journal article·2025-12-01Open access

Benchmarking interfacial magnetic interactions and spin Hall angle in heavy metal /CoFeB/MgO heterostructures

Royston J. J. Lim, T. S. Suraj, Anuj Kumar, Liming Wang, Jifei Huang, Hang Khume Tan, Hui Ru Tan, Nelson C. B. Lim, Pin Ho, Hongxin Yang, Shaohai Chen, Anjan Soumyanarayanan

APL Materials· Volume 13· Issue 12

Abstract

The stability and efficient electrical control of chiral spin textures (CSTs) is critical for their implementation in racetrack device architectures. Three principal properties determine the utility of material platforms for spin-texture dynamics: perpendicular magnetic anisotropy (PMA), Dzyaloshinskii–Moriya interaction (DMI), and spin Hall angle (SHA). Notwithstanding individual studies, a comprehensive benchmarking of these key interactions across racetrack-compatible material systems remains lacking. Here, we systematically evaluate tunnel-readout compatible HM/CoFeB/MgO trilayers fabricated using wafer-scale techniques. Their key properties—PMA, DMI, and SHA—were characterized across four heavy metals (Pt, W, Ta, and Ir) and two CoFeB compositions using magnetometry, spectroscopy, and transport techniques, respectively. Our results reveal that the W-based stacks exhibit robust PMA and high SHA, while the Pt-based stacks provide the strongest DMI. Notably, both DMI and SHA depend strongly on both heavy metal and CoFeB composition, underscoring the critical role of alloy engineering in controlling interfacial magnetic properties. Our work provides quantitative benchmarks and materials design principles for developing next-generation CST-based racetrack devices.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Magnetic properties of thin films · Heusler alloys: electronic and magnetic properties · Magnetic Properties and Synthesis of Ferrites

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Institute of Materials Research and Engineering (IMRE), Agency for Science, Technology and Research (A*STAR) 1 , Singapore 138634,

Department of Physics, National University of Singapore 2 , Singapore 117551,

Center for Quantum Matter, School of Physics, Zhejiang University 3 , Hangzhou 310058,

Funding

Agency for Science, Technology and Research · National University of Singapore · Ministry of Education - Singapore

References (71)

