journal article·2021-08

Metal–Nitrogen–Carbon Catalysts of Specifically Coordinated Configurations toward Typical Electrochemical Redox Reactions

Yongxia Wang, Xiangzhi Cui, Luwei Peng, Lulu Li, Jinli Qiao, Haitao Huang, Jianlin Shi

Advanced Materials· Volume 33· Issue 34
Publisher page

Abstract

Abstract Metal–nitrogen–carbon (M–N–C) material with specifically coordinated configurations is a promising alternative to costly Pt‐based catalysts. In the past few years, great progress is made in the studies of M–N–C materials, including the structure modulation and local coordination environment identification via advanced synthetic strategies and characterization techniques, which boost the electrocatalytic performances and deepen the understanding of the underlying fundamentals. In this review, the most recent advances of M–N–C catalysts with specifically coordinated configurations of M–Nx (x = 1–6) are summarized as comprehensively as possible, with an emphasis on the synthetic strategy, characterization techniques, and applications in typical electrocatalytic reactions of the oxygen reduction reaction, oxygen evolution reaction, hydrogen evolution reaction, CO2 reduction reaction, etc., along with mechanistic exploration by experiments and theoretical calculations. Furthermore, the challenges and potential perspectives for the future development of M–N–C catalysts are discussed.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Electrocatalysts for Energy Conversion · Fuel Cells and Related Materials · Catalytic Processes in Materials Science

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Environmental Science and Engineering Donghua University 2999 Ren'min North Road Shanghai 201620 China

State Key Lab of High Performance Ceramics and Superfine Microstructure Shanghai Institute of Ceramics Chinese Academy of Sciences 1295 Dingxi Road Shanghai 200050 China

School of Chemistry and Materials Science Hangzhou Institute for Advanced Study University of Chinese Academy of Sciences Hangzhou 310024 P. R. China

Shanghai Institute of Pollution Control and Ecological Security 1515 North Zhongshan Road Shanghai 200092 China

Department of Applied Physics Hong Kong Polytechnic University 11 Yucai road Kowloon Hong Kong 999077 China

Funding

National Natural Science Foundation of China · Science and Technology Commission of Shanghai Municipality

References (100+)

