Soft Electronic Platforms Combining Elastomeric Stretchability and Biodegradability
Source abstract
Abstract
Abstract Soft and stretchable electronic devices are expected to offer technological advances in the field of robotics, human–machine interfacing, and healthcare. Employing biodegradable elastomers, hydrogels, and nontoxic conductors would add significant value to and minimize the ecological impact of such disposable and transient electronic applications. Here, the biodegradable and photo‐crosslinkable elastomer poly(glycerol sebacic) acrylate (PGSA) is characterized for its use in soft and stretchable electronics. Its mechanical properties are investigated in terms of their chemical composition and compared to commonly used gelatin hydrogels. Furthermore, these materials are combined with interconnects made of liquid Galinstan in order to create functional substrates with certified biodegradability under ISO standards. The combination of these materials produces elastic circuit boards that act as soft platforms for body‐mounted sensors or biodegradable stretchable light‐emitting devices. These soft platforms reveal linear elongations at a break of 130% to 350% and similar moduli to nondegradable elastomers and human tissue, without any decrease in conductivity. Advanced applications in biofriendly packaging, soft robotics, and healthcare will greatly benefit from these biodegradable devices.
Source: crossref · Quality: baseline
Research context
OpenAlex topics: Advanced Sensor and Energy Harvesting Materials · Conducting polymers and applications · Electrospun Nanofibers in Biomedical Applications
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Light Technology Institute Karlsruhe Institute of Technology Engesserstr. 13 76131 Karlsruhe Germany
InnovationLab Speyererstr. 4 69115 Heidelberg Germany
Institute of Organic Chemistry Heidelberg University Im Neuenheimer Feld 270 69120 Heidelberg Germany
Faculty of Pharmacy University of Castilla‐La Mancha Calle Almansa 14‐Edif. Bioincubadora Albacete 02008 Spain
Funding
Bundesministerium für Bildung und Forschung
References (98)
Show source-provided references
1. 10.1021/acs.chemmater.9b0121110.1021/acs.chemmater.9b01211 ↗
2. Lee G.‐H. · Nat. Rev. Mater. · 2020 · 1 · 8
3. 10.1007/s41315-017-0016-810.1007/s41315-017-0016-8 ↗
4. 10.1007/s13593-016-0352-310.1007/s13593-016-0352-3 ↗
5. 10.1007/s13197-015-1766-710.1007/s13197-015-1766-7 ↗
6. 10.1007/s10008-014-2607-810.1007/s10008-014-2607-8 ↗
7. 10.1021/acs.chemrev.8b0057310.1021/acs.chemrev.8b00573 ↗
8. 10.1289/ehp.150969910.1289/ehp.1509699 ↗
9. 10.1016/j.progpolymsci.2007.05.01710.1016/j.progpolymsci.2007.05.017 ↗
10. 10.1016/j.ijbiomac.2017.11.02910.1016/j.ijbiomac.2017.11.029 ↗
11. 10.1039/C6TC00678G10.1039/C6TC00678G ↗
12. 10.1039/C7CS00278E10.1039/C7CS00278E ↗
13. 10.1039/C8TA07246A10.1039/C8TA07246A ↗
14. 10.1039/C3CS60235D10.1039/C3CS60235D ↗
15. 10.1002/admt.20160005910.1002/admt.201600059 ↗
16. 10.1002/adfm.20170579510.1002/adfm.201705795 ↗
17. 10.1021/acssuschemeng.6b0195310.1021/acssuschemeng.6b01953 ↗
18. 10.1038/srep3664310.1038/srep36643 ↗
19. 10.1007/s10570-016-1049-010.1007/s10570-016-1049-0 ↗
20. 10.1016/j.msec.2018.01.00710.1016/j.msec.2018.01.007 ↗
21. 10.1016/j.tifs.2008.10.00210.1016/j.tifs.2008.10.002 ↗
22. 10.1016/j.foodhyd.2012.10.00910.1016/j.foodhyd.2012.10.009 ↗
23. 10.1039/C8CS00161H10.1039/C8CS00161H ↗
24. 10.1016/j.progpolymsci.2012.05.00310.1016/j.progpolymsci.2012.05.003 ↗
25. 10.1021/acs.accounts.7b0054810.1021/acs.accounts.7b00548 ↗
26. 10.1002/adma.20170762410.1002/adma.201707624 ↗
27. 10.1007/b11219610.1007/b112196 ↗
28. 10.1126/science.297.5582.80310.1126/science.297.5582.803 ↗
29. 10.1038/nbt0602-60210.1038/nbt0602-602 ↗
30. 10.1039/c0sm00476f10.1039/c0sm00476f ↗
31. 10.1016/j.progpolymsci.2012.02.00110.1016/j.progpolymsci.2012.02.001 ↗
32. 10.1088/1748-6041/8/3/03500610.1088/1748-6041/8/3/035006 ↗
33. 10.1021/bm070423u10.1021/bm070423u ↗
34. 10.1016/j.biomaterials.2007.07.03910.1016/j.biomaterials.2007.07.039 ↗
