Multi-Objective Optimization of CO2 Sequestration in Heterogeneous Saline Aquifers under Geological Uncertainty

This paper presents a Pareto-based multi-objective optimization for operating CO2 sequestration with a multi-well system under geological uncertainty; the optimal well allocation, i.e., the optimal allocation of CO2 rates at injection wells, is obtained when there is minimum operation pressure as well as maximum sequestration efficiency. The distance-based generalized sensitivity analysis evaluates the influence of geological uncertainty on the amount of CO2 sequestration through four injection wells at 3D heterogeneous saline aquifers. The spatial properties significantly influencing the trapping volume, in descending order of influence, are mean sandstone porosity, mean sandstone permeability, shale volume ratio, and the Dykstra–Parsons coefficient of permeability. This confirms the importance of storable capacity and heterogeneity in quantitatively analyzing the trapping mechanisms. Multi-objective optimization involves the use of two aquifer models relevant to heterogeneity; one is highly heterogeneous and the other is less so. The optimal well allocations converge to non-dominated solutions and result in a large injection through one specific well, which generates the wide spread of a highly mobile CO2 plume. As the aquifer becomes heterogeneous with a large shale volume and a high Dykstra–Parsons coefficient, the trapping performances of the combined structural and residual sequestration plateau relatively early. The results discuss the effects of spatial heterogeneity on achieving CO2 geological storage, and they provide an operation strategy including multi-objective optimization.