journal article·2023-08Open access

Self‐Assembled Artificial Light‐Harvesting System Constructed Using Electrostatic Interactions in Aqueous Solution for the Sensing of Heavy Metal Cations

Meng Li, Quanyu Shi, Ningxin Song, Zhijun Chen, Lidong Wang, Tony D. James

Advanced Optical Materials· Volume 11· Issue 15

Abstract

Abstract A supramolecular artificial light‐harvesting system (LHS) is successfully constructed in an aqueous environment using carbon dots (CDs) and α, β, γ, δ‐Tetrakis(1‐methylpyridinium‐4‐yl) porphyrin p‐Toluenesulfonate (TMPyP) via electrostatic interactions. Specifically, the CDs act as a donor, and TMPyP, which is loaded to the surface of the CDs, acts as an acceptor for the LHS. Energy transfer occurs from the CDs to the TMPyP in the assembled CDs‐TMPyP upon UV excitation. To demonstrate the applicability, the CDs‐TMPyP system is used as a sensor for Hg(II) in an aqueous solution. Subsequently, a functional material suitable for the detection and removal of Hg(II) is fabricated by integrating the CDs‐TMPyP into a polymer network.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Carbon and Quantum Dots Applications · Luminescence and Fluorescent Materials · Molecular Sensors and Ion Detection

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Hebei Key Lab of Power Plant Flue Gas Multi‐Pollutants Control Department of Environmental Science and Engineering North China Electric Power University Baoding 071003 P. R. China

Key Laboratory of Bio‐based Material Science and Technology of Ministry of Education Material Science and Engineering College Northeast Forestry University Hexing Road 26 Harbin 150040 PR China

Department of Chemistry University of Bath Bath BA2 7AY UK

School of Chemistry and Chemical Engineering Henan Normal University Xinxiang 453007 P. R. China

Funding

National Natural Science Foundation of China · Fundamental Research Funds for the Central Universities · Henan Normal University

References (69)

