journal article·2020-02-07Open access

A Carbon Nanotube Packed Bed Electrode for Small Molecule Electrosorption: An Electrochemical and Chromatographic Approach for Process Description

Tatjana Trunzer, Timothy Stummvoll, Melanie Porzenheim, Paula Fraga-García, Sonja Berensmeier

Applied Sciences· Volume 10· Issue 3

Abstract

Triggering the interaction of nanomaterials with molecules by means of electrical potentials in aqueous media remains challenging, especially if 3D through-flow systems are used as electrodes, as in potential-controlled liquid chromatography (PCC). In this paper, multi-walled carbon nanotubes (MWCNTs) function as a particulate packed bed electrode in order to study the system’s response to various applied potentials and electrolyte compositions. The process principle was analyzed using chronoamperometry and cyclic voltammetry. Applying an electrical potential to the hydrophilic MWCNTs induces the presence of both capacitive and faradaic currents. This leads, over time, to a degradation of the electrode due to structural changes of the MWCNT matrix and an increase in redox reactions on the surface. The role of the electrochemical double layer (EDL) is highlighted as a main player in the process, directly influencing the adsorption capability of the electrode. The EDL rearrangement time and coverage radius depend on the composition of the mobile phase and on the potential applied. The capacity of the electrode for the target (maleic acid) increases at high positive potentials (+800 mV vs. Ag/AgCl), while the presence of electrolytes leads to a capacity decrease. Our research enhances the understanding of capacitive through-flow cells.
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Research context

OpenAlex topics: Electrochemical Analysis and Applications · Microfluidic and Capillary Electrophoresis Applications · Electrochemical sensors and biosensors

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Bioseparation Engineering Group, Department of Mechanical Engineering, Technical University of Munich, 85748 Garching, Germany

Funding

Bundesministerium für Bildung und Forschung

References (68)

