Additive manufacturing of polymer composites: Sustainability, recycling, life cycle, safety and environmental perspectives
Source abstract
Abstract
Additive manufacturing (AM) enables the fabrication of complex and customised, on-demand products from various materials across multiple industries in aerospace, automotive, Industry 4.0, and biomedical domains. Advancing material development, improving process efficiency, and ensuring sustainable waste management are crucial for AM to achieve its full capability as a sustainable technology. This review focuses on the recent progress in AM of polymer composites by 3D and 4D printing techniques. Their sustainability, environmental, recycling, lifecycle assessments (LCA), safety, and economic impacts have been systematically reviewed. The effect of incorporating eco-friendly materials in the manufacturing of polymer composites to enable a sustainable future has also been evaluated. The sustainability of additively manufactured polymer composites is evaluated from a social, environmental, and economic perspective. By using recycled materials in the AM processes, the environmental impact can be reduced, circularity promoted, and resources conserved. The challenges of AM techniques regarding scalability, including slow printing speeds, cost limitations, and health and environmental concerns due to the emission of toxic matter and compounds, have been addressed. It also provides a perspective on the potential role of AM in promoting sustainability and circular economic practices for a greener future.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Additive Manufacturing and 3D Printing Technologies · Innovations in Concrete and Construction Materials · Polymer Foaming and Composites
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (100+)
Show source-provided references
1. 3D printing of polymer matrix composites: a review and prospective10.1016/j.compositesb.2016.11.034 ↗
2. Rapid manufacturing and rapid tooling with layer manufacturing (LM) technologies, state of the art and future perspectives10.1016/S0007-8506(07)60206-6 ↗
3. Additive manufacturing: toward holistic design10.1016/j.scriptamat.2017.02.029 ↗
4. Biodegradable polymers for biomedical additive manufacturing
5. Significant potential and materials used in additive manufacturing technologies towards sustainability
6. Life cycle assessment of additive manufacturing processes: a review10.1016/j.jmsy.2023.05.007 ↗
7. Applications of additive manufacturing (AM) in sustainable energy generation and battle against COVID-19 pandemic: The knowledge evolution of 3D printing10.1016/j.jmsy.2021.07.023 ↗
8. Chapter 3 - Classification of 3D printing methods
9. Material extrusion additive manufacturing of multifunctional sandwich panels with load-bearing and acoustic capabilities for aerospace applications
10. Shear-driven solid-state additive manufacturing of aerospace aluminum on impurity contaminated surfaces10.1016/j.matdes.2025.114312 ↗
11. Defect-Driven topology optimization for fatigue design of additive manufacturing structures: Application on a real industrial aerospace component10.1016/j.engfailanal.2022.106737 ↗
12. Ultrasonic rolling-enhanced additive manufacturing of IN718 superalloy: Microstructural refinement and mechanical property improvement through variable power modulation
13. Additive manufacturing of polypropylene micro and nano composites through fused filament fabrication for automotive repair applications10.1002/pat.5952 ↗
14. Sustainable supply chain: An optimization and resource efficiency in additive manufacturing for automotive spare part10.1016/j.sftr.2025.100563 ↗
15. Additive manufacturing for the automotive industry: on the life-cycle environmental implications of material substitution and lightweighting through re-design10.1007/s40964-023-00395-x ↗
16. The Implementation of Additive Technologies in the Army and Key Personnel Training
17. Additive manufacturing of multidimensional Al/PVDF-based energetic composite structures featuring enhanced safety and combustion performance10.1016/j.jiec.2024.03.007 ↗
18. Enhanced engineering and biocidal polypropylene filaments enabling melt reduction of AgNO3 through PVP agent: A scalable process for the defense industry with MEX additive manufacturing10.1016/j.dt.2024.09.007 ↗
