journal article·2026-06

Impact of nanocrystal parameters on the threshold hydrostatic pressure for driving ordered coalescence in gold supercrystals

Xuepeng Liu, Chengheng Ling

Applied Physics A· Volume 132· Issue 6
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Abstract

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OpenAlex topics: Gold and Silver Nanoparticles Synthesis and Applications · Luminescence and Fluorescent Materials · Quantum Dots Synthesis And Properties

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References (58)

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1. I. Coropceanu, E.M. Janke, J. Portner et al., Self-assembly of nanocrystals into strongly electronically coupled all-inorganic supercrystals. Science 375, 1422–1426 (2022). https://doi.org/10.1126/science.abm675310.1126/science.abm6753 ↗
2. C.L. Bassani, G. Anders, U. Banin et al., Nanocrystal assemblies: current advances and open problems. ACS Nano 18, 14791–14840 (2024). https://doi.org/10.1021/acsnano.3c1020110.1021/acsnano.3c10201 ↗
3. S. Wan, X. Xia, Y. Gao et al., Curvature-guided depletion stabilizes Kagome superlattices of nanocrystals. Science 387, 978–984 (2025). https://doi.org/10.1126/science.adu412510.1126/science.adu4125 ↗
4. M.A. Boles, D. Ling, T. Hyeon, D.V. Talapin, The surface science of nanocrystals. Nature Materials 15, 141–153 (2016). https://doi.org/10.1038/NMAT452610.1038/NMAT4526 ↗
5. E.V. Shevchenko, D.V. Talapin, N.A. Kotov, S. O’Brien, C.B. Murray, Structural diversity in binary nanoparticle superlattices. Nature 439, 55–59 (2006). https://doi.org/10.1038/nature0441410.1038/nature04414 ↗
6. A. Dong, J. Chen, P.M. Vora, J.M. Kikkawa, C.B. Murray, Binary nanocrystal superlattice membranes self-assembled at the liquid-air interface. Nature. 466, 474–477 (2010). https://doi.org/10.1038/nature0918810.1038/nature09188 ↗
7. E. Marino, R.A. LaCour, T.C. Moore et al., Crystallization of binary nanocrystal superlattices and the relevance of short-range attraction. Nat. Synth. 3, 111–122 (2024). https://doi.org/10.1038/s44160-023-00407-210.1038/s44160-023-00407-2 ↗
8. Y. Nagaoka, R. Tan, R. Li et al., Superstructures generated from truncated tetrahedral quantum dots. Nature 561, 378–382 (2018). https://doi.org/10.1038/s41586-018-0512-510.1038/s41586-018-0512-5 ↗
9. Y. Zhang, D.D. Xu, I. Tanriover et al., Nonlinear optical colloidal metacrystals. Nat. Photonics 19, 20–27 (2025). https://doi.org/10.1038/s41566-024-01558-010.1038/s41566-024-01558-0 ↗
10. X. Lan, M. Chen, M.H. Hudson et al., Quantum dot solids showing state-resolved band-like transport. Nat. Mater. 19, 323–329 (2020). https://doi.org/10.1038/s41563-019-0582-210.1038/s41563-019-0582-2 ↗
11. D.V. Talapin, E.V. Shevchenko, C.B. Murray, A.V. Titov, P. Král, Dipole-dipole interactions in nanoparticle superlattices. Nano Lett. 7, 1213–1219 (2007). https://doi.org/10.1021/nl070058c10.1021/nl070058c ↗
12. S. Dhulipala, D.W. Yee, Z. Zhou et al., Tunable mechanical response of self-assembled nanoparticle superlattices. Nano Lett. 23, 5155–5163 (2023). https://doi.org/10.1021/acs.nanolett.3c0105810.1021/acs.nanolett.3c01058 ↗
13. F.P. García de Arquer, D.V. Talapin, V.I. Klimov, Y. Arakawa, M. Bayer, E.H. Sargent, Semiconductor quantum dots: technological progress and future challenges. Science 373, eaaz8541 (2021). https://doi.org/10.1126/science.aaz854110.1126/science.aaz8541 ↗
