journal article·2022-01Open access

Thermal Properties of Nanocrystalline Silicon Nanobeams

Jeremie Maire, Emigdio Chávez‐Ángel, Guillermo Arregui, Martin F. Colombano, Nestor E. Capuj, Amadeu Griol, Alejandro Martínez, Daniel Navarro‐Urrios, Jouni Ahopelto, Clivia M. Sotomayor‐Torres

Advanced Functional Materials· Volume 32· Issue 4

Abstract

Abstract Controlling thermal energy transfer at the nanoscale and thermal properties has become critically important in many applications since it often limits device performance. In this study, the effects on thermal conductivity arising from the nanoscale structure of free‐standing nanocrystalline silicon films and the increasing surface‐to‐volume ratio when fabricated into suspended optomechanical nanobeams are studied. Thermal transport and elucidate the relative impact of different grain size distributions and geometrical dimensions on thermal conductivity are characterized. A micro time‐domain thermoreflectance method to study free‐standing nanocrystalline silicon films and find a drastic reduction in the thermal conductivity, down to values below 10 W m–1 K–1 is used, with a stronger decrease for smaller grains. In optomechanical nanostructures, this effect is smaller than in membranes due to the competition of surface scattering in decreasing thermal conductivity. Finally, a novel versatile contactless characterization technique that can be adapted to any structure supporting a thermally shifted optical resonance is introduced. The thermal conductivity data agrees quantitatively with the thermoreflectance measurements. This study opens the way to a more generalized thermal characterization of optomechanical cavities and to create hot‐spots with engineered shapes at the desired position in the structures as a means to study thermal transport in coupled photon‐phonon structures.
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Research context

OpenAlex topics: Thermal properties of materials · Mechanical and Optical Resonators · Thermal Radiation and Cooling Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Catalan Institute of Nanoscience and Nanotechnology (ICN2) CSIC and BIST Campus UAB Bellaterra Barcelona 08193 Spain

Institut de Mécanique et d'ingénierie (I2M) UMR5295, CNRS‐UB‐ENSAM Talence 33405 France

Depto. Física Universidad Autónoma de Barcelona Bellaterra Barcelona 08193 Spain

Depto. Física Universidad de La Laguna San Cristóbal de La Laguna 38200 Spain

Instituto Universitario de Materiales y Nanotecnología Universidad de La Laguna Santa Cruz de Tenerife 38071 Spain

Nanophotonics Technology Center Universitat Politècnica de València València 46022 Spain

MIND‐IN2UB Departament d'Enginyeria Electrònica i Biomèdica, Facultat de Física Universitat de Barcelona Martí i Franquès 1 Barcelona 08028 Spain

Microelectronics and Quantum Technology VTT Technical Research Centre of Finland Ltd P.O. Box 1000 Espoo FI‐02044 VTT Finland

Catalan Institute for Research and Advances Studies ICREA Barcelona 08010 Spain

Funding

European Commission · Generalitat de Catalunya · Ministerio de Ciencia, Innovación y Universidades · Generalitat Valenciana · Agencia Estatal de Investigación · H2020 Future and Emerging Technologies

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