Show source-provided references
1. Electrolytic chromatography and coulometric detection with the column electrode10.1351/pac197125040709 ↗
2. Electrolytic chromatography and coulopotentiography—A rapid electrolysis at the column electrode used for the preparation, separation, concentration, and estimation of trace and/or unstable substances10.1080/10408347708085589 ↗
3. Electrosorption and separation of quinones on a column of graphite particles10.1021/ac60321a012 ↗
4. Deinhammer, R.S. (1994). The development of novel chromatographic systems utilizing charge-controllable stationary phases for optimization of separation in liquid chromatography. [Ph.D. Thesis, Iowa State University].
5. Electrochemical separation of ionic compounds using a conductive stationary phase coated with polyaniline or polypyrrole film, and ion exchange properties of conductive polymers10.1016/0022-0728(93)02913-3 ↗
6. Electrochemically modulated liquid chromatographic separations of inorganic anions10.1016/j.chroma.2004.10.004 ↗
7. Yakes, B.J., Keller, D.W., and Porter, M.D. (2010). Electrochemically modulated liquid chromatographic separation of triazines and the effect of pH on retention. J. Chrom. A, 4395–4401.10.1016/j.chroma.2010.04.031 ↗
8. Fundamental studies on the electrolysis with the glassy carbon column electrode10.5189/revpolarography.15.154 ↗
9. Electrochromatography using high applied voltage10.1021/ac00130a032 ↗
10. Separations of benzodiazepines using electrochemically modulated liquid chromatography10.1016/S0021-9673(97)00855-8 ↗
11. Separations of corticosteroids using electrochemically modulated liquid chromatography: Selectivity enhancements at a porous graphitic carbon stationary phase10.1021/ac960880t ↗
12. Electrochromatography—a preliminary study of the effect of applied potential on a carbonaceous chromatographic column10.1016/S0003-2670(00)85641-X ↗
13. The effect of supporting electrolytes in electrochromatography10.1080/00032718808071934 ↗
14. Characterization of novel conducting polymeric stationary phases and electrochemically controlled high-performance liquid chromatography10.1021/ac00196a014 ↗
15. Porter, M.D., and Takano, H. (2000). Electrochemically modulated liquid chromatography. Chromatography II, 636–646.10.1016/B0-12-226770-2/04311-8 ↗
16. Electrochemically modulated liquid chromatography (EMLC): A new approach to gradient elution separations10.1016/0022-0728(93)80034-F ↗
17. Electrochemically modulated liquid chromatography (EMLC) as a probe of the adsorption characteristics of monosubstituted benzenes at porous graphitic carbon10.1016/S0022-0728(97)00551-2 ↗
18. Electrochemically modulated liquid chromatography: An electrochemical strategy for manipulating chromatographic retention10.1039/b105249g ↗
19. Effects of electrolytes on manipulation of the stationary phase in electrochemically modulated liquid chromatography10.1080/00032719808005256 ↗
20. Investigation of adsorption thermodynamics at electrified liquid–solid interfaces by electrochemically modulated liquid chromatography10.1021/acs.jpcc.9b07717 ↗
21. Electrochemically modulated liquid chromatography in fused silica capillary columns10.1021/acs.analchem.9b03581 ↗
22. Dynamic elution control in electrochemical ion chromatography using pulse perturbation of stationary phase potential10.1016/0022-0728(94)03400-1 ↗
23. Electrochemically modulated liquid chromatography using a boron-doped diamond particle stationary phase10.1016/j.chroma.2008.09.069 ↗
24. Assessment of supporting electrolyte contributions in electrochemically modulated liquid chromatography10.1016/j.chroma.2005.06.082 ↗
25. Effect of electrolytes on the retention behavior of some benzenesulfonates in electrochemically modulated liquid chromatography10.1016/S0039-9140(98)00107-6 ↗
26. Potential-controlled chromatography of short-chain carboxylic acids10.1002/elan.200390004 ↗
27. Potential-controlled chromatography for the separation of amino acids and peptides10.1007/s10800-005-9034-6 ↗
28. Brammen, M., Fraga-Garcia, P., and Berensmeier, S. (2016). Carbon nanotubes-A resin for electrochemically modulated liquid chromatography. J. Sep. Sci., 1–9.
29. Analytical application of carbon nanotubes, fullerenes and nanodiamonds in nanomaterials-based chromatographic stationary phases: A review10.1016/j.aca.2013.03.041 ↗
30. Incorporation of single-wall carbon nanotubes into an organic polymer monolithic stationary phase for mu-HPLC and capillary electrochromatography10.1021/ac048299h ↗
31. Single-wall carbon nanotubes used as stationary phase in HPLC10.1080/10826070701589057 ↗
32. Single-walled carbon nanotubes for improved enantioseparations on a chiral ionic liquid stationary phase in GC10.1007/s00216-010-4079-8 ↗
