Liquid‐Based Adaptive Structural Materials

Abstract Structural materials are used to provide stable mechanical architectures and transmit or support forces, and they play an important role in materials science and technology. During the long process of the exploitation of structural materials, the functionality of structural materials has gained prominence. Adaptive structures responding to external stimuli have come to the fore with significant advantages in structural materials. However, many solid adaptive structural materials still suffer from their single function and the lack of dynamic performance, such as issue around fouling and energy consumption, defects present everywhere in materials at the microscale, etc. To meet the increasing demands, more and more researchers have started turning their attention to liquid‐based materials owing to their intrinsic spontaneous, dynamic, and functional properties. Liquid‐based adaptive structural materials (LASMs) have been proposed and developed. Building upon both dynamic liquids and fixed solids, LASMs have been demonstrated to possess both dynamic adaptivity (from the active liquid part) and stable mechanical structure (from the fixed solid part), which are desired in many applications such as 3D printing, droplet manipulation, omniphobic surfaces, microfluidics, mass separation, etc. A unifying view of the recent progress of LASMs is presented, including liquid with particles, liquid with surfaces, as well as liquid with membranes. In addition, the discussion of the prospects and challenges are provided for promoting the development of LASMs.