journal article·2022-07Open access

Porous fixed-bed photoreactor for boosting C–C coupling in photocatalytic CO2 reduction

Shengjie Bai, Haoran Qiu, Mengmeng Song, Guiwei He, Feng Wang, Ya Liu, Liejin Guo

eScience· Volume 2· Issue 4

Abstract

Solar-driven CO2 conversion to chemical fuels in an aqueous solution is restricted not only by photocatalysts but also by mass transfer. Here, a regulatable three-phase interface on a porous fixed-bed is constructed for efficient C–C coupling in photocatalytic CO2 reduction. The photocatalytic results show that ∼90% selectivity towards C2+ products is obtained by a Cu/Cd0.5Zn0.5S photocatalyst, with a yield of 6.54 ​μmol/h (an irradiation area of 0.785 cm2), while only 0.94 ​μmol/h (an irradiation area of 19.625 cm2) is achieved with a commonly used suspension photocatalytic reactor. We find that under the same CO2 feed rate, the local CO2 concentration in this porous fixed-bed photoreactor is obviously higher than in the suspension photoreactor. The larger local CO2 coverage derived from a higher CO2 supply and aggregation enhances the C–C coupling, thereby generating more C2+. Even an observable three-phase interface on the porous fixed-bed can be regulated by adjusting the CO2 supply, for which the optimal gas inlet rate is 5–10 sccm.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Advanced Photocatalysis Techniques · CO2 Reduction Techniques and Catalysts · Catalytic Processes in Materials Science

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (59)

