journal article·2023-06Open access

Light‐Induced Giant Rashba Spin–Orbit Coupling at Superconducting KTaO3(110) Heterointerfaces

Yulin Gan, Fazhi Yang, Lingyuan Kong, Xuejiao Chen, Hao Xu, Jin Zhao, Gang Li, Yuchen Zhao, Lei Yan, Zhicheng Zhong, Yunzhong Chen, Hong Ding

Advanced Materials· Volume 35· Issue 25

Abstract

Abstract The 2D electron system (2DES) at the KTaO3 surface or heterointerface with 5d orbitals hosts extraordinary physical properties, including a stronger Rashba spin–orbit coupling (RSOC), higher superconducting transition temperature, and potential of topological superconductivity. Herein, a huge enhancement of RSOC under light illumination achieved at a superconducting amorphous‐Hf0.5Zr0.5O2/KTaO3(110) heterointerfaces is reported. The superconducting transition is observed with Tc = 0.62 K and the temperature‐dependent upper critical field reveals the interaction between spin–orbit scattering and superconductivity. A strong RSOC with Bso = 1.9 T is revealed by weak antilocalization in the normal state, which undergoes sevenfold enhancement under light illumination. Furthermore, RSOC strength develops a dome‐shaped dependence of carrier density with the maximum of Bso = 12.6 T achieved near the Lifshitz transition point nc ≈ 4.1 × 1013 cm−2. The highly tunable giant RSOC at KTaO3(110)‐based superconducting interfaces show great potential for spintronics.
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Research context

OpenAlex topics: Electronic and Structural Properties of Oxides · Magnetic and transport properties of perovskites and related materials · Advanced Condensed Matter Physics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Beijing National Laboratory of Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences Beijing 100190 China

Key Laboratory of Magnetic Materials and Devices and Zhejiang Province Key Laboratory of Magnetic Materials and Application Technology Ningbo Institute of Materials Technology and Engineering (NIMTE) Chinese Academy of Sciences Ningbo 315201 China

Tsung‐Dao Lee Institute & School of Physics and Astronomy Shanghai Jiao Tong University Shanghai 200240 China

CAS Center for Excellence in Topological Quantum Computation University of Chinese Academy of Sciences Beijing 100190 China

Funding

National Natural Science Foundation of China · National Key Research and Development Program of China · China Postdoctoral Science Foundation

References (65)

