of porous structure based on selective laser melting (SLM)10.1016/j.jmatprotec.2013.05.001 ↗
29. The numerical computation of turbulent flows10.1016/0045-7825(74)90029-2 ↗
30. Fluent Inc (2001). Fluent 6.0 Users Guide, Fluent Inc.
31. A numerical study of mixing in a microchannel with circular mixing chambers10.1002/aic.11833 ↗
32. Characterisation of micromixing efficiency by the iodide–iodate reaction system. Part, I. Experimental procedure10.1016/S0009-2509(00)00068-3 ↗
33. Triodide ion formation equilibrium and activity coefficients in aqueous solution10.1007/BF00650374 ↗
34. The Application of the Beer-Lambert Law to Optically Anisotropic Systems10.1126/science.110.2845.41.b ↗
35. A New Parallel Competing Reaction System for Assessing Micromixing Efficiency-Experimental Approach10.1016/0009-2509(96)00270-9 ↗
36. Micro Mixing Time in the Eddy Dissipation Concept10.1080/00102200008947277 ↗
37. Micromixers-a review on passive and active mixing principles10.1016/j.ces.2004.11.033 ↗
38. Helical flows and chaotic mixing in curved micro channels10.1002/aic.10188 ↗
39. Villermaux-Dushman protocol for experimental characterization of micromixers10.1016/j.cep.2011.06.006 ↗