33. A novel stationary phase based on amino derivatized nanotubes for HPLC separations: Theoretical and practical aspects10.1002/jssc.200800683 ↗
34. Carbon nanotubes paste electrode10.1016/S1388-2481(03)00168-1 ↗
35. Ion-separation and water-purification using single-walled carbon nanotube electrodes10.1016/j.desal.2011.04.028 ↗
36. Carbon electrodes for capacitive technologies10.1016/j.ensm.2018.04.031 ↗
37. Electrochemical properties of nitrogen-doped carbon nanotube anode in Li-ion batteries10.1016/j.carbon.2011.05.043 ↗
38. Saeed, K., and Kahn, I. (2013). Carbon nanotubes - properties and applications: A review. Carbon letters, 131–144.10.5714/CL.2013.14.3.131 ↗
39. Carbon nanotubes for biological and biomedical application10.1088/0957-4484/18/41/412001 ↗
40. Sensors and actuators based on carbon nanotubes and their composites: A review10.1016/j.compscitech.2008.01.006 ↗
41. Carbon nanotubes: Past, present, and future10.1016/S0921-4526(02)00869-4 ↗
42. High-energy and high-power nonaqueous lithium-ion capacitors based on polypyrrole/carbon nanotube composites as pseudocapacitive cathodes10.1021/acsami.9b02781 ↗
43. Three-dimensional ordered porous electrode materials for electrochemical energy storage10.1038/s41427-019-0112-3 ↗
44. Reactor concepts for bioelectrochemical syntheses and energy conversion10.1016/j.tibtech.2014.10.004 ↗
45. Cyclic voltammogram profile of single-walled carbon nanotube electric double-layer capacitor electrode reveals dumbbell shape10.1021/jp300802z ↗
46. Kaempgen, M. (2006). Eigenschaften und Anwendungen von Netzwerken aus Kohlenstoff-Nanoröhren. [Ph.D. Thesis, Universität Stuttgart].
47. Specific surface area of carbon nanotubes and bundles of carbon nanotubes10.1016/S0008-6223(00)00155-X ↗
48. Properties that influence the specific surface areas of carbon nanotubes and nanofibers
49. Supercapacitor electrodes from multiwalled carbon nanotubes10.1063/1.1290146 ↗
50. Super-hydrophobicity of large-area honeycomb-like aligned carbon nanotubes10.1021/jp0209401 ↗
51. Generation of hydrophilic, bamboo-shaped multiwalled carbon nanotubes by solid-state pyrolysis and its electrochemical studies10.1021/jp055749g ↗
52. In situ chemical experiments in carbon nanotubes10.1016/S0009-2614(02)01496-3 ↗
53. Electrochemical oxidation of multi-walled carbon nanotubes and its application to electrochemical double layer capacitors10.1016/j.elecom.2005.01.008 ↗
54. Potential-controlled tensiometry: A tool for understanding wetting and surface properties of conductive powders by electroimbibition10.1021/acs.analchem.8b03475 ↗
55. Superstable ultrathin water film confined in a hydrophilized carbon nanotube10.1021/acs.nanolett.7b05169 ↗
56. Multi-walled carbon nanotubes: Innovative sorbents for pre-concentration of polychlorinated biphenyls in aqueous environments10.1039/C5AY01496D ↗
57. Carbon Nanotubes Functionalized in Oxygen and Water Low Pressure Discharges used as Reinforcement of Polyurethane Composites
58. Characterization of multiwalled carbon nanotubes dispersing in water and association with biological effects
59. Chromatographic behaviour of oxidised porous graphitic carbon columns10.1039/B303076H ↗
60. Helical crystallization of proteins on carbon nanotubes: A first step towards the development of new biosensors10.1002/(SICI)1521-3773(19990712)38:13/14<1912::AID-ANIE1912>3.0.CO;2-2 ↗
61. Electrochemical properties of single-wall carbon nanotube electrodes10.1149/1.1593045 ↗
62. Electrochemical processing of discrete single-walled carbon nanotube anions10.1021/nn305919p ↗
63. On-column electrochemical redox derivatization for enhancement of separation selectivity of liquid chromatography use of redox reaction as secondary chemical equilibrium10.1016/j.chroma.2007.12.003 ↗
64. Alignment of carbon nanotubes in carbon nanotube fibers through nanoparticles: A route for controlling mechanical and electrical properties10.1021/acsami.6b12869 ↗
65. Electrochemical characterization of multi-walled carbon nanotube coated electrodes for biological applications10.1016/j.carbon.2008.11.045 ↗
66. Electrosorption of anions with carbon nanotube and nanofibre composite film electrodes10.1016/j.desal.2008.05.019 ↗
67. Electrochemical characterization of carbon nanotubes as electrode in electrochemical double-layer capacitors10.1016/S0008-6223(01)00266-4 ↗
68. Review of nanostructured carbon materials for electrochemical capacitor applications: Advantages and limitations of activated carbon, carbide-derived carbon, zeolite-templated carbon, carbon aerogels, carbon nanotubes, onion-like carbon, and graphene10.1002/wene.102 ↗