journal article·2025-12-18Open access

PLA-Based Films Reinforced with Cellulose Nanofibres from Salicornia ramosissima By-Product with Proof of Concept in High-Pressure Processing

Alexandre R. Lima, Nathana L. Cristofoli, Inès Delahousse, Renata A. Amaral, Jorge A. Saraiva, Margarida C. Vieira

Applied Sciences· Volume 15· Issue 24

Abstract

Biocomposite films based on polylactic acid (PLA) reinforced with cellulose nanofibers (CNFs) extracted from Salicornia ramosissima by-products were developed and characterised using solvent casting (SC) and electrospinning (ES) techniques. The primary objective was to assess their suitability as sustainable food packaging materials that are compatible with high-pressure processing (HPP). The SC films exhibited a transparent, homogeneous morphology with superior ductility and water vapour barrier performance, whereas the ES films displayed a fibrous, porous structure with enhanced tensile strength and rigidity. The incorporation of CNFs significantly improved the mechanical properties, particularly the tensile strength and Young’s modulus, with optimal reinforcement achieved at a loading of 0.5%. Thermal and spectroscopic analyses confirmed the effective integration of CNF without compromising the thermal stability of PLA. Pouch-type packages from CNF-reinforced SC films withstood industrial HPP conditions without rupture or leakage, demonstrating their technical feasibility for food packaging applications. This study presents the first demonstration of Salicornia ramosissima by-product valorisation for CNF production and its application in HPP-compatible food packaging, addressing both circular economy goals and emerging food processing technologies.
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Research context

OpenAlex topics: Advanced Cellulose Research Studies · Nanocomposite Films for Food Packaging · Electrospun Nanofibers in Biomedical Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

MED—Mediterranean Institute for Agriculture, Environment and Development & CHANGE—Global Change and Sustainability Institute, Faculty of Sciences and Technology, Campus de Gambelas, Universidade do Algarve, 8005-139 Faro, Portugal

LAQV–REQUIMTE—Associated Laboratory for Green Chemistry of the Network of Chemistry and Technology, Department of Chemistry, Universidade de Aveiro, 3810-193 Aveiro, Portugal

GreenCoLab—Associação Oceano Verde, Universidade do Algarve, 8005-139 Faro, Portugal

L’Institut Agro Dijon, Université Bourgogne Franche Comté, 26 Bd Docteur Petitjean—BP 87999, 21079 Dijon, France

ISE—High Institute of Engineering, Department of Food Engineering, Campus da Penha, Universidade do Algarve, 8000-139 Faro, Portugal

Funding

R&D unit MED—Mediterranean Institute for Agriculture, Environment and Development · Associate Laboratory CHANGE—Global Change and Sustainability Institute · Laboratório Associado para a Química Verde—66 e Processos Limpos · Portuguese Foundation for Science and Technology (FCT) through FCT PhD grants

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