Three-way metal cluster catalysts confined in zeolites produced by pulsed laser ablation in liquid
Source abstract
Abstract
We synthesized three-way catalysts consisting of rhodium, platinum, or palladium clusters confined in zeolites produced by pulsed laser ablation (LA) in liquid acetone. A plate of the catalytic metals was irradiated with a pulsed laser in an acetone suspension of zeolite powder. The catalytic properties of the samples were evaluated for the three-way reaction, CO oxidation reaction, and NO–CO reaction. The zeolite-confined clusters generated by LA had higher thermal stability than those supported on α-Quartz (αQ) particles produced by LA. The cluster size matched those of the pores, resulting in a large contact area with the surface of the pores. Therefore, the metal clusters supported by zeolite were efficiently stabilized in the zeolite pores by a larger number of Rh–O–Si bonds than those supported on αQ particles produced by LA. Moreover, the zeolite-confined clusters generated by LA had higher catalytic activity than clusters on zeolite produced by traditional metal-ion exchange followed by reduction.
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Research context
OpenAlex topics: Catalytic Processes in Materials Science · Laser-Ablation Synthesis of Nanoparticles · Catalysis and Oxidation Reactions
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References (32)
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