19. Multifunctional HDPE/Cu biocidal nanocomposites for MEX additive manufactured parts: Perspectives for the defense industry10.1016/j.dt.2024.03.004 ↗
20. 3D-printed cellulose nanocrystals and gelatin scaffolds with bioactive cues for regenerative medicine: Advancing biomedical applications10.1016/j.ijbiomac.2024.134402 ↗
21. Machine learning-based design for additive manufacturing in biomedical engineering10.1016/j.ijmecsci.2023.108828 ↗
22. Advances in Polylactic acid-based composites as a promising biomaterial for food packaging and biomedical Applications: Reinforcement strategies, functional enhancements, and future research directions
23. Mechanical behaviour of additive manufactured PEEK/HA porous structure for orthopaedic implants: Materials, structures and manufacturing processes10.1016/j.jmbbm.2024.106848 ↗
24. Effect of nozzle diameter and cross-linking on the micro-structure, compressive and biodegradation properties of 3D printed gelatin/collagen/hydroxyapatite hydrogel10.1016/j.bprint.2023.e00266 ↗
25. Predicting the compressive strength of additively manufactured PLA-based orthopedic bone screws: A machine learning framework10.1002/pc.26881 ↗
26. Role of CT and MRI in the design and development of orthopaedic model using additive manufacturing10.1016/j.jcot.2018.07.002 ↗
27. β-spodumene-doped lithium disilicate glass-ceramics via additive manufacturing for dental applications10.1016/j.jmst.2025.04.082 ↗
28. Effect of additive manufacturing process and storage condition on the dimensional accuracy and stability of 3D-printed dental casts10.1016/j.prosdent.2021.02.028 ↗
29. Additive manufacturing of TiO₂-doped 3Y-ZrO₂ ceramics via DLP-3D printing for dental implant applications: Enhanced mechanical strength, biocompatibility, and antibacterial performance10.1016/j.jallcom.2025.182246 ↗
30. Effect of Fe2O3 doping on color and mechanical properties of dental 3Y-TZP ceramics fabricated by stereolithography-based additive manufacturing10.1016/j.ceramint.2022.12.062 ↗
31. 3D Printing and Additive Manufacturing: Recent Trends in Fashion and Textile Production
32. Application of 3D printing cellulose fabrics based on cotton fibers in the textile and fashion industry
33. AI-based additive manufacturing for future food: potential applications, challenges and possible solutions10.1016/j.ifset.2024.103599 ↗
34. On the additive manufacturing (3D printing) of viscoelastic materials and flow behavior: From composites to food manufacturing
35. Additive manufacturing for the food industry10.1016/j.tifs.2015.02.004 ↗
36. 3D printing of biodegradable polymers and their composites – Current state-of-the-art, properties, applications, and machine learning for potential future applications10.1016/j.pmatsci.2024.101336 ↗
37. Advances in 3D printing with eco-friendly materials: a sustainable approach to manufacturing10.1039/D4SU00718B ↗
38. A review on additive manufacturing of polymers composites10.1016/j.matpr.2020.10.490 ↗
39. I.S.O. Astm, ISO/ASTM 52900:2015(en) Additive manufacturing — General principles — Terminology, (n.d.).
40. Investigating impact of five build parameters on the maximum flexural force in FDM specimens – a definitive screening design approach10.1108/RPJ-09-2015-0116 ↗
41. Environmentally friendly polylactic acid/ferronickel slag composite filaments for material extrusion 3D printing: A comprehensive optimization of the filler content
42. Characterization and Performance of Additive Manufactured Novel bio-waste Polylactic acid eco-friendly Composites10.1007/s10924-023-02758-5 ↗
43. Sustainable and eco-friendly 3D printing filament fabricated from different recycled solid wastes and evaluate its impact on interior and furniture design10.1016/j.rineng.2024.102428 ↗
44. Eco-friendly material extrusion 3D printing for fabricating W-Ni-Fe lattices with improved compressive resistance
45. Effect of crystalline Si3N4 fillers on the mechanical strength and thermal stability of complex SiCN(O) ceramic architectures produced by powder bed fusion and densified via polymer infiltration and pyrolysis
46. Mechanical property of powder bed fusion printed carbon fiber reinforced polyetheretherketone and enhanced interlayer strength by post-processing10.1002/pc.28719 ↗