14. J. Kim, Q. Zhao, I. Choi et al., Ensemble hot-spots in 3D supercrystals of plasmonic octahedral nanoparticles in tip-to-tip configured superlattices. Nat. Commun. 16, 2762 (2025). https://doi.org/10.1038/s41467-025-58029-510.1038/s41467-025-58029-5 ↗
15. S. Sun, M. Lu, P. Lu et al., Perovskite nanocrystal superlattices and their application in light-emitting devices. Mater. Sci. Eng. R. Rep. 164, 100984 (2025). https://doi.org/10.1016/j.mser.2025.10098410.1016/j.mser.2025.100984 ↗
16. W. Wei, F. Bai, H. Fan, Oriented gold nanorod arrays: self-assembly and optoelectronic applications. Angew. Chem. Int. Ed. Engl. 58, 11956–11966 (2019). https://doi.org/10.1002/anie.20190262010.1002/anie.201902620 ↗
17. F. Bai, K. Bian, X. Huang, Z. Wang, H. Fan, Pressure induced nanoparticle phase behavior, property, and applications. Chem. Rev. 119, 7673–7717 (2019). https://doi.org/10.1021/acs.chemrev.9b0002310.1021/acs.chemrev.9b00023 ↗
18. H. Wu, F. Bai, Z. Sun et al., Pressure-driven assembly of spherical nanoparticles and formation of 1D‐nanostructure arrays. Angew. Chem. Int. Ed. 49, 8431–8434 (2010). https://doi.org/10.1002/ange.20100158110.1002/ange.201001581 ↗
19. B. Li, X. Wen, R. Li et al., Stress-induced phase transformation and optical coupling of silver nanoparticle superlattices into mechanically stable nanowires. Nat. Commun. 5, 4179 (2014). https://doi.org/10.1038/ncomms517910.1038/ncomms5179 ↗
20. J. Zhu, Z. Quan, C. Wang et al., Structural evolution and mechanical behaviour of Pt nanoparticle superlattices at high pressure. Nanoscale 8, 5214 (2016). https://doi.org/10.1039/c5nr08291a10.1039/c5nr08291a ↗
21. B. Li, K. Bian, J.M.D. Lane et al., Superfast assembly and synthesis of gold nanostructures using nanosecond low-temperature compression via magnetic pulsed power. Nat. Commun. 8, 14778 (2017). https://doi.org/10.1038/ncomms1477810.1038/ncomms14778 ↗
22. B. Li, K. Bian, X. Zhou et al., Pressure compression of CdSe nanoparticles into luminescent nanowires. Sci. Adv. 3, e1602916 (2017). https://doi.org/10.1126/sciadv.160291610.1126/sciadv.1602916 ↗
23. K.J. Si, Y. Chen, Q. Shi, W. Cheng, Nanoparticle superlattices: the roles of soft ligands. Adv. Sci. 5, 1700179 (2018). https://doi.org/10.1002/advs.20170017910.1002/advs.201700179 ↗
24. K.M. Salerno, D.S. Bolintineanu, J.M.D. Lane, G.S. Grest, High strength, molecularly thin nanoparticle membranes. Phys. Rev. Lett. 113, 258301 (2014). https://doi.org/10.1103/PhysRevLett.113.25830110.1103/PhysRevLett.113.258301 ↗
25. A.P. Kaushik, P. Clancy, Explicit all-atom modeling of realistically sized ligand-capped nanocrystals. J. Chem. Phys. 136, 114702 (2012). https://doi.org/10.1063/1.368997310.1063/1.3689973 ↗
26. W.D. Luedtke, U. Landman, Structure, dynamics, and thermodynamics of passivated gold nanocrystallites and their assemblies. J. Phys. Chem. 100, 13323–13329 (1996). https://doi.org/10.1021/jp961721g10.1021/jp961721g ↗
27. U. Landman, W.D. Luedtke, Small is different: energetic, structural, thermal, and mechanical properties of passivated nanocluster assemblies. Faraday Discuss. 125, 1–22 (2004). https://doi.org/10.1039/B312640B10.1039/B312640B ↗
