Eutectic gels: Presentation and prospect
Source abstract
Abstract
The optimization of conductive hydrogels, pivotal components in wearable devices, has garnered significant attention from researchers worldwide. Utilizing deep eutectic solvents (DES), the emergence of novel soft materials known as conductive gels has gained traction due to their cost-effectiveness, non-volatility, non-toxicity, and exceptional biocompatibility. However, a comprehensive understanding of their characteristics, preparation methods, and application potential is needed to fully harness these benefits. This review begins by contrasting the technical specifications of eutectic gels and delineating key performance parameters to encapsulate their properties. Subsequently, it delves into the preparation methods and structural design classifications of eutectic gels, evaluating the advantages and drawbacks of various structural types. Finally, it outlines the primary application domains and scenarios of eutectic gels, highlighting certain deficiencies while envisioning their future developmental prospects.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Advancements in Transdermal Drug Delivery · Hydrogels: synthesis, properties, applications · Surfactants and Colloidal Systems
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (100+)
Show source-provided references
1. Flexible wearable devices for intelligent health monitoring10.1002/VIW.20220027 ↗
2. Self-powered wireless flexible ionogel wearable devices
3. Review of flexible wearable sensor devices for biomedical application10.3390/mi13091395 ↗
4. Conductive hydrogel for flexible bioelectronic device: current progress and future perspective10.1002/adfm.202308974 ↗
5. Flexible memristor-based nanoelectronic devices for wearable applications: a review10.1021/acsanm.3c03397 ↗
6. Applications of flexible electronics related to cardiocerebral vascular system
7. Hydrogels and hydrogel-derived materials for energy and water sustainability10.1021/acs.chemrev.0c00345 ↗
8. A review of conventional and emerging technologies for hydrogels sterilization10.1016/j.ijpharm.2023.122671 ↗
9. Going beyond traditional applications? the potential of hydrogels10.1002/smtd.201800270 ↗
10. Biphasic organohydrogels based on phase change materials with excellent thermostability for thermal management applications10.1016/j.cej.2021.129181 ↗
11. Advances and challenges in conductive hydrogels: from properties to applications10.1016/j.eurpolymj.2022.111454 ↗
12. Recyclable, stretchable and conductive double network hydrogels towards flexible strain sensors10.1039/C8TC04958K ↗
13. Long-term in vivo degradation and biocompatibility of degradable pHEMA hydrogels containing graphene oxide10.1016/j.actbio.2023.11.012 ↗
14. Ultrastrong and tough supramolecular hydrogels from multiurea linkage segmented copolymers with tractable processablity and recyclability10.1002/marc.201700275 ↗
15. Physically crosslinked polyvinyl alcohol/chitosan-phytic acid hydrogels for wearable sensors with highly conductive, recyclable and antibacterial properties10.1007/s40843-023-2530-4 ↗
16. Bioinspired, recyclable, stretchable hydrogel with boundary ultra lubrication10.1021/acsami.1c12631 ↗
17. Gel–polymer electrolytes based on poly(ionic liquid)/ionic liquid networks10.1021/acsapm.0c01042 ↗
18. Emerging applications of tough ionogels10.1038/s41427-023-00514-8 ↗
19. Ionogels: preparation, properties and applications10.1002/adfm.202314408 ↗
20. A highly conductive and thermally stable ionic liquid gel electrolyte for calcium-ion batteries10.1021/acsapm.9b01223 ↗
21. Flexible ionic-gel strain sensor with double network, high conductivity and high frost-resistance using electrohydrodynamic printing method
22. Ionic liquid-based gels for biomedical applications10.1016/j.cej.2022.139248 ↗
23. X. Huang, Y. Liu, W. Park, Z. Zhao, J. Li, C.K. Lim, T.H. Wong, C.K. Yiu, Y. Gao, J. Zhou, H. Li, L. Zhao, J. Li, B. Zhang, Y. Huang, R. Shi, D. Li, J. Mo, J. Wang, C. Zhang, Y. Li, Z. Wang, X. Yu, Stretchable magnesium–air battery based on dual ions conducting hydrogel for intelligent biomedical applications, InfoMat 5(3) (2023) e12388.10.1002/inf2.12388 ↗
24. Ionotropic gelation of chitosan flat structures and potential applications10.3390/molecules26030660 ↗
25. Using chitosan nanofibers to simultaneously improve the toughness and sensing performance of chitosan-based ionic conductive hydrogels10.1016/j.ijbiomac.2024.129272 ↗
26. Micropatterned elastic ionic polyacrylamide hydrogel for low-voltage capacitive and organic thin-film transistor pressure sensors10.1016/j.nanoen.2019.01.032 ↗
27. Degradable supramolecular eutectogel-based ionic skin with antibacterial, adhesive, and self-healable capabilities10.1021/acsami.3c04434 ↗