Show source-provided references
1. 10.1038/nmat436010.1038/nmat4360 ↗
2. 10.1038/s41928-019-0273-710.1038/s41928-019-0273-7 ↗
3. 10.1038/nature1982010.1038/nature19820 ↗
4. 10.1038/s41578-021-00395-910.1038/s41578-021-00395-9 ↗
5. 10.1103/PhysRevLett.68.10610.1103/PhysRevLett.68.106 ↗
6. 10.1103/PhysRevB.101.20541410.1103/PhysRevB.101.205414 ↗
7. 10.1103/PhysRevLett.106.16680510.1103/PhysRevLett.106.166805 ↗
8. 10.1103/PhysRevLett.104.12680310.1103/PhysRevLett.104.126803 ↗
9. 10.1021/acs.nanolett.7b0212810.1021/acs.nanolett.7b02128 ↗
10. 10.1038/nmat472610.1038/nmat4726 ↗
11. 10.1038/s41586-018-0770-210.1038/s41586-018-0770-2 ↗
12. 10.1038/nature0757610.1038/nature07576 ↗
13. 10.1021/acs.nanolett.2c0099210.1021/acs.nanolett.2c00992 ↗
14. 10.1038/nmat367410.1038/nmat3674 ↗
15. 10.1103/PhysRevLett.107.05680210.1103/PhysRevLett.107.056802 ↗
16. 10.1103/PhysRevB.98.07540910.1103/PhysRevB.98.075409 ↗
17. 10.1038/srep1530210.1038/srep15302 ↗
18. 10.1038/s41928-020-0383-210.1038/s41928-020-0383-2 ↗
19. 10.1103/PhysRevLett.126.05770110.1103/PhysRevLett.126.057701 ↗
20. 10.1021/acsnano.8b0762210.1021/acsnano.8b07622 ↗
21. 10.1126/science.aba551110.1126/science.aba5511 ↗
22. 10.1103/PhysRevLett.126.02680210.1103/PhysRevLett.126.026802 ↗
23. 10.1126/sciadv.abn427310.1126/sciadv.abn4273 ↗
24. 10.1073/pnas.131830411110.1073/pnas.1318304111 ↗
25. 10.1126/science.119878110.1126/science.1198781 ↗
26. 10.1007/s11664-022-09844-910.1007/s11664-022-09844-9 ↗
27. 10.1038/s41535-022-00506-x10.1038/s41535-022-00506-x ↗
28. 10.1126/science.abb384810.1126/science.abb3848 ↗
29. 10.1103/PhysRev.147.29510.1103/PhysRev.147.295 ↗
30. 10.1088/1674-1056/27/10/10740110.1088/1674-1056/27/10/107401 ↗
31. 10.1103/PhysRevB.100.12513410.1103/PhysRevB.100.125134 ↗
32. 10.1103/PhysRevB.92.07530910.1103/PhysRevB.92.075309 ↗
33. 10.1016/0370-1573(84)90103-010.1016/0370-1573(84)90103-0 ↗
34. 10.1021/acs.jpclett.2c0038410.1021/acs.jpclett.2c00384 ↗
35. 10.1103/PhysRevLett.89.04680110.1103/PhysRevLett.89.046801 ↗
36. 10.1021/acsnano.0c0759810.1021/acsnano.0c07598 ↗
37. 10.1103/PhysRevResearch.4.01303910.1103/PhysRevResearch.4.013039 ↗
38. 10.1103/PhysRevB.102.12514510.1103/PhysRevB.102.125145 ↗
39. 10.1016/0008-6223(76)90077-410.1016/0008-6223(76)90077-4 ↗
40. 10.1103/PhysRevLett.94.18680510.1103/PhysRevLett.94.186805 ↗
41. 10.1103/PhysRevB.96.16130310.1103/PhysRevB.96.161303 ↗
42. 10.1038/ncomms211610.1038/ncomms2116 ↗
43. 10.1002/adma.20180597010.1002/adma.201805970 ↗
44. 10.1002/admi.20220010310.1002/admi.202200103 ↗
45. 10.1103/PhysRevB.87.16110210.1103/PhysRevB.87.161102 ↗
46. 10.1038/ncomms702810.1038/ncomms7028 ↗
47. 10.1103/PhysRevLett.119.23700210.1103/PhysRevLett.119.237002 ↗
48. 10.1002/adma.20210210210.1002/adma.202102102 ↗
49. 10.1002/qute.20200008110.1002/qute.202000081 ↗
50. 10.1103/PhysRevB.96.02450910.1103/PhysRevB.96.024509 ↗
51. 10.1143/JPSJ.77.03100810.1143/JPSJ.77.031008 ↗
52. 10.1103/PhysRevLett.78.133510.1103/PhysRevLett.78.1335 ↗
53. 10.1103/PhysRevB.74.03330210.1103/PhysRevB.74.033302 ↗
54. 10.1126/science.117366710.1126/science.1173667 ↗
55. 10.1063/1.10273010.1063/1.102730 ↗
56. 10.1038/s41467-022-33621-110.1038/s41467-022-33621-1 ↗
57. 10.1038/s41578-018-0003-110.1038/s41578-018-0003-1 ↗
58. 10.1103/PhysRevLett.121.11680310.1103/PhysRevLett.121.116803 ↗
59. 10.1126/science.aax144410.1126/science.aax1444 ↗
60. 10.1103/PhysRevB.90.16510810.1103/PhysRevB.90.165108 ↗
61. 10.1002/aelm.20180086010.1002/aelm.201800860 ↗
62. 10.1103/PhysRevB.106.12512710.1103/PhysRevB.106.125127 ↗
63. 10.1088/2515-7639/acb01710.1088/2515-7639/acb017 ↗
64. P.Krantz A.Tyner P.Goswami V.Chandrasekhar arXiv: 2209.10534v2 2022.
65. 10.1038/s42254-022-00490-y10.1038/s42254-022-00490-y ↗