journal article·2023-04Open access

Coexistence of Merons with Skyrmions in the Centrosymmetric Van Der Waals Ferromagnet Fe5–xGeTe2

Brian W. Casas, Yue Li, Alex Moon, Yan Xin, Conor McKeever, Juan Macy, Amanda K. Petford‐Long, Charudatta M. Phatak, Elton J. G. Santos, Eun Sang Choi, Luis Balicas

Advanced Materials· Volume 35· Issue 17

Abstract

Fe5–xGeTe2 is a centrosymmetric, layered van der Waals (vdW) ferromagnet that displays Curie temperatures Tc (270–330 K) that are within the useful range for spintronic applications. However, little is known about the interplay between its topological spin textures (e.g., merons, skyrmions) with technologically relevant transport properties such as the topological Hall effect (THE) or topological thermal transport. Here, via high‐resolution Lorentz transmission electron microscopy, it is shown that merons and anti‐meron pairs coexist with Néel skyrmions in Fe5–xGeTe2 over a wide range of temperatures and probe their effects on thermal and electrical transport. A THE is detected, even at room T, that senses merons at higher T's, as well as their coexistence with skyrmions as T is lowered, indicating an on‐demand thermally driven formation of either type of spin texture. Remarkably, an unconventional THE is also observed in absence of Lorentz force, and it is attributed to the interaction between charge carriers and magnetic field‐induced chiral spin textures. These results expose Fe5–xGeTe2 as a promising candidate for the development of applications in skyrmionics/meronics due to the interplay between distinct but coexisting topological magnetic textures and unconventional transport of charge/heat carriers.
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Research context

OpenAlex topics: Graphene research and applications · 2D Materials and Applications · Topological Materials and Phenomena

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

National High Magnetic Field Laboratory Tallahassee FL 32310 USA

Materials Science Division Argonne National Laboratory Lemont IL 60439 USA

Department of Physics Florida State University Tallahassee FL 32306 USA

Institute for Condensed Matter and Complex Systems School of Physics and Astronomy The University of Edinburgh Edinburgh EH9 3FD UK

Department of Materials Science and Engineering Northwestern University Evanston IL 60208 USA

Higgs Centre for Theoretical Physics The University of Edinburgh Edinburgh EH9 3FD UK

Donostia International Physics Center (DIPC) 20018 Donostia‐San Sebastián Basque Country Spain

Funding

Basic Energy Sciences · U.S. Department of Energy

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