journal article·2017-03Open access

Nanocomposites from Solution‐Synthesized PbTe‐BiSbTe Nanoheterostructure with Unity Figure of Merit at Low‐Medium Temperatures (500–600 K)

Biao Xu, Matthias T. Agne, Tianli Feng, Thomas C. Chasapis, Xiulin Ruan, Yilong Zhou, Haimei Zheng, Je‐Hyeong Bahk, Mercouri G. Kanatzidis, Gerald Jeffrey Snyder, Yue Wu

Advanced Materials· Volume 29· Issue 10

Abstract

A scalable, low-temperature solution process is used to synthesize precursor material for Pb-doped Bi0.7Sb1.3Te3 thermoelectric nanocomposites. The controllable Pb-doping leads to the increase in the optical bandgap, thus delaying the onset of bipolar conduction. Furthermore, the solution synthesis enables nanostructuring, which greatly reduces thermal conductivity. As a result, this material exhibits a zT = 1 over the 513–613 K range. As a service to our authors and readers, this journal provides supporting information supplied by the authors. Such materials are peer reviewed and may be re-organized for online delivery, but are not copy-edited or typeset. Technical support issues arising from supporting information (other than missing files) should be addressed to the authors. Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article.
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Research context

OpenAlex topics: Advanced Thermoelectric Materials and Devices · Thermal properties of materials · Thermal Radiation and Cooling Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Chemical and Biological Engineering Iowa State University Ames IA 50011 USA

Department of Materials Science and Engineering Northwestern University Evanston IL 60208 USA

School of Mechanical Engineering Purdue University West Lafayette IN 47907 USA

Materials Sciences Division Lawrence Berkeley National Laboratory Building 62 Room 211, 1 Cyclotron Road Berkeley CA 94720 USA

Department of Mechanical and Materials Engineering University of Cincinnati Cincinnati OH 45221 USA

Department of Chemistry Northwestern University Evanston IL 60208 USA

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