Tunable Microlasers Modulated by Intracavity Spherical Confinement with Chiral Liquid Crystal

Abstract Manipulation of laser emission offers promising opportunities for the generation of new spatial dimensions and applications, particularly in nanophotonics, super‐resolution imaging, and data transfer devices. However, the ability to control laser modes and wavelength in a microcavity remains challenging. Here, a novel approach is demonstrated to control laser modes by manipulating the 3D‐optical confinement, chirality, and orientations in a Fabry−Pérot microcavity with cholesteric liquid crystal droplets. Different configurations of intracavity micro‐/nanostructures generate versatile dimensions of laser modes, while the significantly reduced laser mode volume further leads to single‐mode lasing. Theoretical analysis is carried out to support this interesting discovery. Finally, switchable lasing wavelength with various surface anchoring forces and pH interactions is demonstrated. This novel concept not only provides a simple yet highly versatile method to manipulate laser emissions, but deepens insight into how molecules interact with and modulate laser light, laying the foundation for the development of tunable photonic devices at the molecular level. Promising applications include highly selective laser devices, laser‐emission imaging, and bioinspired sensing.