28. X. Liu, P. Lu, H. Zhai, Ligand coverage dependence of structural stability and interparticle spacing of gold supracrystals. J. Appl. Phys. 123, 045101 (2018). https://doi.org/10.1063/1.500509410.1063/1.5005094 ↗
29. X.P. Liu, Y. Ni, L.H. He, Molecular dynamics simulation of interparticle spacing and many-body effect in gold supracrystals. Nanotechnology 27, 135707 (2016). https://doi.org/10.1088/0957-4484/27/13/13570710.1088/0957-4484/27/13/135707 ↗
30. A.P. Kaushik, P. Clancy, Solvent-driven symmetry of self‐assembled nanocrystal superlattices-a computational study. J. Comput. Chem. 34, 523–532 (2013). https://doi.org/10.1002/jcc.2315210.1002/jcc.23152 ↗
31. M.B. Zanjani, J.R. Lukes, Size dependent elastic moduli of CdSe nanocrystal superlattices predicted from atomistic and coarse grained models. J. Chem. Phys. 139, 144702 (2013). https://doi.org/10.1063/1.482203910.1063/1.4822039 ↗
32. X.P. Liu, Y. Ni, L.H. He, Elastic properties of gold supracrystals: effects of nanocrystal size, ligand length, and nanocrystallinity. J. Chem. Phys. 144, 144507 (2016). https://doi.org/10.1063/1.494602910.1063/1.4946029 ↗
33. X. Liu, K. Xu, Y. Ni et al., Strain-dependent elastic asymmetry of alkylthiol-coated gold superlattices: an atomistic molecular dynamics study. J. Appl. Phys. 132, 075104 (2022). https://doi.org/10.1063/5.009134510.1063/5.0091345 ↗
34. J. Lequieu, A. Córdoba, D. Hinckley, J.J. de Pablo, Mechanical response of DNA–nanoparticle crystals to controlled deformation. ACS Cent. Sci. 2, 614–620 (2016). https://doi.org/10.1021/acscentsci.6b0017010.1021/acscentsci.6b00170 ↗
35. M.B. Zanjani, J.R. Lukes, Phonon dispersion and thermal conductivity of nanocrystal superlattices using three-dimensional atomistic models. J. Appl. Phys. 115, 143515 (2014). https://doi.org/10.1063/1.487094310.1063/1.4870943 ↗
36. M.B. Zanjani, J.R. Lukes, Shape-and structure-based phonon bandgap tuning with nanocrystal superlattices. J. Phys. Chem. C 119, 16889–16896 (2015). https://doi.org/10.1021/acs.jpcc.5b0113210.1021/acs.jpcc.5b01132 ↗
37. X. Liu, P. Lu, H. Zhai, F. Xie, Molecular insights into the thermal stability of gold superlattices. Nanotechnology 31, 085704 (2019). https://doi.org/10.1088/1361-6528/ab546d10.1088/1361-6528/ab546d ↗
38. K.M. Salerno, G.S. Grest, Temperature effects on nanostructure and mechanical properties of single-nanoparticle thick membranes. Faraday Discuss. 181, 339–354 (2015). https://doi.org/10.1039/C4FD00249K10.1039/C4FD00249K ↗
39. W.L. Ong, S. Majumdar, J.A. Malen, A.J.H. McGaughey, Coupling of organic and inorganic vibrational states and their thermal transport in nanocrystal arrays. J. Phys. Chem. C 118, 7288–7295 (2014). https://doi.org/10.1021/jp412015710.1021/jp4120157 ↗
40. W. Li, H. Fan, J. Li, Deviatoric stress-driven fusion of nanoparticle superlattices. Nano Lett. 14, 4951–4958 (2014). https://doi.org/10.1021/nl501197710.1021/nl5011977 ↗
41. X. Liu, Y. Wu, G. Li, Y. Zhang, H. Zhai, Structural evolution and fusion behavior of gold supercrystals under stress: insights from atomistic simulations. J. Appl. Phys. 128, 035109 (2020). https://doi.org/10.1063/5.001244510.1063/5.0012445 ↗
42. J.M.D. Lane, K.M. Salerno, I. Srivastava, G.S. Grest, H. Fan, (2018) Modeling pressure-driven assembly of polymer coated nanoparticles. AIP Conf. Proc. 1979:090007 https://doi.org/10.1063/1.504486410.1063/1.5044864 ↗
