journal article·2020-02

A facile fabrication of Ag2O-Ag/ZnAl-oxides with enhanced visible-light photocatalytic performance for tetracycline degradation

Jia-Chao Shen, Hong-Yan Zeng, Chao-Rong Chen, Sheng Xu

Publisher page

Abstract

Abstract A facile and low-cost method to prepare novel Ag2O-Ag/LDO photocatalysts was demonstrated, where the Ag2O/Ag nanoparticles were decorated on the ZnAl oxide (LDO) supports. The LDO supports were obtained by calcining their ZnAl layered double hydroxide precursor (LDH) at different temperatures. The structure, composition, morphology and optical and electrochemical properties of the as-prepared Ag2O-Ag/LDO were characterized using various techniques. Under visible light irradiation, the Ag2O-Ag/LDO showed higher photoactivity and stability of tetracycline (TC) degradation than pure Ag2O-Ag. Especially, the Ag2O-Ag/LDO5 (Ag2O-Ag/LDO calcined at 500 °C) had the most excellent photoactivity with the highest rate constant k (0.0242 min−1), suggesting that the photocatalytic activity depended on the calcination temperature. The enhancement of the photocatalytic performance was attributed to the formation of the heterostructure between Ag2O/Ag and ZnO, the strong visible-light absorption and outstanding separation efficiency of photoinduced electron-hole pairs under visible light irradiation.
Source: openaire · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Advanced Photocatalysis Techniques · Layered Double Hydroxides Synthesis and Applications · Quantum Dots Synthesis And Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (44)

