Controlling Magnetic Properties at BiFe1−xMnxO3/La2/3Ca1/3MnO3 Interfaces by Tuning the Spatial Distribution of Interfacial Electronic States
Source abstract
Abstract
Abstract One major challenge in engineering the magnetism of oxide heterostructures is controlling orbital reconstruction by tuning the charge transfer effect. This paper investigates the forward and backward charge transfer effect and the induced magnetic properties of BiFe1−xMnxO3/La2/3Ca1/3MnO3 heterostructures. Interfacial ferromagnetism is found to be qualitatively tunable by tuning the spatial distribution of interfacial electronic states. The subtle balance of magnetic coupling between FeOMn and MnOMn changed as the electronic structures are modified by charge transfer. The ions' valence is strongly correlated with the interfacial magnetic properties, extending the concept of the charge degrees of freedom affecting the magnetic coupling properties.
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Research context
OpenAlex topics: Magnetic and transport properties of perovskites and related materials · Multiferroics and related materials · Electronic and Structural Properties of Oxides
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Hebei Key Lab of Optic‐electronic Information and Materials The College of Physics Science and Technology Hebei University Baoding 071002 P. R. China
Nanostructures Research Laboratory Japan Fine Ceramics Center Nagoya 456‐8587 Japan
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences Beijing 100190 P. R. China
Department of Materials Science and Engineering Virginia Tech Blacksburg VA 24061 USA
Funding
National Natural Science Foundation of China
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