journal article·2019-10-01Open access

Engineering antiphase boundaries in epitaxial SrTiO3 to achieve forming free memristive devices

Felix V. E. Hensling, Hongchu Du, Nicolas Raab, Chun-Lin Jia, Joachim Mayer, Regina Dittmann

APL Materials· Volume 7· Issue 10

Abstract

We here present a method to engineer Ruddlesden-Popper-type antiphase boundaries in stoichiometric homoepitaxial SrTiO3 thin films. This is achieved by using a substrate with an intentionally high miscut, which stabilizes the growth of additional SrO at the bottom interface. We prove the success of this strategy utilizing transmission electron microscopy. We find that these antiphase boundaries significantly influence the resistive switching properties. In particular, devices based on SrTiO3 thin films with intentionally induced antiphase boundaries do not require a forming step, which is ascribed to the existence of preformed filaments.
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Research context

OpenAlex topics: Advanced Memory and Neural Computing · Electronic and Structural Properties of Oxides · Ferroelectric and Negative Capacitance Devices

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

PGI-7, Forschungszentrum Jülich GmbH 1 , 52425 Jülich, Germany

JARA-FIT, Forschungszentrum Jülich GmbH 2 , 52425 Jülich, Germany

ER-C 2, Forschungszentrum Jülich GmbH 3 , 52425 Jülich, Germany

GFE, RWTH Aachen University 4 , 52074 Aachen, Germany

ER-C 1, Forschungszentrum Jülich GmbH 5 , 52425 Jülich, Germany

PGI-5, Forschungszentrum Jülich GmbH 6 , 52425 Jülich, Germany

Funding

Deutsche Forschungsgemeinschaft · Helmholtz Association

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