journal article·2023-08

Programmable Wavefront Control in the Visible Spectrum Using Low‐Loss Chalcogenide Phase‐Change Metasurfaces

Parikshit Moitra, Yunzheng Wang, Xinan Liang, Li Lu, Alyssa Poh, Tobias W.W. Mass, Robert E. Simpson, Arseniy I. Kuznetsov, Ramon Paniagua‐Dominguez

Advanced Materials· Volume 35· Issue 34
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Abstract

Abstract All‐dielectric metasurfaces provide unique solutions for advanced wavefront manipulation of light with complete control of amplitude and phase at sub‐wavelength scales. One limitation, however, for most of these devices is the lack of any post‐fabrication tunability of their response. To break this limit, a promising approach is employing phase‐change materials (PCMs), which provide fast, low energy, and non‐volatile means to endow metasurfaces with a switching mechanism. In this regard, great advancements have been done in the mid‐infrared and near‐infrared spectrum using different chalcogenides. In the visible spectral range, however, very few devices have demonstrated full phase manipulation, high efficiencies, and reversible optical modulation. In this work, a programmable all‐dielectric Huygens’ metasurface made of antimony sulfide (Sb2S3) PCM is experimentally demonstrated, a low loss and high‐index material in the visible spectral range with a large contrast (≈0.5) between its amorphous and crystalline states. ≈2π phase modulation is shown with high associated transmittance and it is used to create programmable beam‐steering devices. These novel chalcogenide PCM metasurfaces have the potential to emerge as a platform for next‐generation spatial light modulators and to impact application areas such as programmable and adaptive flat optics, light detection and ranging (LiDAR), and many more.
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Research context

OpenAlex topics: Metamaterials and Metasurfaces Applications · Advanced Optical Imaging Technologies · Liquid Crystal Research Advancements

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Institute of Materials Research and Engineering A*STAR (Agency for Science Technology and Research) Singapore 138634 Singapore

Singapore University of Technology and Design Singapore 487372 Singapore

Optics Research and Engineering Shandong University Qingdao 266237 P. R. China

Funding

National Research Foundation Singapore

References (65)