35. 10.1088/1748-6041/3/3/03410410.1088/1748-6041/3/3/034104 ↗
36. 10.1016/j.biomaterials.2008.09.03810.1016/j.biomaterials.2008.09.038 ↗
37. 10.1016/j.biomaterials.2004.08.00210.1016/j.biomaterials.2004.08.002 ↗
38. 10.1039/c001605e10.1039/c001605e ↗
39. 10.1163/092050609X1256717820416910.1163/092050609X12567178204169 ↗
40. 10.1016/j.biomaterials.2010.08.02210.1016/j.biomaterials.2010.08.022 ↗
41. 10.1021/acsbiomaterials.5b0052510.1021/acsbiomaterials.5b00525 ↗
42. 10.1021/acscentsci.7b0059510.1021/acscentsci.7b00595 ↗
43. 10.1126/scitranslmed.300655710.1126/scitranslmed.3006557 ↗
44. 10.1002/adhm.20150041910.1002/adhm.201500419 ↗
45. 10.1073/pnas.071211710510.1073/pnas.0712117105 ↗
46. 10.1016/S0169-409X(02)00052-210.1016/S0169-409X(02)00052-2 ↗
47. 10.1002/adma.20120044810.1002/adma.201200448 ↗
48. 10.1126/science.118238310.1126/science.1182383 ↗
49. 10.1021/cr300143v10.1021/cr300143v ↗
50. 10.1021/cm061164310.1021/cm0611643 ↗
51. 10.1039/C6SC00142D10.1039/C6SC00142D ↗
52. 10.1038/ncomms846110.1038/ncomms8461 ↗
53. 10.1038/nphoton.2013.24210.1038/nphoton.2013.242 ↗
54. 10.1021/nl072838r10.1021/nl072838r ↗
55. 10.1002/1521-4095(20021203)14:23<1717::AID-ADMA1717>3.0.CO;2-G10.1002/1521-4095(20021203)14:23<1717::AID-ADMA1717>3.0.CO;2-G ↗
56. 10.1021/cm06103210.1021/cm061032 ↗
57. 10.1039/c2lc21176a10.1039/c2lc21176a ↗
58. 10.1155/2012/46050810.1155/2012/460508 ↗
59. 10.1039/C8LC01093E10.1039/C8LC01093E ↗
60. 10.1039/C6LC00046K10.1039/C6LC00046K ↗
61. 10.1039/C5TC00330J10.1039/C5TC00330J ↗
62. 10.1186/s40508-016-0055-810.1186/s40508-016-0055-8 ↗
63. 10.1016/j.msec.2020.11142910.1016/j.msec.2020.111429 ↗
64. 10.1007/s12221-015-5522-410.1007/s12221-015-5522-4 ↗
65. 10.1080/09205063.2017.134892710.1080/09205063.2017.1348927 ↗
66. 10.1016/j.ijbiomac.2014.04.02710.1016/j.ijbiomac.2014.04.027 ↗
67. 10.1007/s10853-019-04271-410.1007/s10853-019-04271-4 ↗
68. 10.1533/9781845695873.14210.1533/9781845695873.142 ↗
69. Kommareddy S. · 2008
70. 10.1016/S0921-0423(03)80005-910.1016/S0921-0423(03)80005-9 ↗
71. 10.3390/polym909040110.3390/polym9090401 ↗
72. DIN EN ISO 14851 Determination of the ultimate aerobic biodegradability of plastic materials in an aqueous medium: Method by measuring the oxygen demand in a closed respirometer2016 https://www.beuth.de/de/norm/din-en-iso-14851/299754641(accessed: March 2020).
73. DIN EN 14995 Plastics – Evaluation of compostability: Test scheme and specifications2007 https://www.beuth.de/de/norm/din-en-14995/90704638(accessed: March 2020).
74. DIN EN 13432 Packaging Requirements for packaging recoverable through composting and biodegradation: Test scheme and evaluation criteria for the final acceptance of packaging2000 https://www.beuth.de/de/norm/din-en-13432/32115376(accessed: March 2020).
75. 10.1016/j.jmbbm.2008.02.00310.1016/j.jmbbm.2008.02.003 ↗
76. 10.1016/j.pmatsci.2007.05.00210.1016/j.pmatsci.2007.05.002 ↗
77. 10.1007/978-1-4757-2257-410.1007/978-1-4757-2257-4 ↗
78. 10.1021/am900403k10.1021/am900403k ↗
79. 10.1039/C7TB00664K10.1039/C7TB00664K ↗
80. 10.1038/s41598-017-04749-810.1038/s41598-017-04749-8 ↗
81. 10.1002/adma.20140316410.1002/adma.201403164 ↗
82. 10.1002/aelm.20180069310.1002/aelm.201800693 ↗
83. 10.1002/adma.20160642510.1002/adma.201606425 ↗
84. Kazem N. · Adv. Mater. · 2017
85. 10.1002/adma.20180185210.1002/adma.201801852 ↗
86. 10.1016/j.jmbbm.2020.10396010.1016/j.jmbbm.2020.103960 ↗
87. 10.1002/admt.20170035110.1002/admt.201700351 ↗
88. 10.1557/mrc.2019.1010.1557/mrc.2019.10 ↗
89. 10.1016/j.microrel.2008.03.02510.1016/j.microrel.2008.03.025 ↗
90. 10.1039/c3sm51360b10.1039/c3sm51360b ↗
91. 10.1016/j.actamat.2013.09.02010.1016/j.actamat.2013.09.020 ↗
92. 10.1002/adfm.20130295710.1002/adfm.201302957 ↗
93. 10.1002/adma.20140153710.1002/adma.201401537 ↗
94. 10.1021/acsami.5b0746410.1021/acsami.5b07464 ↗
95. 10.1002/admi.20170159610.1002/admi.201701596 ↗
96. 10.1088/0964-1726/24/6/06500110.1088/0964-1726/24/6/065001 ↗
97. 10.1039/D0TC04627B10.1039/D0TC04627B ↗
98. 10.1021/acs.chemmater.0c0301910.1021/acs.chemmater.0c03019 ↗