journal article·2018-09

Ultrafast Multilevel Optical Tuning with CSb2Te3 Thin Films

Yun Meng, Jitendra K. Behera, Shuai Wen, Robert E. Simpson, Jianjun Shi, Liangcai Wu, Zhitang Song, Jingsong Wei, Yang Wang

Advanced Optical Materials· Volume 6· Issue 17
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Abstract

Abstract Tunable and reconfigurable functionalities are crucial for advanced photonic devices. In this study, CSb2Te3 is proposed as a new optical tuning material. Single‐shot picosecond laser pulses are used to transform the CSb2Te3 into six different optical states; each optical state can be achieved from any other state. The dielectric function for each optical state is unique and the switching is achieved on a picosecond time scale. The impact of the crystal structure on the optical tuning mechanism is studied using transmission electron microscopy and density functional theory. Second harmonic generation in the CSb2Te3 films indicates that the crystal orientation for the switched layer is influenced by the pump laser polarization. Thus electric field may provide a further degree of freedom to design phase change materials.
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Research context

OpenAlex topics: Phase-change materials and chalcogenides · Solid State Laser Technologies · Photorefractive and Nonlinear Optics

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Affiliations

Key Laboratory of High Power Laser Materials Shanghai Institute of Optics and Fine Mechanics Chinese Academy of Sciences Shanghai 201800 China

University of the Chinese Academy of Sciences Beijing 100080 China

ACTA Lab Singapore University of Technology and Design 8 Somapah Road Singapore 487372 Singapore

College of Science Donghua University Shanghai 201620 China

State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Micro‐system and Information Technology Chinese Academy of Sciences Shanghai 200050 China

Funding

National Natural Science Foundation of China

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