47. Surface modification of oriented glass fibers for improving the mechanical properties and flame retardancy of polyamide 12 composites printed by powder bed fusion
48. Development of low-shrinkage eco-friendly composite materials for the DLP 3D printing technique10.1039/D4MA00722K ↗
49. Eco-friendly, mechanically robust, weather-resistant and rapidly cured polyurea elastomer synthesized by vat photopolymerization 3D printing10.1016/j.compositesa.2025.108985 ↗
50. Bio-based polymer composites obtained by vat photopolymerization of photocurable resins modified with biochar as sustainable filler10.1016/j.compositesa.2025.109102 ↗
51. Biochar-reinforced polyamide 12 composites for sustainable selective laser sintering 3D printing: Performance enhancement and carbon footprint reduction10.1016/j.cej.2025.165502 ↗
52. Influence of particle size on the mechanical performance and sintering quality of peanut husk powder/PES composites fabricated through selective laser sintering10.3390/polym15193913 ↗
53. Selective Laser Sintering of Lignin-Based Composites10.1021/acssuschemeng.0c07996 ↗
54. 3D printing of PBAT-based composites filled with agro-wastes via selective laser sintering10.1016/j.eurpolymj.2024.113197 ↗
55. Rheological properties of gelatine hydrogels affected by flow- and horizontally-induced cooling rates during 3D cryo-printing10.1016/j.colsurfa.2021.126356 ↗
56. Additive manufacturing techniques for designing advanced scaffolds for bone tissue engineering
57. Bio-inspired conductive ink: Harnessing plant based binder for customizing electrochemical, rheological and printing applications
58. Electrochemically synthesized graphene/TEMPO-oxidized cellulose nanofibrils hydrogels: Highly conductive green inks for 3D printing of robust structured EMI shielding aerogels10.1016/j.carbon.2023.118037 ↗
59. Direct Ink Writing as an Eco-Friendly PCB Manufacturing Technique for Rapid Prototyping
60. Direct-Ink-Writing Printing of Shape Memory Cross-Linked Networks from Biomass-Derived Small Molecules10.70322/spe.2024.10008 ↗
61. 3D Printing photo-induced lignin nanotubes/polyurethane shape memory composite10.1016/j.polymertesting.2023.107934 ↗
62. UV-assisted direct ink writing of near-infrared light-responsive shape memory plant-based resin bone scaffold10.1016/j.bioadv.2025.214381 ↗
63. From 3D to 4D printing of lignin towards green materials and sustainable manufacturing10.1039/D4MH01680G ↗
64. J.A. Dicks, C. Woolard, Leveraging Itaconic Acid in Microcrystalline Cellulose Reinforced Shape Memory Photopolymers for Sustainable 4D Printing, Macromol. Mater. Eng. n/a (n.d.) e00227. https://doi.org/https://〈doi.org/10.1002/mame.202500227〉.
65. 4D printed stereolithography printed plant-based sustainable polymers: Preliminary investigation and optimization10.1002/app.50903 ↗
66. 4D Printed Thermoplastic Polyamide Elastomers with Reversible Two-Way Shape Memory Effect10.1002/admt.202202066 ↗
67. 4D Printing of a Fully Biobased Shape Memory Copolyester via a UV-Assisted FDM Strategy10.1021/acssuschemeng.2c00721 ↗
68. Manufacturing of Conductive Filaments for 3D/4D Printing through In Situ Polymerization of Biobased Thermoplastic Polyurethane/Multiwall Carbon Nanotube Composites10.1021/acsapm.3c02558 ↗
69. 3D printing of shape memory poly(d,l-lactide-co-trimethylene carbonate) by direct ink writing for shape-changing structures10.1002/app.48177 ↗
70. 4D printing of multiscale filler–reinforced thermoplastic polyurethane nanocomposites with electro-activated shape memory properties10.1080/17452759.2025.2474537 ↗
71. 4D Printing of Multifunctional and Biodegradable PLA-PBAT-Fe3O4 Nanocomposites with Supreme Mechanical and Shape Memory Properties10.1002/marc.202400661 ↗
72. Co-continuous structure enhanced magnetic responsive shape memory PLLA/TPU blend fabricated by 4D printing10.1080/17452759.2023.2290186 ↗
73. 4D printing of polymers: Techniques, materials, and prospects10.1016/j.progpolymsci.2022.101506 ↗
74. Poly(ethylene terephthalate) glycol/carbon black composites for 4D printing10.1016/j.matchemphys.2024.129737 ↗
75. S. Ali, M. Alshihabi, L. Beard, I. Deiab, S. Pervaiz, Dual-Stimuli Responsive and Sustainable PLA/APHA/TPU Blend for 4D Printing, Macromol. Rapid Commun. n/a (n.d.) e00414. https://doi.org/https://〈doi.org/10.1002/marc.202500414〉.
