journal article·2025-03-18Open access

On the Formation of Carbonaceous By-Product Species in Spray Flame Synthesis of Maghemite Nanoparticles

Ricardo Tischendorf, Kristina Duschik, Fabian Fröde, Manuel Reddemann, Reinhold Kneer, Heinz Pitsch, Mirko Schaper, Hans-Joachim Schmid

Applied Sciences· Volume 15· Issue 6

Abstract

This study investigates the formation of by-product species during flame spray synthesis (SFS) of superparamagnetic maghemite (γ-Fe2O3) nanoparticles. Four samples are synthesized by utilizing two standardized burner types (SpraySyn1 and SpraySyn2) and varying the iron (III) nonahydrate (INN) concentration (0.1 M and 0.2 M) in the precursor feed while using ethanol and 2-ethylhexanoic acid as solvent. Conducting complementary powder analysis revealed a predominant presence of carboxylates and carbonates as by-product species (~14–18 wt.%), while no strong indications for elemental carbon and precursor/solvent residues can be found. Carbonates/carboxylates are located on particle surfaces, and the particles’ surface loadings by these species are independent of the precursor concentration but depend on burner type, with SpraySyn2 exhibiting lower values, indicating a more complete combustion for this burner. Through time-resolved thermophoretic sampling, we further demonstrate that carbon forms temporally in the visible flame center when using SpraySyn1. Since carbon solely forms momentarily within large flame pulses and decomposes further downstream, its temporal formation is of minor relevance for the final particle purity. However, its local co-existence aside from γ-Fe2O3 in the flame has potential to bias in situ diagnostics.
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Research context

OpenAlex topics: Thermal and Kinetic Analysis · Laser-Ablation Synthesis of Nanoparticles · Coagulation and Flocculation Studies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Particle Technology Group, University of Paderborn, 33102 Paderborn, Germany

Department of Material Science, University of Paderborn, 33100 Paderborn, Germany

Institute for Combustion Technology, RWTH Aachen University, 52056 Aachen, Germany

Institute of Heat and Mass Transfer, RWTH Aachen University, 52056 Aachen, Germany

Funding

DFG (German Research Foundation)

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