Bionic Artificial Skin Based on Self‐Healable Ionogel Composites with Tailored Mechanics and Robust Interfaces

Abstract Bionic artificial skin which imitates the features and functions of human skin, has broad applications in wearable human‐machine interfaces. However, equipping artificial materials with skin‐like mechanical properties, self‐healing ability, and high sensitivity remains challenging. Here, inspired by the structure of human skin, an artificial skin based on ionogel composites with tailored mechanical properties and robust interface is prepared. Combining finite element analysis and direct ink writing (DIW) 3D printing technology, an ionogel composite with a rigid skeleton and an ionogel matrix is precisely designed and fabricated, realizing the mechanical anisotropy and nonlinear mechanical response that accurately mimic human skin. Robust interface is created through co‐curing of the skeleton and matrix resins, significantly enhancing the stability of the composite. The realization of self‐healing ability and resistance to crack growth further ensure the remarkable durability of the artificial skin for sensing application. In summary, the bionic artificial skin mimics the characteristics of human skin, including mechanical anisotropy, nonlinear mechanical response, self‐healing capability, durability and high sensitivity when applied as flexible sensors. These strategies provide strong support for the fabrication of tissue‐like materials with adaptive mechanical behaviors.