Show source-provided references
1. 10.1126/science.aag247210.1126/science.aag2472 ↗
2. 10.1021/acs.nanolett.8b0036810.1021/acs.nanolett.8b00368 ↗
3. 10.1002/adom.20140058410.1002/adom.201400584 ↗
4. 10.1021/nl404448210.1021/nl4044482 ↗
5. 10.1126/science.125321310.1126/science.1253213 ↗
6. 10.1002/lpor.20150004110.1002/lpor.201500041 ↗
7. 10.1103/PhysRevLett.102.13390110.1103/PhysRevLett.102.133901 ↗
8. 10.1103/PhysRevLett.98.15740310.1103/PhysRevLett.98.157403 ↗
9. 10.1103/PhysRevB.80.19511910.1103/PhysRevB.80.195119 ↗
10. 10.1021/acsphotonics.5b0014810.1021/acsphotonics.5b00148 ↗
11. 10.1021/acs.nanolett.5b0292610.1021/acs.nanolett.5b02926 ↗
12. 10.1038/nmat383910.1038/nmat3839 ↗
13. 10.1126/science.121071310.1126/science.1210713 ↗
14. 10.1038/nnano.2015.210.1038/nnano.2015.2 ↗
15. 10.1126/science.aaf664410.1126/science.aaf6644 ↗
16. 10.1109/JPROC.2019.294318310.1109/JPROC.2019.2943183 ↗
17. 10.1126/science.aaw674710.1126/science.aaw6747 ↗
18. 10.1126/science.aat310010.1126/science.aat3100 ↗
19. 10.1021/acsphotonics.7b0134310.1021/acsphotonics.7b01343 ↗
20. 10.1021/acs.nanolett.8b0047510.1021/acs.nanolett.8b00475 ↗
21. 10.1021/acsphotonics.1c0037110.1021/acsphotonics.1c00371 ↗
22. 10.1021/acs.nanolett.1c0010410.1021/acs.nanolett.1c00104 ↗
23. 10.1038/s41377-022-00832-610.1038/s41377-022-00832-6 ↗
24. A. V.Baranikov S.Li D.Eschimese X.Xu S.Thiele S.Ristok R. M.Veetil T. W. W.Mass P.Moitra H.Giessen R.Paniagua‐Domínguez A. I.Kuznetsov arXiv: 2107.11096 v1 2021.
25. 10.1021/acsphotonics.0c0159910.1021/acsphotonics.0c01599 ↗
26. 10.1002/adom.20210189310.1002/adom.202101893 ↗
27. 10.1021/acsnano.0c0126910.1021/acsnano.0c01269 ↗
28. 10.1021/acs.nanolett.6b0055510.1021/acs.nanolett.6b00555 ↗
29. 10.1038/s41565-020-00787-y10.1038/s41565-020-00787-y ↗
30. 10.1038/srep1575410.1038/srep15754 ↗
31. 10.1021/ph500327910.1021/ph5003279 ↗
32. 10.1038/s41566-020-0624-y10.1038/s41566-020-0624-y ↗
33. 10.1021/nl403253c10.1021/nl403253c ↗
34. 10.1021/acs.nanolett.7b0035910.1021/acs.nanolett.7b00359 ↗
35. 10.1021/nl503104n10.1021/nl503104n ↗
36. 10.1038/s41467-017-00019-310.1038/s41467-017-00019-3 ↗
37. 10.1021/acs.nanolett.7b0152910.1021/acs.nanolett.7b01529 ↗
38. 10.1021/acs.nanolett.5b0253410.1021/acs.nanolett.5b02534 ↗
39. 10.1021/acs.nanolett.9b0124610.1021/acs.nanolett.9b01246 ↗
40. 10.1038/s41467-022-29374-610.1038/s41467-022-29374-6 ↗
41. 10.1038/nphoton.2015.24710.1038/nphoton.2015.247 ↗
42. 10.1038/s41565-021-00881-910.1038/s41565-021-00881-9 ↗
43. 10.1002/adma.20150202310.1002/adma.201502023 ↗
44. 10.1063/1.495927210.1063/1.4959272 ↗
45. 10.1364/OPTICA.38413810.1364/OPTICA.384138 ↗
46. 10.1002/adom.20180178210.1002/adom.201801782 ↗
47. 10.1002/adfm.20170499310.1002/adfm.201704993 ↗
48. 10.1002/adom.20190017110.1002/adom.201900171 ↗
49. 10.1002/adma.20150623810.1002/adma.201506238 ↗
50. 10.1038/s41524-021-00655-w10.1038/s41524-021-00655-w ↗
51. 10.1126/science.122156110.1126/science.1221561 ↗
52. 10.1038/nphoton.2017.12610.1038/nphoton.2017.126 ↗
53. 10.1515/nanoph-2020-003910.1515/nanoph-2020-0039 ↗
54. 10.1002/adpr.20200020510.1002/adpr.202000205 ↗
55. 10.1038/s41467-019-12196-410.1038/s41467-019-12196-4 ↗
56. 10.1002/adfm.20180618110.1002/adfm.201806181 ↗
57. 10.1021/acsnano.1c0711410.1021/acsnano.1c07114 ↗
58. 10.1002/adom.20200204910.1002/adom.202002049 ↗
59. O.Hemmatyar S.Abdollahramezani I.Zeimpekis S.Lepeshov A. I.Khan K. M.Neilson C.Teichrib T.Brown D. W.Hewak M.Wuttig A.Al O. L.Muskens A.Adibi arXiv: 2107.12159 v1 2021.
60. 10.1002/adfm.20210332710.1002/adfm.202103327 ↗
61. 10.1002/adfm.20200244710.1002/adfm.202002447 ↗
62. 10.1364/OL.42.00263910.1364/OL.42.002639 ↗
63. 10.1002/adfm.20190685110.1002/adfm.201906851 ↗
64. 10.1126/sciadv.abb717110.1126/sciadv.abb7171 ↗
65. 10.1364/AO.44472810.1364/AO.444728 ↗