Show source-provided references
1. 10.1002/celc.20190099610.1002/celc.201900996 ↗
2. 10.1002/aenm.20180095510.1002/aenm.201800955 ↗
3. 10.1007/s10853-018-2245-010.1007/s10853-018-2245-0 ↗
4. 10.1039/C7TA10555J10.1039/C7TA10555J ↗
5. 10.1016/j.jelechem.2018.01.01310.1016/j.jelechem.2018.01.013 ↗
6. 10.1680/jsuin.20.0002810.1680/jsuin.20.00028 ↗
7. 10.1016/j.jpowsour.2016.06.09810.1016/j.jpowsour.2016.06.098 ↗
8. 10.1039/C9TA09104A10.1039/C9TA09104A ↗
9. 10.1149/2.0171816jes10.1149/2.0171816jes ↗
10. 10.1039/C9RA01330J10.1039/C9RA01330J ↗
11. 10.1021/acsami.7b1444310.1021/acsami.7b14443 ↗
12. 10.1039/C6TA10496G10.1039/C6TA10496G ↗
13. 10.1016/j.jechem.2018.09.01910.1016/j.jechem.2018.09.019 ↗
14. 10.1016/j.jpowsour.2018.08.07410.1016/j.jpowsour.2018.08.074 ↗
15. 10.1039/C6CC06608A10.1039/C6CC06608A ↗
16. 10.1016/j.apsusc.2019.14438010.1016/j.apsusc.2019.144380 ↗
17. 10.1016/j.electacta.2020.13606610.1016/j.electacta.2020.136066 ↗
18. 10.1088/2053-1591/ab33ad10.1088/2053-1591/ab33ad ↗
19. 10.1021/acs.jpca.0c0244910.1021/acs.jpca.0c02449 ↗
20. 10.1002/celc.20200013710.1002/celc.202000137 ↗
21. 10.1007/BF0103938510.1007/BF01039385 ↗
22. 10.1039/C7NR02165H10.1039/C7NR02165H ↗
23. 10.1016/0013-4686(86)80022-610.1016/0013-4686(86)80022-6 ↗
24. 10.1038/2011212a010.1038/2011212a0 ↗
25. 10.1021/acsami.5b0583410.1021/acsami.5b05834 ↗
26. 10.1016/j.jechem.2018.06.00810.1016/j.jechem.2018.06.008 ↗
27. 10.1016/j.electacta.2018.11.20010.1016/j.electacta.2018.11.200 ↗
28. 10.1002/cssc.20170086410.1002/cssc.201700864 ↗
29. 10.1007/s12274-017-1615-210.1007/s12274-017-1615-2 ↗
30. 10.1007/s10751-017-1485-810.1007/s10751-017-1485-8 ↗
31. 10.3390/nano905074210.3390/nano9050742 ↗
32. 10.1002/smll.20170428210.1002/smll.201704282 ↗
33. 10.1016/S0013-4686(98)00382-X10.1016/S0013-4686(98)00382-X ↗
34. 10.1007/s12274-020-2768-y10.1007/s12274-020-2768-y ↗
35. 10.1039/c1cp21228a10.1039/c1cp21228a ↗
36. 10.1007/s00894-019-4071-y10.1007/s00894-019-4071-y ↗
37. 10.1149/2.0371907jes10.1149/2.0371907jes ↗
38. 10.1016/j.ensm.2016.11.00110.1016/j.ensm.2016.11.001 ↗
39. 10.1039/c2gc35309a10.1039/c2gc35309a ↗
40. 10.1002/smll.20190381610.1002/smll.201903816 ↗
41. 10.1016/j.apcatb.2019.02.02410.1016/j.apcatb.2019.02.024 ↗
42. 10.1016/j.apsusc.2019.14365910.1016/j.apsusc.2019.143659 ↗
43. 10.1038/s41929-018-0063-z10.1038/s41929-018-0063-z ↗
44. 10.1016/j.carbon.2017.12.12110.1016/j.carbon.2017.12.121 ↗
45. 10.1039/C9CY01935A10.1039/C9CY01935A ↗
46. 10.1016/j.apsusc.2020.14658810.1016/j.apsusc.2020.146588 ↗
47. 10.1088/1361-6528/ab97d510.1088/1361-6528/ab97d5 ↗
48. 10.1016/j.carbon.2020.05.02410.1016/j.carbon.2020.05.024 ↗
49. 10.1002/chem.20180571610.1002/chem.201805716 ↗
50. 10.1038/am.2017.21210.1038/am.2017.212 ↗
51. 10.1016/j.electacta.2018.11.10510.1016/j.electacta.2018.11.105 ↗
52. 10.1016/j.jechem.2019.12.00510.1016/j.jechem.2019.12.005 ↗
53. 10.1016/j.jallcom.2020.15455810.1016/j.jallcom.2020.154558 ↗
54. 10.1021/acsami.8b2000310.1021/acsami.8b20003 ↗
55. 10.1134/S102319352004007210.1134/S1023193520040072 ↗
56. 10.1016/j.jcat.2017.02.02810.1016/j.jcat.2017.02.028 ↗
57. 10.1016/j.matpr.2018.10.07710.1016/j.matpr.2018.10.077 ↗
58. 10.1021/jp030349j10.1021/jp030349j ↗
59. 10.1016/0013-4686(82)80036-410.1016/0013-4686(82)80036-4 ↗
60. 10.1016/S0022-0728(98)00390-810.1016/S0022-0728(98)00390-8 ↗
61. 10.1023/A:100328860941110.1023/A:1003288609411 ↗
62. 10.1016/S0013-4686(98)80010-810.1016/S0013-4686(98)80010-8 ↗
63. 10.1016/j.electacta.2007.11.00210.1016/j.electacta.2007.11.002 ↗
64. 10.1039/c4cp01634c10.1039/c4cp01634c ↗
65. 10.1016/j.jpowsour.2014.01.00810.1016/j.jpowsour.2014.01.008 ↗
66. 10.1021/jp026608710.1021/jp0266087 ↗
67. 10.1038/nmat436710.1038/nmat4367 ↗
68. 10.1021/jp802456e10.1021/jp802456e ↗
69. 10.1021/jp057135h10.1021/jp057135h ↗
70. 10.1002/anie.20171245110.1002/anie.201712451 ↗
71. 10.1016/j.ijhydene.2018.09.04310.1016/j.ijhydene.2018.09.043 ↗
72. 10.1007/s12274-016-1400-710.1007/s12274-016-1400-7 ↗
73. 10.1021/acscatal.7b0271810.1021/acscatal.7b02718 ↗
74. 10.1016/j.coelec.2018.03.03910.1016/j.coelec.2018.03.039 ↗
75. 10.1007/s41918-019-00031-910.1007/s41918-019-00031-9 ↗
76. 10.1007/s11426-018-9425-510.1007/s11426-018-9425-5 ↗
77. 10.1002/adma.20180654510.1002/adma.201806545 ↗
78. 10.1002/celc.20180130210.1002/celc.201801302 ↗
79. 10.1002/cctc.20180167910.1002/cctc.201801679 ↗
80. 10.1002/smtd.20200001610.1002/smtd.202000016 ↗
81. 10.1007/s12274-020-2755-310.1007/s12274-020-2755-3 ↗
82. 10.1002/anie.20191030910.1002/anie.201910309 ↗
83. 10.1016/j.coelec.2020.08.00610.1016/j.coelec.2020.08.006 ↗
84. 10.1002/smll.20200290210.1002/smll.202002902 ↗
85. 10.1002/adma.20180484610.1002/adma.201804846 ↗
86. 10.1007/s41918-019-00030-w10.1007/s41918-019-00030-w ↗
87. 10.1021/acssuschemeng.7b0284110.1021/acssuschemeng.7b02841 ↗
88. 10.1002/adma.20180266910.1002/adma.201802669 ↗
89. 10.1002/celc.20190116710.1002/celc.201901167 ↗
90. 10.1039/C9TA08532G10.1039/C9TA08532G ↗
91. 10.1021/jp076443810.1021/jp0764438 ↗
92. 10.1002/smll.20170281710.1002/smll.201702817 ↗
93. 10.1002/asia.20190161610.1002/asia.201901616 ↗
94. 10.1039/C6RA16539G10.1039/C6RA16539G ↗
95. 10.1016/j.carbon.2018.06.00710.1016/j.carbon.2018.06.007 ↗
96. 10.1039/C8NR01457D10.1039/C8NR01457D ↗
97. 10.1016/j.carbon.2020.02.05910.1016/j.carbon.2020.02.059 ↗
98. 10.1039/B713096A10.1039/B713096A ↗
99. 10.1126/science.117005110.1126/science.1170051 ↗
100. 10.1002/advs.20200154510.1002/advs.202001545 ↗