Two-Dimensional OER Catalysts: Is There a Win-Win Solution for Their Activity and Stability?
Source abstract
Abstract
Since the oxygen evolution reaction (OER) is the critical half reaction for highly efficient water splitting, OER catalysts with synergistically enhanced activity and stability are now under vigorous development. Two dimensional (2D) OER catalysts possess unique structural characteristics with tunable surface chemistry and electronic properties and thus have received extensive investigation. High activity and high stability of the catalysts are often incompatible because the highly active catalytic species on the 2D framework tend to degrade or reconstruct under the OER operating conditions, which is unfavorable for the long-term stability. In this review, we emphasize the relationship between activity and stability from the perspective of the mechanisms of the OER, the current progress, and the challenges over the widely explored 2D OER catalysts. We will analyze the reconstruction and degradation processes of these catalysts and outline rational strategies to synergistically enhance their activity and stability.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Electrocatalysts for Energy Conversion · Catalytic Processes in Materials Science · Advanced battery technologies research
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Guangdong Provincial Key Laboratory of Nano-Micro Materials Research, School of Advanced Materials, Peking University Shenzhen Graduate School, Shenzhen 518055, China
School of Energy and Environment, City University of Hong Kong, Kowloon, Hong Kong SAR 999077, China
College of Chemistry and Chemical Engineering, Qiqihar University, Qiqihar 161006, China
Institute of Biomedical Engineering, Shenzhen Bay Laboratory, Shenzhen 518055, China
CAS-HKU Joint Laboratory on New Materials & Department of Chemistry, The University of Hong Kong, Pokfulam Road, Hong Kong SAR, 999077, China
Funding
Guangdong Provincial Department of Science and Technology · Research Grants Council, University Grants Committee · Shenzhen Fundamental Research Program · City University of Hong Kong · National Natural Science Foundation of China · Guangdong-Hong Kong-Macao Joint Innovation Foundation
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