Multiple Fano Resonances Enabled by the Interference between an Out‐of‐Plane Plasmon Mode and Fabry–Pérot Cavity Modes

Abstract Multiple Fano resonances (mFRs) are arising as a promising optical platform to achieve precise sensing and detection. However, experimentally achieving mFRs by simple structures has remained challenging, which impedes the widespread applications of mFRs. Herein a simple structure composed of a single colloidal metal nanoparticle and a transition metal dichalcogenide flake to simultaneously achieve up to 8 FRs in experiments is demonstrated. Combining theoretical and experimental techniques, that an out‐of‐plane plasmon mode of the metal nanoparticle interferes with the Fabry–Pérot cavity modes from the WS₂ flake to form mFRs in the visible region is proved. The simplicity and generality of the method further allow us to systematically study the tunability of the mFRs, in terms of the peak/dip positions and the number of FRs, by changing the structural parameters, which include the thickness of the WS₂ flake, size and shape of the plasmonic nanoparticle. In addition, the quality of the mFRs is proved to be adjustable by tuning the reflectivity of the substrate in the system. The highest quality factor and spectral contrast of the achieved resonances are up to ≈180 and ≈0.95, respectively. The simple structure and high‐quality optical modes will prosper applications in precise sensing and light modulation.