Show source-provided references
1. Polyethersulfone (PES)-silver composite UF membrane: effect of silver loading and PVP molecular weight on membrane morphology and antibacterial activity10.1016/j.desal.2010.11.010 ↗
2. A review on photocatalysis for air treatment: from catalyst development to reactor design10.1016/j.cej.2016.06.090 ↗
3. In situ surfactant removal from MCM-type mesostructures by ozone treatment10.1039/b005297n ↗
4. Fabrication of a ternary plasmonic photocatalyst CQDs/Ag/Ag2O to harness charge flow for photocatalytic elimination of pollutants10.1016/j.apcatb.2016.03.056 ↗
5. A nanosheet-like α-Bi2O3/g-C3N4 heterostructure modified by plasmonic metallic Bi and oxygen vacancies with high photodegradation activity of organic pollutants10.1016/j.seppur.2017.11.011 ↗
6. Pyrolysis kinetics and pore-forming mechanism of hydrotalcite/carbon composite10.1016/j.clay.2018.05.016 ↗
7. Facile fabrication of CdS/ZnAlO heterojunction with enhanced photocatalytic activity for Cr(VI) reduction under visible light10.1016/j.clay.2018.08.019 ↗
8. Three-dimensional Ag2O/Bi5O7I p-n heterojunction photocatalyst harnessing UV-vis-NIR broad spectrum for photodegradation of organic pollutants10.1016/j.jhazmat.2017.10.015 ↗
9. Anion-doped mixed metal oxide nanostructures derived from layered double hydroxide as visible light photocatalysts10.1002/adfm.201201883 ↗
10. Fabrication of Ag-Ag2O/reduced TiO2 nanophotocatalyst and its enhanced visible light driven photocatalytic performance for degradation of diclofenac solution10.1016/j.apcatb.2017.01.014 ↗
11. Effect of Ag+ reduction on the photocatalytic activity of Ag-doped TiO210.1016/j.spmi.2017.05.043 ↗
12. Promoting visible-light-induced photocatalytic degradation of tetracycline by an efficient and stable beta-Bi2O3@g-C3N4 core/shell nanocomposite10.1016/j.cej.2017.12.108 ↗
13. Enhanced solar photodegradation of toxic pollutants by long-lived electrons in Ag2O-Ag nanocomposites10.1016/j.apcatb.2015.04.040 ↗
14. Zn-Al layered double oxides as high-performance anode materials for zinc-based secondary battery10.1039/C5TA00279F ↗
15. Thermo-responsive PNIPAM@AgBr/CSs composite photocatalysts for switchable degradation of tetracycline antibiotics10.1016/j.jallcom.2016.11.219 ↗
16. Construction of fiber-shaped silver oxide/tantalum nitride pn heterojunctions as highly efficient visible-light-driven photocatalysts10.1016/j.jcis.2017.06.018 ↗
17. Electro-oxidation of tetracycline by a Magnéli phase Ti4O7 porous anode: Kinetics, products, and toxicity10.1016/j.cej.2017.09.109 ↗
18. Enhanced photocatalysis of electrospun Ag-ZnO heterostructured nanofibers10.1021/cm900225p ↗
19. In situ synthesis of MOF membranes on ZnAl-CO3 LDH buffer layer-modified substrates10.1021/ja507408s ↗
20. Efficient removal of radioactive iodide ions from water by three-dimensional Ag2O-Ag/TiO2 composites under visible light irradiation10.1016/j.jhazmat.2014.10.054 ↗
21. Fabrication of a Ag/Bi3TaO7 plasmonic photocatalyst with enhanced photocatalytic activity for degradation of tetracycline10.1021/acsami.5b03535 ↗
22. Dual oxygen and tungsten vacancies on a WO3 photoanode for enhanced water oxidation10.1002/anie.201605247 ↗
23. Nanostructured CeO2/MgAl-LDH composite for visible light induced water reduction reaction10.1016/j.ijhydene.2016.08.062 ↗
24. Dynamics of charge-transfer behavior in a plasmon-induced quasi-type-II p–n/n–n dual heterojunction in Ag@ Ag3PO4/g-C3N4/NiFe LDH nanocomposites for photocatalytic Cr (VI) reduction and phenol oxidation10.1021/acsomega.8b00847 ↗
25. Deciphering Z-scheme charge transfer dynamics in heterostructure NiFe-LDH/N-rGO/gC3N4 nanocomposite for photocatalytic pollutant removal and water splitting reactions
26. Visible light-driven novel gC3N4/NiFe-LDH composite photocatalyst with enhanced photocatalytic activity towards water oxidation and reduction reaction10.1039/C5TA05002B ↗
27. Topotactic transformation of solvated MgCr-LDH nanosheets to highly efficient porous MgO/MgCr2O4 nanocomposite for photocatalytic H2 evolution10.1021/acs.inorgchem.8b01517 ↗
28. Enhanced photocatalytic activities of RhB degradation and H2 evolution from in situ formation of the electrostatic heterostructure MoS2/NiFe LDH nanocomposite through the Z-Scheme mechanism via p-n heterojunctions10.1021/acsami.9b06511 ↗
29. A review of ZnO nanoparticles as solar photocatalysts: Synthesis, mechanisms and applications10.1016/j.rser.2017.08.020 ↗
30. Ecofriendly synthesis and solar photocatalytic activity of S-doped ZnO10.1016/j.jhazmat.2010.07.026 ↗
31. Iron improving bio-char derived from microalgae on removal of tetracycline from aqueous system10.1007/s11356-014-2677-2 ↗
32. Preparation of zinc/iron layered double hydroxide intercalated by citrate anion for capturing lead(II) from aqueous solution10.1016/j.molliq.2018.02.018 ↗
33. Three dimensional Ag2O/TiO2 type-II (p-n) nanoheterojunctions for superior photocatalytic activity10.1021/am302136y ↗
34. Enhanced photocatalytic activity over the Ag2O-gC3N4 composite under visible light10.1039/c3cy00871a ↗
35. In situ synthesis of Z-scheme Ag3PO4/CuBi2O4 photocatalysts and enhanced photocatalytic performance for the degradation of tetracycline under visible light irradiation10.1016/j.apcatb.2017.03.048 ↗
36. ZnAl2O4/Bi2MoO6 heterostructures with enhanced photocatalytic activity for the treatment of organic pollutants and eucalyptus chemomechanical pulp wastewater
37. Preparation and characterization of Ag2O/SWNTs photocatalysts and its photodegradation on tetracycline10.1016/j.jiec.2015.05.002 ↗
38. Facile synthesis of an Ag2O-ZnO nanohybrid and its high photocatalytic activity10.1002/cplu.201200159 ↗
39. Construction of carbon dots modified MoO3/g-C3N4 Z-scheme photocatalyst with enhanced visible-light photocatalytic activity for the degradation of tetracycline10.1016/j.apcatb.2018.02.011 ↗
40. Mg-Fe mixed oxides as solid base catalysts for the transesterification of microalgae oil10.1039/C5RA14144C ↗
41. Plasma-induced formation of flower-like Ag2O nanostructures10.1016/j.apsusc.2015.05.055 ↗
42. Degradation of tetracycline by immobilized laccase and the proposed transformation pathway10.1016/j.jhazmat.2016.10.019 ↗
43. Hydrogen peroxide biosensor based on chitosan/2D layered double hydroxide composite for the determination of H2O210.1016/j.bioelechem.2018.04.009 ↗
44. Preparation of Mg-Al hydrotalcite by urea method and its catalytic activity for transesterification10.1002/aic.11722 ↗