Dynamic Structural Color from Wrinkled Thin Films

Abstract Structural color caused by thin‐film interference is widespread and simple in nature. Many researchers have already showed the reversible color change of structural color system, but it is difficult to regulate dynamically with tunable intensity and viewable angle. Herein, a dynamic structural color platform is reported by combining spontaneous thin film interference and wrinkling phenomenon in nature. This robust yet low cost strategy enables large‐scale and spatially arbitrary preparation of a uniform structural color surface through the whole visible spectral range. Furthermore, the prepared isotropic and anisotropic structural colors on disordered and ordered wrinkled thin films (WTFs) exhibit different optical properties that can be precisely and reversibly regulated by ultraviolet (UV) light and near‐infrared (NIR) light irradiation. This exquisite and tunable structural color platform may find applications in information storage, smart display, anticounterfeiting and encryption.