Show source-provided references
1. Magnetic skyrmions: Advances in physics and potential applications10.1038/natrevmats.2017.31 ↗
2. Chiral spintronics10.1038/s42254-021-00302-9 ↗
3. Magnetic domain-wall racetrack memory10.1126/science.1145799 ↗
4. A spin–orbit torque switching scheme with collinear magnetic easy axis and current configuration10.1038/nnano.2016.29 ↗
5. Current-driven magnetic domain-wall logic10.1038/s41586-020-2061-y ↗
6. Multicore memristor from electrically readable nanoscopic racetracks10.1126/science.adh3419 ↗
7. Fast current-induced skyrmion motion in synthetic antiferromagnets10.1126/science.add5751 ↗
8. Domain-wall velocities of up to 750 ms−1 driven by exchange-coupling torque in synthetic antiferromagnets10.1038/nnano.2014.324 ↗
9. 230% room-temperature magnetoresistance in CoFeB∕MgO∕CoFeB magnetic tunnel junctions10.1063/1.1871344 ↗
10. Spin polarization of amorphous CoFeB determined by point-contact Andreev reflection10.1063/1.2949740 ↗
11. Perpendicular switching of a single ferromagnetic layer induced by in-plane current injection10.1038/nature10309 ↗
12. Current-induced spin-orbit torques in ferromagnetic and antiferromagnetic systems10.1103/revmodphys.91.035004 ↗
13. Emergent phenomena induced by spin–orbit coupling at surfaces and interfaces10.1038/nature19820 ↗
14. Dzyaloshinsky–Moriya interactions induced by symmetry breaking at a surface10.1016/S0304-8853(97)01044-5 ↗
15. Spin-torque switching with the giant spin hall effect of tantalum10.1126/science.1218197 ↗
16. Unveiling the emergent traits of chiral spin textures in magnetic multilayers10.1002/advs.202103978 ↗
17. Dynamics of dzyaloshinskii domain walls in ultrathin magnetic films10.1209/0295-5075/100/57002 ↗
18. Current-driven dynamics of chiral ferromagnetic domain walls10.1038/nmat3675 ↗
19. Tunable room-temperature magnetic skyrmions in Ir/Fe/Co/Pt multilayers10.1038/nmat4934 ↗
20. Asymmetric magnetic domain-wall motion by the Dzyaloshinskii–Moriya interaction10.1103/physrevb.88.214401 ↗
21. Memory on the racetrack10.1038/nnano.2015.41 ↗
22. First-principles investigation of the very large perpendicular magnetic anisotropy at Fe| MgO and Co| MgO interfaces10.1103/physrevb.84.054401 ↗
23. Role of boron diffusion in CoFeB/MgO magnetic tunnel junctions10.1103/physrevb.91.085311 ↗
24. Influence of boron diffusion on the perpendicular magnetic anisotropy in Ta|CoFeB|MgO ultrathin films10.1063/1.4906096 ↗
25. Giant interfacial perpendicular magnetic anisotropy in MgO/CoFe/capping layer structures10.1063/1.4976517 ↗
26. Extremely large perpendicular magnetic anisotropy of an Fe(001) surface capped by 5d transition metal monolayers: A density functional study10.1103/physrevb.88.184405 ↗
27. Perpendicular magnetic anisotropy caused by interfacial hybridization via enhanced orbital moment in Co/Pt multilayers: Magnetic circular X-Ray dichroism Study10.1103/physrevlett.81.5229 ↗
28. Probing the Dzyaloshinskii–Moriya interaction in CoFeB ultrathin films using domain wall creep and Brillouin light spectroscopy10.1103/physrevb.94.104431 ↗
29. Interfacial Dzyaloshinskii–Moriya interaction: Effect of 5d band filling and correlation with spin mixing conductance10.1103/physrevlett.120.157204 ↗
30. Enhanced spin Hall torque efficiency in Pt100−xAlx and Pt100−xHfx alloys arising from the intrinsic spin Hall effect10.1063/1.4953768 ↗
31. Unveiling the mechanisms of the spin Hall effect in Ta10.1103/physrevb.98.060410 ↗
32. Temperature study of the giant spin Hall effect in the bulk limit of β-W10.1103/physrevb.98.134411 ↗
33. Role of transparency of platinum–ferromagnet interfaces in determining the intrinsic magnitude of the spin Hall effect10.1038/nphys3304 ↗
34. A perpendicular-anisotropy CoFeB–MgO magnetic tunnel junction10.1038/nmat2804 ↗
35. First-principles calculations for Dzyaloshinskii–Moriya interaction10.1038/s42254-022-00529-0 ↗
36. Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set10.1103/PhysRevB.54.11169 ↗
37. Spin pumping damping and magnetic proximity effect in Pd and Pt spin-sink layers10.1103/physrevb.94.014414 ↗
38. Structure, magnetic and thermal properties of FePt–C–BN granular films for heat assisted magnetic recording10.1088/1361-6463/ab680d ↗
