journal article·2024-12-05Open access

Radon Exhalation Rate, Radioactivity Content, and Mineralogy Assessment of Significant Historical and Artistic Interest Construction Materials

Francesco Caridi, Daniele Chiriu, Stefania Da Pelo, Giuliana Faggio, Michele Guida, Giacomo Messina, Maurizio Ponte, Silvestro Antonio Ruffolo, Domenico Majolino, Valentina Venuti

Applied Sciences· Volume 14· Issue 23

Abstract

In this paper, an investigation focused on assessing the radon exhalation, the natural radioactivity level, and the mineralogy of natural stones of particular historical–artistic interest employed as building materials was carried out. The Closed Chamber Method (CCM) with the Durridge Rad7 apparatus for short-lived radon progeny alpha spectrometry and High Purity Germanium (HPGe) gamma spectrometry were used to determine the radon exhalation rate and specific activities of 226Ra, 232Th, and 40K, respectively. Furthermore, several indices were evaluated to determine the radiological risk due to radiation exposure from the investigated natural stones, i.e., the absorbed gamma dose rate (D), the activity concentration index (ACI), and the alpha index (Iα). Finally, X-ray diffraction (XRD) and Micro-Raman Scattering (MRS) investigations were performed to correlate the chemical composition and mineralogical characteristics of natural stones with the radon exhalation rate and the natural radioactivity content. It is worth noting that the findings from this study can be used to guide future research into the background levels of radioactivity in stones used as construction materials.
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Research context

OpenAlex topics: Radioactivity and Radon Measurements · Radiation Shielding Materials Analysis · Nuclear Physics and Applications

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Affiliations

Dipartimento di Scienze Matematiche e Informatiche, Scienze Fisiche e Scienze della Terra, Università degli Studi di Messina, V.le F. Stagno D’Alcontres, 31, 98166 Messina, Italy

Dipartimento di Fisica, Università degli Studi di Cagliari, Cittadella Universitaria di Monserrato, S.P. Monserrato-Sestu Km 0,700, 09042 Monserrato, Italy

Dipartimento di Scienze Chimiche e Geologiche, Università degli Studi di Cagliari, Cittadella Universitaria di Monserrato, S.P. Monserrato-Sestu Km 0,700, 09042 Monserrato, Italy

Dipartimento di Ingegneria dell’Informazione, delle Infrastrutture e dell’Energia Sostenibile (DIIES), Università “Mediterranea”, Via Zehender, 89122 Reggio Calabria, Italy

Dipartimento di Ingegneria dell’Informazione ed Elettrica e Matematica applicata (DIEM), Università Degli Studi di Salerno, Via Giovanni Paolo II, 132, 84084 Fisciano, Italy

Dipartimento di Biologia, Ecologia e Scienze della Terra (DiBEST), Università della Calabria, Via Pietro Bucci, 87036 Arcavacata di Rende, Italy

Funding

European Union—Next Generation EU

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