DataVXAdvanced Sustainable SystemsPaper
journal article·2024-08Open access

Facile Fabrication of FePO4–V2O5–Graphene Oxide Recovered From Spent LiFePO4 Batteries as High‐Performance Cathode for Lithium/Sodium‐Ion Batteries

Fuyu Xiao, Wenbin Lai, Shihan Zeng, Lingjun He, Mingyang Ge, Fenqiang Luo, Peixun Xiong, Hui Lin, Chuyuan Lin, Yongjin Luo, Jixiang Zhang, Qingrong Qian, Qinghua Chen, Lingxing Zeng

Advanced Sustainable Systems· Volume 8· Issue 8
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Abstract

Abstract The resource scarcity and pollution leakage risk caused by discarding the spent power lithium‐ion batteries has aroused growing concern. Recovering and regenerating the cathode material from spent power lithium‐ion batteries in an easy and environmentally friendly manner remains a significant challenge and an area of focus in battery research. Hence, a green and convenient method to recover FePO4 from spent LiFePO4 cathode powder by using Na2S2O8 as an oxidizer and as cathode materials for lithium/sodium‐ion batteries (LIBs/SIBs) is reported. Benefiting from the remarkable graphene oxide (GO) and vanadium oxide (V2O5) coating, the regenerated FePO4–V2O5–graphene oxide (FePO4–V2O5–GO) is suitable for Li/Na storage (153 mAh g−1 at 0.2C/118 mAh g−1 at 0.5C). The high capacity retention, that stable for 300 cycles in LIBs and 300 cycles for SIBs, is also realized due to the stable structure. This work provides a green strategy for regenerating the cathode of spent lithium‐ion batteries and designing cathodes of alkali metal ion batteries.
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Research context

Energy storageNanomaterials

OpenAlex topics: Advancements in Battery Materials · Extraction and Separation Processes · Advanced Battery Materials and Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Engineering Research Center of Polymer Green Recycling of Ministry of Education Fujian Key Laboratory of Pollution Control & Resource Reuse College of Environmental and Resources Fujian Normal University Fuzhou Fujian 350007 P. R. China

PV Metrology Institute Fujian Metrology Institute Fuzhou 350005 P. R. China

Inorganic Chemistry I Technische Universität Dresden Bergstrasse 66 01069 Dresden Germany

Department of Ecology and Environment of Fujian Province Center of Fujian Solid Waste and Chemical Environmental Management Technology Fuzhou Fujian 350003 P. R. China

Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), College of Chemistry Nankai University Tianjin 300071 P. R. China

Funding

National Basic Research Program of China · National Natural Science Foundation of China

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