39. Enhancement of perpendicular magnetic anisotropy and transmission of spin-Hall-effect-induced spin currents by a Hf spacer layer in W/Hf/CoFeB/MgO layer structures10.1063/1.4866965 ↗
40. Co-Ir interface alloying induced by thermal annealing10.1063/1.4967845 ↗
41. Effects of MgO thickness and roughness on perpendicular magnetic anisotropy in MgO/CoFeB/Ta multilayers10.1088/0256-307x/33/10/107804 ↗
42. Tailoring magnetic properties of CoFeB films via tungsten buffer and capping layers10.1016/j.jmmm.2024.172701 ↗
43. Enhancing perpendicular magnetic anisotropy through dead layer reduction utilizing precise control of Mg insertions10.1016/j.jmmm.2020.166956 ↗
44. Contributions of Co and Fe orbitals to perpendicular magnetic anisotropy of MgO/CoFeB bilayers with Ta, W, IrMn, and Ti underlayers10.7567/apex.10.073006 ↗
45. Intermixing induced anisotropy variations in CoB-based chiral multilayer films10.1088/1361-6463/ac09b6 ↗
46. Magnetic properties of nanostructured Fe-Co alloys10.1063/1.4795267 ↗
47. Ferromagnetic alloy material CoFeC with high thermal tolerance in MgO/CoFeC/Pt structure and comparable intrinsic damping factor with CoFeB10.1088/1361-6463/aaa30a ↗
48. Stack structure and CoFeB composition dependence of perpendicular magnetic anisotropy employing Pt heavy metal layer10.1016/j.jallcom.2022.167205 ↗
49. First-principles study of origin of perpendicular magnetic anisotropy in MgO|CoFeB|Ta structures10.1016/j.rinp.2023.106239 ↗
50. Measuring interfacial Dzyaloshinskii–Moriya interaction in ultrathin magnetic films10.1103/revmodphys.95.015003 ↗
51. Quantifying symmetric exchange in ultrathin ferromagnetic films with chirality10.1103/physrevb.107.094405 ↗
52. Quantitative accordance of Dzyaloshinskii–Moriya interaction between domain-wall and spin-wave dynamics10.1103/physrevb.100.224419 ↗
53. Direct observation of the Dzyaloshinskii–Moriya interaction in a Pt/Co/Ni film10.1103/physrevlett.114.047201 ↗
54. Linear relation between Heisenberg exchange and interfacial Dzyaloshinskii–Moriya interaction in metal films10.1038/nphys3418 ↗
55. Critical role of orbital hybridization in the Dzyaloshinskii–Moriya interaction of magnetic interfaces10.1038/s42005-022-00932-0 ↗
56. Quantifying the Dzyaloshinskii–Moriya interaction induced by the bulk magnetic asymmetry10.1103/physrevlett.128.167202 ↗
57. Investigation of the Dzyaloshinskii–Moriya interaction and room temperature skyrmions in W/CoFeB/MgO thin films and microwires10.1063/1.4991360 ↗
58. Role of B diffusion in the interfacial Dzyaloshinskii–Moriya interaction in Ta/Co20Fe60B20/MgO nanowires10.1103/physrevb.91.014433 ↗
59. Dzyaloshinskii–Moriya interaction and spin-orbit torque at the Ir/Co interface10.1103/physrevb.99.134421 ↗
60. Gueneau, C., , “Dzyaloshinskii–Moriya interaction chirality reversal with ferromagnetic thickness,” arXiv:2501.12098 (2025).
61. Giant spin torque efficiency in single-crystalline antiferromagnet Mn2Au films10.1007/s40843-020-1574-5 ↗
62. Spin–orbit torque characterization in a nutshell10.1063/5.0041123 ↗
63. Large planar Hall effect in perpendicularly magnetized W/CoFeB/MgO structures10.1016/j.cap.2015.04.002 ↗
64. Spin transfer torque devices utilizing the giant spin Hall effect of tungsten10.1063/1.4753947 ↗
65. Spin Hall effect in the α and β phases of TaxW1−x alloys10.1103/PhysRevB.102.094438 ↗
66. Spin-orbit torques in laminated tungsten multilayers with nominally doped oxygen10.1103/physrevapplied.23.014009 ↗
67. Modulation of spin-orbit torque and large enhancement of perpendicular magnetic anisotropy in W/Co20Fe60B20/MgO by Ir insertion layer10.1103/PhysRevApplied.19.034043 ↗
68. Evolution of zero-field skyrmionic states in exchange-coupled composite multilayer nanodots10.1103/physrevapplied.22.024036 ↗
69. Electrical detection of magnetic skyrmions in a magnetic tunnel junction10.1002/aelm.202200570 ↗
70. All-electrical skyrmionic magnetic tunnel junction10.1038/s41586-024-07131-7 ↗
71. Electrical detection and nucleation of a magnetic skyrmion in a magnetic tunnel junction observed via operando magnetic microscopy10.1021/acs.nanolett.4c00316 ↗