Show source-provided references
1. How to make an efficient gas-phase heterogeneous CO2 hydrogenation photocatalyst10.1039/D0EE01124J ↗
2. Regulating the ∗OCCHO intermediate pathway towards highly selective photocatalytic CO2 reduction to CH3CHO over locally crystallized carbon nitride10.1039/D1EE02073K ↗
3. Systematic assessment of solvent selection in photocatalytic CO2 reduction10.1021/acsenergylett.1c01522 ↗
4. S-Scheme heterojunction photocatalyst for CO2 photoreduction
5. Recent advances in surface-modified g-C3N4-based photocatalysts for H2 production and CO2 reduction
6. Photoelectrochemical technology for solar fuel generation, from single photoelectrodes to unassisted cells: a review10.1007/s10311-021-01364-y ↗
7. Comparative analysis of solar-to-fuel conversion efficiency: a direct, one-step electrochemical CO2 reduction reactor versus a two-step, cascade electrochemical CO2 reduction reactor10.1021/acsenergylett.8b01077 ↗
8. Addressing the stability gap in photoelectrochemistry: molybdenum disulfide protective catalysts for tandem III-V unassisted solar water splitting10.1021/acsenergylett.0c01132 ↗
9. Visible-light-driven methane formation from CO2 with a molecular iron catalyst10.1038/nature23016 ↗
10. Ni single-atom sites supported on carbon aerogel for highly efficient electroreduction of carbon dioxide with industrial current densities10.1016/j.esci.2022.03.007 ↗
11. Photocatalytic conversion of CO2 into value-added and renewable fuels10.1016/j.apsusc.2015.03.050 ↗
12. Photocatalytic CO2 reduction by carbon-coated Indium-Oxide nanobelts10.1021/jacs.7b00266 ↗
13. Design and fabrication of semiconductor photocatalyst for photocatalytic reduction of CO2 to solar fuel10.1007/s40843-014-0003-1 ↗
14. Enhanced photocatalytic CO2 reduction over 2D/1D BiOBr0.5Cl0.5/WO3 S-scheme heterostructure
15. Solar-heating boosted catalytic reduction of CO2 under full-solar spectrum10.1016/S1872-2067(19)63393-0 ↗
16. Step-scheme CdS/TiO2 nanocomposite hollow microsphere with enhanced photocatalytic CO2 reduction activity10.1016/j.jmst.2020.02.062 ↗
17. Cooperative syngas production and C-N bond formation in one photoredox cycle10.1002/ange.202015756 ↗
18. Cu2O nanocubes with mixed oxidation-state facets for (photo)catalytic hydrogenation of carbon dioxide10.1038/s41929-019-0338-z ↗
19. Photo-enhanced thermal catalytic CO2 methanation activity and stability over oxygen-deficient Ru/TiO2 with exposed TiO2 {001} facets: adjusting photogenerated electron behaviors by metal-support interactions10.1016/S1872-2067(21)63825-1 ↗
20. Managing hydration at the cathode enables efficient CO2 electrolysis at commercially relevant current densities10.1021/acsenergylett.0c00637 ↗
21. Active-Site modulation in an Fe-porphyrin-based metal-organic framework through ligand axial coordination: accelerating electrocatalysis and charge-transport kinetics10.1021/jacs.9b11355 ↗
22. Product selectivity of photocatalytic CO2 reduction reactions10.1016/j.mattod.2019.06.009 ↗
23. A critical review on TiO2 based photocatalytic CO2 reduction system: strategies to improve efficiency10.1016/j.jcou.2018.04.026 ↗
24. Photocatalytic uphill conversion of natural gas beyond the limitation of thermal reaction systems10.1038/s41929-019-0419-z ↗
25. Thermal coupled photoconductivity as a tool to understand the photothermal catalytic reduction of CO210.1016/S1872-2067(19)63475-3 ↗
26. Photoredox coupling of benzyl alcohol oxidation with CO2 reduction over CdS/TiO2 heterostructure under visible light irradiation10.1016/j.apcatb.2022.121158 ↗
27. Copper and platinum dual-single-atoms supported on crystalline graphitic carbon nitride for enhanced photocatalytic CO2 reduction10.1016/S1872-2067(21)63879-2 ↗
28. Structural engineering of 3D hierarchical Cd0.8Zn0.2S for selective photocatalytic CO2 reduction10.1016/S1872-2067(20)63623-3 ↗
29. 2D/2D black phosphorus/g-C3N4 S-Scheme heterojunction photocatalysts for CO2 reduction investigated using DFT calculations
30. Construction of Z-scheme In2S3-TiO2 for CO2 reduction under concentrated natural sunlight[J]
31. Enhanced CO2 electrolysis with metal-oxide interface structures
32. Graphdiyne: a new photocatalytic CO2 reduction cocatalyst10.1002/adfm.201904256 ↗
33. Facet-dependent active sites of a single Cu2O particle photocatalyst for CO2 reduction to methanol10.1038/s41560-019-0490-3 ↗
34. Nanostructured metal phosphides: from controllable synthesis to sustainable catalysis10.1039/D1CS00323B ↗
35. Surface strategies for particulate photocatalysts toward artificial photosynthesis10.1016/j.joule.2018.07.030 ↗
36. 3D porous Cu-NPs/g-C3N4 foam with excellent CO2 adsorption and Schottky junction effect for photocatalytic CO2 reduction10.1016/j.apsusc.2019.144347 ↗
37. Photocatalytic CO2 reduction to C2+ products10.1021/acscatal.0c00478 ↗
38. Three-phase photocatalysis for the enhanced selectivity and activity of CO2 reduction on a hydrophobic surface10.1002/anie.201908058 ↗
39. Improving artificial photosynthesis over carbon nitride by gas-liquid-solid interface management for full light-induced CO2 reduction to C1 and C2 fuels and O210.1002/cssc.201903515 ↗
40. Photocatalytic hydrogen production using twinned nanocrystals and an unanchored NiSx co-catalyst10.1038/nenergy.2016.151 ↗
41. Twin-induced one-dimensional homojunctions yield high quantum efficiency for solar hydrogen generation10.1038/ncomms3278 ↗
42. Atomic-scale spacing between copper facets for the electrochemical reduction of carbon dioxide
43. CO2 hydrogenation to ethanol over Cu@Na-Beta10.1016/j.chempr.2020.07.001 ↗
44. Electrocatalytic reduction of CO2 to ethylene and ethanol through hydrogen-assisted C–C coupling over fluorine-modified copper10.1038/s41929-020-0450-0 ↗
45. Improving selectivity and activity of CO2 reduction photocatalysts with oxygen10.1016/j.chempr.2019.04.006 ↗
46. Photo-generated dinuclear {Eu(II)}2 active sites for selective CO2 reduction in a photosensitizing metal-organic framework10.1038/s41467-018-05659-7 ↗
47. Rationally designed transition metal hydroxide nanosheet arrays on graphene for artificial CO2 reduction10.1038/s41467-020-18944-1 ↗
48. Enhanced catalytic reaction at an air-liquid-solid triphase interface10.1039/C9SC06505A ↗
49. Efficient wettability-controlled electroreduction of CO2 to CO at Au/C interfaces10.1038/s41467-020-16847-9 ↗
50. Modulating local CO2 concentration as a general strategy for enhancing C–C coupling in CO2 electroreduction10.1016/j.joule.2020.03.013 ↗
51. Mechanistic insights into electrochemical reduction of CO2 over Ag using density functional theory and transport models10.1073/pnas.1713164114 ↗
52. Photocatalytic and electrocatalytic transformations of C1 molecules involving C–C coupling, Energy
53. MOF-templated preparation of highly dispersed Co/Al2O3 composite as the photothermal catalyst with high solar-to-fuel efficiency for CO2 methanation10.1021/acsami.0c11576 ↗
54. Unravelling the CC coupling in CO2 photocatalytic reduction with H2O on Au/TiO2-x: combination of plasmonic excitation and oxygen vacancy10.1016/j.apcatb.2021.120147 ↗
55. Cocatalysts for selective photoreduction of CO2 into solar fuels10.1021/acs.chemrev.8b00400 ↗
56. Amine-modified S-scheme porous g-C3N4/CdSe-diethylenetriamine composite with enhanced photocatalytic CO2 reduction activity10.1021/acsaem.0c02896 ↗
57. Understanding selectivity for the electrochemical reduction of carbon dioxide to formic acid and carbon monoxide on metal electrodes10.1021/acscatal.7b00687 ↗
58. Numerical study of flow reversal during bubble growth and confinement of flow boiling in microchannels10.1016/j.ijheatmasstransfer.2021.121491 ↗
59. VOF modelling of gas-liquid flow in PEM water electrolysis cell micro-channels10.1016/j.ijhydene.2017.05.079 ↗