journal article·2021-07Open access

Interfacial Adhesion of Mussel‐Inspired Hydrogels: Interfacial Adhesion of Fully Transient, Mussel‐Inspired Hydrogels with Different Network Crosslink Modalities (Adv. Mater. Interfaces 14/2021)

Daniel R. Darby, Erica Lai, Niels Holten‐Andersen, Jonathan T. Pham

Advanced Materials Interfaces· Volume 8· Issue 14

Abstract

Fully transient, mussel-inspired hydrogels are supramolecular networks where polymers are crosslinked by reversible, metal-ligand coordination bonds. In article number 2100319, Niels Holten-Andersen, Jonathan T. Pham, and co-workers demonstrate an inverse correlation between tris- coordinate crosslinks and peak adhesive stress for hydrogels comprising either histidine-Ni2+ ion crosslinks or nitrodopamine-Fe3+ ion crosslinks. This exhibits tunability of supramolecular hydrogels for soft materials and interfacial applications.
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Research context

OpenAlex topics: biodegradable polymer synthesis and properties · Polymer Surface Interaction Studies · Hydrogels: synthesis, properties, applications

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Affiliations

Department of Chemical and Materials Engineering University of Kentucky Lexington KY 40506 USA

Department of Materials Science and Engineering Massachusetts Institute of Technology Cambridge MA 02139 USA

References

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