journal article·2022-12

Efficient InP Green Quantum‐Dot Light‐Emitting Diodes Based on Organic Electron Transport Layer

Peili Gao, Yong Zhang, Pan Qi, Shuming Chen

Advanced Optical Materials· Volume 10· Issue 24
Publisher page

Abstract

Abstract ZnMgO thin film is commonly used as an electron transport layer (ETL) in quantum‐dot light‐emitting diodes (QLEDs); however, it often induces the problems of interface exciton quenching and electron over‐injection in the devices. Herein, an organic molecule 2,4,6‐tris(3‐(diphenylphosphoryl)phenyl)‐1,3,5‐triazine (PO‐T2T) is investigated as a ETL material for InP green QLEDs. Due to the high injection barrier and moderate electron mobility, the PO‐T2T can prevent electron over‐injection and accumulation in the InP QLEDs. Besides, with the organic ETL, the interfacial exciton quenching is effectively suppressed. By depositing the PO‐T2T using a solution‐assisted evaporation method, efficient InP green QLEDs are achieved, which exhibit a maximum external quantum efficiency of 15.0% and a luminance of 10 010 cd m−2, corresponding to 211% and 237% enhancements, respectively, compared to 7.1% and 4207 cd m−2 of the devices with ZnMgO ETL.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Quantum Dots Synthesis And Properties · Nanocluster Synthesis and Applications · Organic Light-Emitting Diodes Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Electrical and Electronic Engineering Southern University of Science and Technology Shenzhen 518055 P. R. China

School of Semiconductor Science and Technology South China Normal University Guangzhou 510631 P. R. China

College of Intelligent Manufacturing Guangzhou Panyu Polytechnic Guangzhou 511483 P. R. China

Funding

National Natural Science Foundation of China

References (54)

Show source-provided references
1. 10.1038/nphoton.2012.32810.1038/nphoton.2012.328 ↗
2. 10.1038/s41566-022-00999-910.1038/s41566-022-00999-9 ↗
3. 10.1038/nature1382910.1038/nature13829 ↗
4. 10.1038/s41566-019-0364-z10.1038/s41566-019-0364-z ↗
5. 10.1021/acsnano.7b0786710.1021/acsnano.7b07867 ↗
6. 10.1016/j.biomaterials.2011.10.07010.1016/j.biomaterials.2011.10.070 ↗
7. 10.1021/acsenergylett.9b0282410.1021/acsenergylett.9b02824 ↗
8. 10.1002/smll.20200245410.1002/smll.202002454 ↗
9. 10.1038/s41586-019-1771-510.1038/s41586-019-1771-5 ↗
10. 10.1038/s43246-021-00203-510.1038/s43246-021-00203-5 ↗
11. 10.1002/advs.20220095910.1002/advs.202200959 ↗
12. 10.1002/aelm.20220025610.1002/aelm.202200256 ↗
13. 10.1038/ncomms366110.1038/ncomms3661 ↗
14. 10.1021/acsnano.9b0487910.1021/acsnano.9b04879 ↗
15. 10.1002/adpr.20220015910.1002/adpr.202200159 ↗
16. 10.1002/adma.20200617810.1002/adma.202006178 ↗
17. 10.1007/s12274-021-3354-710.1007/s12274-021-3354-7 ↗
18. 10.1021/acsami.8b0472110.1021/acsami.8b04721 ↗
19. 10.1016/j.cap.2019.05.01610.1016/j.cap.2019.05.016 ↗
20. 10.1021/nn403594j10.1021/nn403594j ↗
21. 10.1002/smll.20160396210.1002/smll.201603962 ↗
22. 10.1109/LED.2021.311932210.1109/LED.2021.3119322 ↗
23. 10.1021/acsami.2c0169910.1021/acsami.2c01699 ↗
24. 10.1021/acsenergylett.2c0106510.1021/acsenergylett.2c01065 ↗
25. 10.1002/adfm.20200768610.1002/adfm.202007686 ↗
26. 10.1002/adfm.20200576510.1002/adfm.202005765 ↗
27. 10.1038/srep0516110.1038/srep05161 ↗
28. 10.1039/C9MH00373H10.1039/C9MH00373H ↗
29. 10.1021/acsami.6b0762910.1021/acsami.6b07629 ↗
30. 10.1016/j.scib.2020.08.02510.1016/j.scib.2020.08.025 ↗
31. 10.1021/acsaelm.0c0043110.1021/acsaelm.0c00431 ↗
32. 10.1002/adfm.20080104510.1002/adfm.200801045 ↗
33. 10.1039/b926348a10.1039/b926348a ↗
34. 10.1002/adfm.20070091310.1002/adfm.200700913 ↗
35. 10.1021/cm201550w10.1021/cm201550w ↗
36. 10.1021/acs.chemmater.8b0204910.1021/acs.chemmater.8b02049 ↗
37. 10.1364/OME.4.00143610.1364/OME.4.001436 ↗
38. 10.1364/OME.4.00143610.1364/OME.4.001436 ↗
39. 10.1007/s13391-015-4420-710.1007/s13391-015-4420-7 ↗
40. 10.1002/adfm.20150554910.1002/adfm.201505549 ↗
41. 10.1021/acsomega.9b0147110.1021/acsomega.9b01471 ↗
42. 10.1039/C9CC06882A10.1039/C9CC06882A ↗
43. 10.1002/adom.20180160210.1002/adom.201801602 ↗
44. 10.1021/acs.jpclett.0c0011210.1021/acs.jpclett.0c00112 ↗
45. 10.1063/5.002074210.1063/5.0020742 ↗
46. 10.1021/acsenergylett.1c0106710.1021/acsenergylett.1c01067 ↗
47. 10.1002/adfm.20200845310.1002/adfm.202008453 ↗
48. 10.1007/s12274-021-3596-410.1007/s12274-021-3596-4 ↗
49. 10.1109/LED.2022.314735010.1109/LED.2022.3147350 ↗
50. 10.1039/D2TC01522F10.1039/D2TC01522F ↗
51. 10.1002/advs.20220095910.1002/advs.202200959 ↗
52. 10.1038/s41377-022-00855-z10.1038/s41377-022-00855-z ↗
53. 10.1002/adom.20190136210.1002/adom.201901362 ↗
54. 10.1007/s10854-020-05206-510.1007/s10854-020-05206-5 ↗