journal article·2023-07Open access

Nanoscale Management of CO Transport in CO2 Electroreduction: Boosting Faradaic Efficiency to Multicarbon Products via Nanostructured Tandem Electrocatalysts (Adv. Funct. Mater. 28/2023)

Chaolong Wei, Yuehua Yang, Haibin Ma, Guangxin Sun, Xin Wang, Yaqi Cheng, Caiwei Zhang, Boon Siang Yeo, Chunnian He, Andrew Barnabas Wong

Advanced Functional Materials· Volume 33· Issue 28

Abstract

Tandem Catalysis In article number 2214992, Andrew Barnabas Wong, Chunnian He, and co-workers illustrate a design principle to improve the performance of tandem electrocatalysts for converting CO2 to C2+ products (ethylene and ethanol) by managing diffusion of the key intermediate, CO, within a 3D model system. This model system consists of Ag nanoparticles within a Cu nanoneedle array to restrict CO diffusion away from Cu active sites, which boosts C-C coupling towards C2+ products.
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Research context

OpenAlex topics: CO2 Reduction Techniques and Catalysts · Catalytic Processes in Materials Science · Electrocatalysts for Energy Conversion

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Affiliations

Joint School of National University of Singapore and Tianjin University International Campus of Tianjin University Binhai New City Fuzhou 350207 P. R. China

Department of Materials Science and Engineering National University of Singapore Singapore 117574 Singapore

CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Modern Mechanics University of Science and Technology of China Hefei Anhui 230026 P. R. China

Department of Chemistry National University of Singapore 3 Science Drive 3 Singapore 117543 Singapore

Department of Chemical and Biomolecular Engineering National University of Singapore Singapore 117585 Singapore

School of Materials Science and Engineering Tianjin Key Laboratory of Composite and Functional Materials Tianjin University Tianjin 300350 P. R. China

References

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