28. An inclusive thermophysical and rheology portrayal of deep eutectic solvents (DES) for metal oxides dissolution enhancement10.1016/j.molliq.2021.115909 ↗
29. Are deep eutectic solvents really green?: a life-cycle perspective10.1039/D2GC01752K ↗
30. DESs: green solvents for transition metal catalyzed organic reactions10.1016/j.cclet.2019.05.063 ↗
31. Deep eutectic solvent-assisted stimuli-responsive smart hydrogels – A review10.1016/j.eurpolymj.2022.111711 ↗
32. Non-covalent interactions in action: advancing eutectogels for enhanced stability and performance10.1016/j.polymer.2024.127262 ↗
33. Deep eutectic solvents towards green polymeric materials10.1039/D4GC00532E ↗
34. Novel solvent properties of choline chloride/urea mixtures10.1039/b210714g ↗
35. Deep eutectic solvent-assisted stimuli-responsive smart hydrogels – A review10.1016/j.eurpolymj.2022.111711 ↗
36. Poly(N-acryloyl glycinamide) eutectogels10.1002/pol.20230603 ↗
37. Deep eutectic solvents as green solvents for materials preparation10.1039/D4GC00136B ↗
38. Strong and tough physical eutectogels regulated by the spatiotemporal expression of non-covalent interactions10.1002/adfm.202206305 ↗
39. Synthesis of hydrogels by polymerization of itaconic acid–choline chloride deep eutectic solvent10.1002/app.40608 ↗
40. Highly stretchable and nonvolatile gelatin-supported deep eutectic solvent gel electrolyte-based ionic skins for strain and pressure sensing10.1039/C8TC05918G ↗
41. Supramolecular G4 eutectogels of guanosine with solvent-induced chiral inversion and excellent electrochromic activity10.1002/anie.202009332 ↗
42. Deep eutectic solvent based self-healable, stretchable and injectable eutectogels: a versatile platform for breast cancer treatment
43. Self-adhesive, stretchable, biocompatible, and conductive nonvolatile eutectogels as wearable conformal strain and pressure sensors and biopotential electrodes for precise health monitoring10.1021/acsami.1c04671 ↗
44. Hydrophobic eutectogels as electrodes for underwater electromyography recording10.1021/acsmaterialslett.3c00938 ↗
45. Preparation of a multifunctional wound dressing based on a natural deep eutectic solvent10.1021/acssuschemeng.0c05754 ↗
46. Evolutionary reinforcement of polymer networks: a stepwise-enhanced strategy for ultrarobust eutectogels10.1002/adma.202309576 ↗
47. Fabrication of gelatin-derived gel electrolyte using deep eutectic solvents through in situ derivatization and crosslinking strategy for supercapacitors and flexible sensors10.1021/acsami.3c06966 ↗
48. Transient dual-response iontronic strain sensor based on gelatin and cellulose nanocrystals eutectogel nanocomposites10.1002/admi.202300536 ↗
49. Insights into the synthesis and properties of deep eutectic solvents based on cholinium chloride and carboxylic acids10.1021/sc500439w ↗
50. Stretchable and conductive physical eutectogel based on type IV deep eutectic solvent through cation-bridging10.1016/j.molliq.2024.124011 ↗
51. Citric acid-based deep eutectic solvent for the anthocyanin recovery from Hibiscus sabdariffa through microwave-assisted extraction10.1007/s13399-020-00606-3 ↗
52. Deep eutectic solvents eutectogels: progress and challenges10.1016/j.gce.2021.06.001 ↗
53. Ultrasound-assisted deep eutectic solvent extraction of echinacoside and oleuropein from Syringa pubescens Turcz10.1016/j.indcrop.2020.112442 ↗
54. Exploring anionic homopolymerization and copolymerization of vinyl monomers in deep eutectic solvent10.1016/j.eurpolymj.2023.112044 ↗
55. Deep eutectic solvents and multicomponent reactions: two convergent items to green chemistry strategies10.1002/open.202100137 ↗
56. Polysaccharide-based supramolecular bicomponent eutectogels as sustainable antioxidant materials10.1039/D3GC00573A ↗
57. A highly adhesive and mechanically robust eutectogel electrolyte for constructing stable integrated stretchable supercapacitors10.1016/j.cej.2023.146378 ↗
58. Cellulose-reinforced highly stretchable and adhesive eutectogels as efficient sensors10.1016/j.ijbiomac.2024.131115 ↗
59. Highly conductive, transparent, adhesive, and self-healable ionogel based on a deep eutectic solvent with widely adjustable mechanical strength10.1002/marc.202200480 ↗
60. Choline chloride-based deep eutectic solvents in the dearomatization of gasolines10.1021/acssuschemeng.7b03362 ↗
61. Insights into the chloride versus bromide effect on the formation of urea-quaternary ammonium eutectic solvents10.1021/acs.iecr.2c01274 ↗
62. Rapid and general access to α-haloketones using quaternary ammonium salts as halogen sources10.1021/acs.joc.3c02195 ↗
63. Ecotoxicological study of glucose: choline chloride and sorbitol: choline chloride at different contents of water10.1007/s11356-023-25538-z ↗
64. Antimicrobial betalains10.1111/jam.15798 ↗
