journal article·2022-11-19Open access

Dual Stimuli-Responsive Polysaccharide Hydrogels Manufactured by Radiation Technique

Radoslaw A. Wach, Giorgia Palmeri, Agnieszka Adamus-Wlodarczyk, Bozena Rokita, Alicja K. Olejnik, Clelia Dispenza, Piotr Ulanski

Applied Sciences· Volume 12· Issue 22

Abstract

This paper describes the results of the radiation-induced crosslinking of polysaccharides modified with hydroxypropyl and carboxymethyl functional groups, hydroxypropylcellulose (HPC) and carboxymethylcellulose (CMC), respectively, without and with poly(ethylene glycol) diacrylate (PEGDA) as a crosslinking agent, to obtain dual stimuli-responsive hydrogels. The gels were characterized in terms of water uptake and gel fraction, parameters that mainly depend on the HPC–CMC compositions, but also on the macromer crosslinker content and the absorbed dose. The swelling of hydrogels is controlled by both the temperature, due to the amphiphilic character of HPC and pH, due to the anionic functional groups of CMC. In spite of a similar degree of substitution in both cellulose derivatives, 1.4 for HPC and 1.2 for CMC, the pH response of hydrogels with an equal content of both polysaccharides is considerably higher—a reduction in swelling of up to 95% with a decrease in the pH to 2 was recorded—than the response to thermal-stimulus—wherein a reduction in swelling of less than 70% with an increasing in temperature to 55 °C was found. These biopolymers-based hydrogels of specific, stimuli-responsive swelling properties are anticipated in applications where a combination of two stimuli is essential and biodegradation may be required.
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Research context

OpenAlex topics: Hydrogels: synthesis, properties, applications · Electrospun Nanofibers in Biomedical Applications · 3D Printing in Biomedical Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Institute of Applied Radiation Chemistry, Faculty of Chemistry, Lodz University of Technology, 93-590 Lodz, Poland

Dipartimento di Ingegneria, Università degli Studi di Palermo, 90128 Palermo, Italy

Funding

International Atomic Energy Agency (IAEA)

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