76. 4D Printing of Multi-Stimuli Responsive Protein-Based Hydrogels for Autonomous Shape Transformations10.1002/adfm.202011012 ↗
77. Polycaprolactone–Itaconic Acid Resins for Additive Manufacturing of Environmentally Degradable 3D and 4D Materials by Thiol-ene Photopolymerization10.1021/acs.macromol.5c01310 ↗
78. Sustainable 4D printable biobased shape memory polymers with linear tunability and multistimuli actuation for advanced applications10.1002/smsc.202500104 ↗
79. 4D printing of polyamide 1212 based shape memory thermoplastic polyamide elastomers by selective laser sintering10.1016/j.jmapro.2023.02.033 ↗
80. Selective laser sintering 4D printing of dynamic cross-linked polyurethane containing Diels–Alder bonds10.1021/acsapm.2c00565 ↗
81. Sustainability performance indicators for additive manufacturing: a literature review based on product life cycle studies10.1007/s00170-020-05249-2 ↗
82. Review of high-performance sustainable polymers in additive manufacturing10.1039/D2GC03474C ↗
83. Sustainability assessment framework of biomedical scaffolds: additive manufacturing versus traditional manufacturing10.1016/j.jclepro.2023.138118 ↗
84. Social life cycle performance of additive manufacturing in the healthcare industry: the orthosis and prosthesis cases10.1080/0951192X.2021.1872100 ↗
85. Research needs and recommendations on environmental implications of additive manufacturing
86. Advancing sustainable practices in additive manufacturing: a comprehensive review on material waste recyclability10.3390/su162310246 ↗
87. Polymeric composites of cubic-octahedron and gyroid lattice for biomimetic dental implants10.1016/j.matchemphys.2022.126454 ↗
88. Evaluating the impact of recycling on polymer of 3D printing for energy and material sustainability10.1016/j.resconrec.2024.107769 ↗
89. Life cycle assessment on fabrication and characterization techniques for additively manufactured polymers and polymer composites
90. Sustainable materials and chemical processes for additive manufacturing10.1021/acs.chemmater.0c02008 ↗
91. A barrier analysis for distributed recycling of 3D printing waste: taking the maker movement perspective10.1016/j.jclepro.2019.118313 ↗
92. Recycled polycarbonate and polycarbonate/acrylonitrile butadiene styrene feedstocks for circular economy product applications with fused granular fabrication-based additive manufacturing
93. Close-looped recycling of polylactic acid used in 3D printing: an experimental investigation and life cycle assessment10.1016/j.jclepro.2018.06.275 ↗
94. Sustainable approach to the revalorization of crab shell waste in polymeric filament extrusion for 3D printing applications10.1007/s13399-023-03795-9 ↗
95. Potential and challenges of recycled polymer plastics and natural waste materials for additive manufacturing
96. Recycled additive manufacturing feedstocks with carboxylated multi-walled carbon nanotubes toward the detection of yellow fever virus cDNA10.1016/j.cej.2023.143513 ↗
97. Characterization of PLA feedstock after multiple recycling processes for large-format material extrusion additive manufacturing
98. Recycling polymer composite granulate/regrind using big area additive manufacturing10.1016/j.compositesb.2023.110652 ↗
99. Life cycle assessment of using firewood and wood pellets in Slovenia as two primary wood-based heating systems and their environmental impact10.3390/su16041687 ↗
100. Environmental impact of Slovenian and Croatian electricity generation using an hourly production-based dynamic life cycle assessment approach10.3390/en18184826 ↗