65. Cellulose-starch hybrid films plasticized by aqueous ZnCl2 solution10.3390/ijms20030474 ↗
66. Electrochemistry of the NaI-AlCl3 molten salt system for use as catholyte in sodium metal batteries10.1149/2.1191814jes ↗
67. One-pot generation of lignin microspheres and digestible substrate with a polyol-DES pretreatment in high solid loading10.1016/j.jclepro.2023.136322 ↗
68. The role of poly(acrylic acid) in conventional glass polyalkenoate cements10.1515/polyeng-2015-0079 ↗
69. Thermophysical properties of glycerol and polyethylene glycol (PEG 600) based DES10.1016/j.molliq.2017.10.030 ↗
70. The solubility and interactions of gelatin in “water-in-sodium acetate trihydrate/urea-DES” system10.1016/j.colsurfa.2021.126916 ↗
71. Self-assembled gels formed in deep eutectic solvents: supramolecular eutectogels with high ionic conductivity10.1002/anie.201810600 ↗
72. Tough and stretchable phenolic-reinforced double network deep eutectic solvent gels for multifunctional sensors with environmental adaptability10.1002/adfm.202303381 ↗
73. An anti-swellable hydrogel strain sensor for underwater motion detection10.1002/adfm.202107404 ↗
74. Rheological properties and 3D-printability of cellulose nanocrystals/deep eutectic solvent electroactive ion gels10.1016/j.carbpol.2022.119475 ↗
75. B. Guo, M. Yao, S. Chen, Q. Yu, L. Liang, C. Yu, M. Liu, H. Hao, H. Zhang, F. Yao, J. Li, Environment-tolerant conductive eutectogels for multifunctional sensing, Adv. Funct. Mater. n/a(n/a) 2315656.
76. Temperature-responsive ionic conductive hydrogel for strain and temperature sensors10.1021/acsami.2c06952 ↗
77. Highly stretchable and self-healing cellulose nanofiber-mediated conductive hydrogel towards strain sensing application10.1016/j.jcis.2021.04.001 ↗
78. An eutectic gel based on polymerizable deep eutectic solvent with self-adhesive, self-adaptive cold and high temperature environments10.1002/admt.202201509 ↗
79. Mussel-inspired adhesive and conductive hydrogel with tunable mechanical properties for wearable strain sensors10.1016/j.jcis.2020.10.023 ↗
80. Self-healing, self-adhesive silk fibroin conductive hydrogel as a flexible strain sensor10.1021/acsami.1c08395 ↗
81. Transparent, stretchable, underwater self-healing, self-adhesive, and recyclable eutectogels enabled by poly(ionic liquid)/eutectic networks10.1021/acsapm.4c00014 ↗
82. Deep eutectic solvents as an emerging green platform for the synthesis of functional materials10.1039/D3GC04289H ↗
83. Cellulose nanocrystalline hydrogel based on a choline chloride deep eutectic solvent as wearable strain sensor for human motion
84. Cellulose eutecticgel electrolytes based on ethylene glycol/zinc chloride deep eutectic solvent for flexible solid-state capacitors
85. Physically entangled multifunctional eutectogels for flexible sensors with mechanically robust10.1039/D4TA02751E ↗
86. Developing transparent and conductive PolyHEMA gels using deep eutectic solvents10.3390/polym15122605 ↗
87. High tensile properties, wide temperature tolerance, and DLP-printable eutectogels for microarrays wearable strain sensors
88. Innovative poly (ionic liquid) s by the polymerization of deep eutectic monomers10.1002/marc.201600026 ↗
89. Poly(N-acryloyl glycinamide) eutectogels10.1002/pol.20230603 ↗
90. Environmentally stable, robust, adhesive, and conductive supramolecular deep eutectic gels as ultrasensitive flexible temperature sensor10.1002/adma.202300114 ↗
91. A highly transparent, underwater self-healing, self-adhesive, and recyclable supramolecular eutectogel for liquid metal encapsulation10.1021/acsmaterialslett.3c00555 ↗
92. Impact of hydrogen bonding interaction energy on the polymerization kinetics of polymerizable deep eutectic solvent monomers
93. Green and sustainable solvents of the future: deep eutectic solvents10.1016/j.molliq.2023.121676 ↗
94. Super-stretchable and extreme temperature-tolerant supramolecular-polymer double-network eutectogels with ultrafast in situ adhesion and flexible electrochromic behaviour10.1039/D1MH00725D ↗
95. Biocompatible, antibacterial, and stable deep eutectic solvent-based ionic gel multimodal sensors for healthcare applications10.1021/acsami.3c09613 ↗
96. Optimal design of THEDES based on perillyl alcohol and ibuprofen10.3390/pharmaceutics12111121 ↗
97. Current status and future potential of transdermal drug delivery10.1038/nrd1304 ↗
98. Elastomeric protein bioactive eutectogels for topical drug delivery10.1002/adfm.202313747 ↗
99. Preparation of a noncytotoxic hemocompatible ion gel by self-polymerization of HEMA in a green deep eutectic solvent10.1002/macp.201600122 ↗
100. Multiple dynamic interaction-enabled eutectogel with strong tissue adhesion, mechanical strength and temperature tolerance for transdermal drug delivery: double monodentate coordination and π-π interaction10.1016/j.cej.2023.146583 ↗