Show source-provided references
1. 10.1002/adfm.20180727510.1002/adfm.201807275 ↗
2. 10.1002/anie.20211185610.1002/anie.202111856 ↗
3. 10.1002/anie.20220728910.1002/anie.202207289 ↗
4. 10.1002/adma.20220173410.1002/adma.202201734 ↗
5. 10.1021/acssuschemeng.0c0934810.1021/acssuschemeng.0c09348 ↗
6. 10.1021/jacs.9b0840310.1021/jacs.9b08403 ↗
7. 10.1002/admt.20210165610.1002/admt.202101656 ↗
8. 10.1002/anie.20181214610.1002/anie.201812146 ↗
9. 10.1002/adma.20170577810.1002/adma.201705778 ↗
10. 10.1021/jacs.1c1011010.1021/jacs.1c10110 ↗
11. Yu Z. · Angew. Chem., Int. Ed. · 2022 · 13410.1002/ange.202200466 ↗
12. 10.1021/jacs.1c1276710.1021/jacs.1c12767 ↗
13. 10.1021/jacs.1c1029110.1021/jacs.1c10291 ↗
14. 10.1002/adfm.20200154910.1002/adfm.202001549 ↗
15. 10.1002/adfm.20210949210.1002/adfm.202109492 ↗
16. 10.1002/anie.20170208410.1002/anie.201702084 ↗
17. 10.1021/jacs.0c1106010.1021/jacs.0c11060 ↗
18. 10.1021/jacs.9b0806510.1021/jacs.9b08065 ↗
19. 10.1002/adma.20227017510.1002/adma.202270175 ↗
20. 10.1002/anie.20210603510.1002/anie.202106035 ↗
21. 10.1021/acssuschemeng.1c0373710.1021/acssuschemeng.1c03737 ↗
22. 10.1002/adma.20210102610.1002/adma.202101026 ↗
23. 10.1021/ja504730j10.1021/ja504730j ↗
24. 10.1039/c2cs35022j10.1039/c2cs35022j ↗
25. 10.1021/ja404930610.1021/ja4049306 ↗
26. 10.1039/D2NA00934J10.1039/D2NA00934J ↗
27. 10.1021/ja509018g10.1021/ja509018g ↗
28. 10.1002/anie.20110329510.1002/anie.201103295 ↗
29. 10.1021/acsnano.6b0752710.1021/acsnano.6b07527 ↗
30. 10.1002/adma.20150245410.1002/adma.201502454 ↗
31. 10.1039/C4SC00333K10.1039/C4SC00333K ↗
32. 10.1002/adfm.20130117810.1002/adfm.201301178 ↗
33. Zhang X. J. · Angew. Chem., Int. Ed. · 2011 · 50 · 5728
34. 10.1021/jacs.5b0809210.1021/jacs.5b08092 ↗
35. 10.1039/C5CC00398A10.1039/C5CC00398A ↗
36. 10.1002/anie.20160450810.1002/anie.201604508 ↗
37. 10.1002/adom.20200026510.1002/adom.202000265 ↗
38. 10.1002/anie.20180017510.1002/anie.201800175 ↗
39. 10.1002/anie.20170716010.1002/anie.201707160 ↗
40. 10.1038/ncomms1204210.1038/ncomms12042 ↗
41. 10.1002/anie.20160151610.1002/anie.201601516 ↗
42. 10.1039/D1CC01339D10.1039/D1CC01339D ↗
43. 10.1002/anie.20191265410.1002/anie.201912654 ↗
44. 10.1039/D2TA04124C10.1039/D2TA04124C ↗
45. 10.1016/j.jcis.2022.11.15610.1016/j.jcis.2022.11.156 ↗
46. 10.1002/adom.20220171010.1002/adom.202201710 ↗
47. 10.1002/anie.20200342710.1002/anie.202003427 ↗
48. 10.1002/smll.20220436010.1002/smll.202204360 ↗
49. 10.1021/acsami.2c0285110.1021/acsami.2c02851 ↗
50. 10.1016/j.carbpol.2021.11775310.1016/j.carbpol.2021.117753 ↗
51. 10.1021/acs.chemmater.8b0101110.1021/acs.chemmater.8b01011 ↗
52. 10.1007/s12274-014-0644-310.1007/s12274-014-0644-3 ↗
53. 10.1002/anie.20200778610.1002/anie.202007786 ↗
54. 10.1039/C7NR06764J10.1039/C7NR06764J ↗
55. 10.1021/acs.chemmater.9b0217610.1021/acs.chemmater.9b02176 ↗
56. 10.3389/fchem.2019.0044710.3389/fchem.2019.00447 ↗
57. 10.1002/anie.20191134210.1002/anie.201911342 ↗
58. Li M. · Chem. Eng. J. · 2021 · 426
59. 10.1002/adfm.20200703210.1002/adfm.202007032 ↗
60. 10.1016/j.dyepig.2007.04.00710.1016/j.dyepig.2007.04.007 ↗
61. 10.1002/smll.20160345910.1002/smll.201603459 ↗
62. 10.1155/2016/190545410.1155/2016/1905454 ↗
63. 10.1016/j.chemosphere.2019.12455210.1016/j.chemosphere.2019.124552 ↗
64. 10.1016/j.snb.2017.07.12510.1016/j.snb.2017.07.125 ↗
65. 10.1016/j.chemosphere.2019.12455210.1016/j.chemosphere.2019.124552 ↗
66. 10.1039/C7TC05564A10.1039/C7TC05564A ↗
67. 10.1016/j.jhazmat.2018.05.05510.1016/j.jhazmat.2018.05.055 ↗
68. 10.1021/acssuschemeng.9b0213910.1021/acssuschemeng.9b02139 ↗
69. 10.1016/j.jhazmat.2020.12335910.1016/j.jhazmat.2020.123359 ↗