DataVXAdvanced MaterialsPaper
journal article·2019-04Open access

Single‐Atom Catalysis: Mixed‐Valence Single‐Atom Catalyst Derived from Functionalized Graphene (Adv. Mater. 17/2019)

Aristides Bakandritsos, Ravishankar G. Kadam, Pawan Kumar, Giorgio Zoppellaro, Miroslav Medved', Jiří Tuček, Tiziano Montini, Ondřej Tomanec, Pavlína Andrýsková, Bohuslav Drahoš, Rajender S. Varma, Michal Otyepka, Manoj B. Gawande, Paolo Fornasiero, Radek Zbořil

Advanced Materials· Volume 31· Issue 17
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Source abstract

Abstract

Metal–metal cooperation in a solid-state mixed-valence single-atom catalyst, boosts yield and selectivity in oxidative amine coupling, with uncompromised reusability, as shown by Manoj B. Gawande, Paolo Fornasiero, Radek Zbořil, and co-workers in article number 1900323. The catalyst, stemming from the chemical entrapment and partial reduction of Cu(II) ions on cyanographene, lays the ground for the exploitation of the large family of covalent graphene derivatives as versatile 2D coordination ligands, beyond the porphyrin motif in nitrogen-doped graphenes.
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Research context

NanomaterialsCatalysis & surfaces

OpenAlex topics: Covalent Organic Framework Applications · Nanomaterials for catalytic reactions · Catalytic Processes in Materials Science

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Affiliations

Regional Centre of Advanced Technologies and Materials Department of Physical Chemistry Faculty of Science Palacký University Olomouc Šlechtitelu˚ 27 783 71 Olomouc Czech Republic

Department of Chemical and Pharmaceutical Sciences INSTM Trieste Research Unit and ICCOM‐CNR Trieste Research Unit University of Trieste via L. Giorgieri 1 I‐34127 Trieste Italy

Regional Centre of Advanced Technologies and Materials Department of Inorganic Chemistry Faculty of Science Palacký University Olomouc 17. listopadu 12 771 46 Olomouc Czech Republic

References

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