journal article·2025-02

Ultra‐Narrowband Green‐Emitting Transparent Composite Ceramics for Laser‐Driven Display

Dahai Hu, Shisheng Lin, Tao Pang, Lingwei Zeng, Guoyu Xi, Fengluan You, TianShuo Wu, Xiaoshuang Li, Bo Wang, Lei Lei, Feng Huang, Daqin Chen

Advanced Materials· Volume 37· Issue 7
Publisher page

Abstract

Abstract Laser‐driven projection displays face a critical challenge in developing laser‐excitable and high‐performance narrowband green emitters. Herein, new Al2O3‐LaMgAl11O19: Mn2+ (Al2O3‐LMA: Mn2+) transparent composite ceramics are reported via high‐temperature vacuum sintering, which produces a high‐color‐purity (95.4%) green emission with full width at half maximum of 24 nm and superior thermal and moisture and laser irradiation stability. These are attributed to low electron‐phonon couple, weak crystal‐field effect, an individual lattice location of Mn2+ activators in high structural rigid host, and the incorporation of a high‐thermal‐conductivity Al2O3 secondary phase. As a result, the composite ceramics are demonstrated as an attractive color converter with a high external quantum efficiency (38%) and absorption coefficient (53%), which ensures a luminous flux of 2012 lm @40.0 W, a luminous efficacy of 67.7 lm W−1, and a green light conversion efficiency of 20.3% upon blue laser irradiation. This enables to construct a brand‐new laser‐driven prototype display with a record color gamut beyond Rec.2020 standard (100.8%), outperforming commercial YAG: Ce3+ and β‐SiAlON: Eu2+. This exploration in ultra‐narrowband green luminescent materials is poised to accelerate the development of “ideal displays” for laser‐driven projection display technology.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Luminescence Properties of Advanced Materials · Photonic Crystals and Applications · Glass properties and applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

College of Physics and Energy Fujian Normal University Fuzhou Fujian 350117 P. R. China

Huzhou Key Laboratory of Materials for Energy Conversion and Storage College of Science Huzhou University Huzhou Zhejiang 313000 P. R. China

School of Chemistry and Chemical Engineering Hunan University of Science and Technology Xiangtan Hunan 411201 P. R. China

School of Applied Physics and Materials Wuyi University Jiangmen Guangdong 529020 P. R. China

Institute of Optoelectronic Materials and Devices China Jiliang University Hangzhou Zhejiang 310018 P. R. China

Fujian Provincial Collaborative Innovation Center for Advanced High‐Field Superconducting Materials and Engineering Fujian Normal University Fuzhou Fujian 350117 P. R. China

Fujian Provincial Engineering Technology Research Center of Solar Energy Conversion and Energy Storage Fujian Normal University Fuzhou Fujian 350117 P. R. China

Funding

National Natural Science Foundation of China · Natural Science Foundation of Fujian Province

References (50)

Show source-provided references
1. 10.1038/s41467-020-17390-310.1038/s41467-020-17390-3 ↗
2. 10.1038/s41586-020-2791-x10.1038/s41586-020-2791-x ↗
3. 10.1016/j.nanoen.2022.10700310.1016/j.nanoen.2022.107003 ↗
4. 10.1002/adma.20240614710.1002/adma.202406147 ↗
5. 10.1126/science.110871210.1126/science.1108712 ↗
6. 10.1021/acsenergylett.1c0274510.1021/acsenergylett.1c02745 ↗
7. 10.1002/adfm.20230776110.1002/adfm.202307761 ↗
8. 10.1038/nphoton.2013.20210.1038/nphoton.2013.202 ↗
9. 10.1002/lpor.20180017310.1002/lpor.201800173 ↗
10. 10.1002/adfm.20221055810.1002/adfm.202210558 ↗
11. 10.1038/s41467-022-32607-310.1038/s41467-022-32607-3 ↗
12. 10.1038/s41467-020-16649-z10.1038/s41467-020-16649-z ↗
13. 10.1002/adom.20230096310.1002/adom.202300963 ↗
14. 10.1002/lpor.20210031710.1002/lpor.202100317 ↗
15. 10.1002/adma.20190788810.1002/adma.201907888 ↗
16. 10.1038/s41467-024-45293-010.1038/s41467-024-45293-0 ↗
17. 10.26599/JAC.2023.922071010.26599/JAC.2023.9220710 ↗
18. 10.1002/adfm.20240102610.1002/adfm.202401026 ↗
19. 10.1002/adom.20200214110.1002/adom.202002141 ↗
20. 10.1002/sdtp.1410210.1002/sdtp.14102 ↗
21. 10.1016/j.cej.2022.13459310.1016/j.cej.2022.134593 ↗
22. 10.1002/advs.20200411810.1002/advs.202004118 ↗
23. 10.1016/j.cej.2021.13137910.1016/j.cej.2021.131379 ↗
24. 10.1021/acs.chemmater.7b0460510.1021/acs.chemmater.7b04605 ↗
25. 10.1016/j.mattod.2020.04.03210.1016/j.mattod.2020.04.032 ↗
26. 10.1002/adma.20180248910.1002/adma.201802489 ↗
27. 10.1021/cm200590210.1021/cm2005902 ↗
28. 10.1039/C9TC02107H10.1039/C9TC02107H ↗
29. 10.1002/adom.20180141910.1002/adom.201801419 ↗
30. 10.1002/adom.20230148010.1002/adom.202301480 ↗
31. 10.1039/C9TC05807A10.1039/C9TC05807A ↗
32. 10.1002/lpor.20210004410.1002/lpor.202100044 ↗
33. 10.1039/D2TC04160J10.1039/D2TC04160J ↗
34. 10.1039/D4TC00890A10.1039/D4TC00890A ↗
35. 10.1039/D2TC00850E10.1039/D2TC00850E ↗
36. 10.1002/anie.20180472110.1002/anie.201804721 ↗
37. 10.1039/C9TC00506D10.1039/C9TC00506D ↗
38. 10.1002/adma.20231324710.1002/adma.202313247 ↗
39. 10.1002/adom.20230234310.1002/adom.202302343 ↗
40. 10.1038/s41586-019-1771-510.1038/s41586-019-1771-5 ↗
41. 10.1002/adfm.20231479510.1002/adfm.202314795 ↗
42. 10.1002/adom.20210079910.1002/adom.202100799 ↗
43. 10.1016/j.jlumin.2019.04.06010.1016/j.jlumin.2019.04.060 ↗
44. 10.1039/D4CC01093K10.1039/D4CC01093K ↗
45. 10.1021/cm501055k10.1021/cm501055k ↗
46. 10.26599/JAC.2023.922080910.26599/JAC.2023.9220809 ↗
47. 10.26599/JAC.2024.922086010.26599/JAC.2024.9220860 ↗
48. 10.1103/PhysRevB.54.1116910.1103/PhysRevB.54.11169 ↗
49. 10.1103/PhysRevB.59.175810.1103/PhysRevB.59.1758 ↗
50. 10.1103/PhysRevB.50.1795310.1103/PhysRevB.50.17953 ↗