43. P. Podsiadlo, B. Lee, V.B. Prakapenka et al., High-pressure structural stability and elasticity of supercrystals self-assembled from nanocrystals. Nano Lett. 11, 579–588 (2011). https://doi.org/10.1021/nl103587u10.1021/nl103587u ↗
44. C. Yan, I. Arfaoui, N. Goubet, M.P. Pileni, Soft supracrystals of Au nanocrystals with tunable mechanical properties. Adv. Funct. Mater. 23, 2315–2321 (2013). https://doi.org/10.1002/adfm.20120256310.1002/adfm.201202563 ↗
45. M. Gauvin, N. Yang, E. Barthel et al., Morphology, nanocrystallinity, and elastic properties of single domain ε-Co supracrystals. J. Phys. Chem. C 119, 7483–7490 (2015). https://doi.org/10.1021/acs.jpcc.5b0035810.1021/acs.jpcc.5b00358 ↗
46. J.E. Martin, J.P. Wilcoxon, J. Odin, P. Provencio, Control of the interparticle spacing in gold nanoparticle superlattices. J. Phys. Chem. B 104, 9475–9486 (2000). https://doi.org/10.1021/jp001292t10.1021/jp001292t ↗
47. S. Plimpton, Fast parallel algorithms for short-range molecular dynamics. J. Comput. Phys. 117, 1–19 (1995). https://doi.org/10.1006/jcph.1995.103910.1006/jcph.1995.1039 ↗
48. A. Stukowski, Visualization and analysis of atomistic simulation data with OVITO–the Open Visualization Tool. Modell. Simul. Mater. Sci. Eng. 18, 015012 (2009). https://doi.org/10.1088/0965-0393/18/1/01501210.1088/0965-0393/18/1/015012 ↗
49. O.H. Nielsen, R.M. Martin, Quantum-mechanical theory of stress and force. Phys. Rev. B 32, 3780–3791 (1985). https://doi.org/10.1103/PhysRevB.32.378010.1103/PhysRevB.32.3780 ↗
50. X. Liu, Z. Zhang, Ligand length dependence of critical deviatoric stress required for the formation of ordered nanowire arrays in alkylthiol-capped gold superlattices. Nanotechnology 37, 025701 (2026). https://doi.org/10.1088/1361-6528/ae308d10.1088/1361-6528/ae308d ↗
51. P. Schapotschnikow, R. Pool, T.J.H. Vlugt, Molecular simulations of interacting nanocrystals. Nano Lett. 8, 2930–2934 (2008). https://doi.org/10.1021/nl801786210.1021/nl8017862 ↗
52. M. Parrinello, Strain fluctuations and elastic constants. J. Chem. Phys. 76, 2662–2666 (1982). https://doi.org/10.1063/1.44324810.1063/1.443248 ↗
53. W.M. Haynes, CRC Handbook of Chemistry and Physics. CRC Press. 97, 2670 (2016). https://doi.org/10.1201/978131538047610.1201/9781315380476 ↗
54. H. Ibrahim, V. Balédent, M. Impéror-Clerc, B. Pansu, Mechanics under pressure of gold nanoparticle supracrystals: the role of the soft matrix. RSC Adv. 12, 23675–23679 (2022). https://doi.org/10.1039/D2RA03484K10.1039/D2RA03484K ↗
55. X. Liu, P. Lu, H. Zhai, Molecular interaction between asymmetric ligand-capped gold nanocrystals. J. Chem. Phys. 150, 034702 (2019). https://doi.org/10.1063/1.506547610.1063/1.5065476 ↗
56. X. Liu, Y. Ni, L. He, Interaction between capped tetrahedral gold nanocrystals: dependence on effective softness. Soft Matter. 15, 8392–8401 (2019). https://doi.org/10.1039/c9sm01389j10.1039/c9sm01389j ↗
57. K.E. Mueggenburg, X.M. Lin, R.H. Goldsmith, H.M. Jaeger, Elastic membranes of close-packed nanoparticle arrays. Nat. Mater. 6, 656–660 (2007). https://doi.org/10.1038/nmat196510.1038/nmat1965 ↗
58. I. Robel, X.M. Lin, M. Sprung, J. Wang, Thermal stability of two-dimensional gold nanocrystal superlattices. J. Phys. Condens. Matter 21, 264011 (2009). https://doi.org/10.1088/0953-8984/21/26/26401110.1088/0953-8984/21/26/264011 ↗