journal article·2024-08Open access

Liquid Crystal Elastomer Lattices with Thermally Programmable Deformation via Multi‐Material 3D Printing

Arda Kotikian, Audrey A. Watkins, Giovanni Bordiga, Andrew Spielberg, Zoey S. Davidson, Katia Bertoldi, Jennifer A. Lewis

Advanced Materials· Volume 36· Issue 34

Abstract

Abstract An integrated design, modeling, and multi‐material 3D printing platform for fabricating liquid crystal elastomer (LCE) lattices in both homogeneous and heterogeneous layouts with spatially programmable nematic director order and local composition is reported. Depending on their compositional topology, these lattices exhibit different reversible shape‐morphing transformations upon cycling above and below their respective nematic‐to‐isotropic transition temperatures. Further, it is shown that there is good agreement between their experimentally observed deformation response and model predictions for all LCE lattice designs evaluated. Lastly, an inverse design model is established and the ability to print LCE lattices with the predicted deformation behavior is demonstrated. This work opens new avenues for creating architected LCE lattices that may find potential application in energy‐dissipating structures, microfluidic pumping, mechanical logic, and soft robotics.
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Research context

OpenAlex topics: Advanced Materials and Mechanics · Advanced Sensor and Energy Harvesting Materials · Structural Analysis and Optimization

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

John A. Paulson School of Engineering and Applied Sciences Harvard University Cambridge MA 02138 USA

Wyss Institute for Biologically Inspired Engineering Harvard University Cambridge MA 02138 USA

Funding

National Science Foundation · Defense Advanced Research Projects Agency

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