journal article·2017-07-08Open access

Collinear FAST CARS for Chemical Mapping of Gases

Anton Shutov, Dmitry Pestov, Narangerel Altangerel, Zhenhuan Yi, Xi Wang, Alexei Sokolov, Marlan Scully

Applied Sciences· Volume 7· Issue 7

Abstract

We examine the concentration dependence of the Coherent Anti-Stokes Raman Scattering (CARS) signal obtained for gas mixtures at various conditions using the Femtosecond Adaptive Spectroscopic Technique (FAST). We use the CARS signal of the Q-branch vibrational oscillation of molecular oxygen (1556 cm−1) to confirm the quadratic dependence of the coherent signal on the number of molecules in a test volume. In addition, we demonstrate multi-shot FAST CARS imaging of a gas flow in free space by raster-scanning the area of interest.
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Research context

OpenAlex topics: Spectroscopy Techniques in Biomedical and Chemical Research · Spectroscopy and Chemometric Analyses · Photoacoustic and Ultrasonic Imaging

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Affiliations

Institute for Quantum Science and Engineering, Department of Physics and Astronomy, Texas A&M University, College Station, TX 77843-4242, USA

Quantum Optics Laboratory at the Baylor Research and Innovation Collaborative, Baylor University, Waco, TX 76706, USA

Department of Mechanical and Aerospace Engineering, Princeton University, Princeton, NJ 08544, USA

Funding

Office of Naval Research · Robert A. Welch Foundation · National Science Foundation

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