journal article·2020-05-08

Molecular Catalysts Boost the Rate of Electrolytic CO2 Reduction

Kristian Torbensen, Dorian Joulié, Shaoxuan Ren, Min Wang, Danielle Salvatore, Curtis P. Berlinguette, Marc Robert

ACS Energy Letters· Volume 5· Issue 5
Publisher page

Abstract

Electrolysis is a potentially useful approach for converting carbon dioxide into chemicals and fuels. The most active electrocatalysts for efficiently mediating the carbon dioxide reduction reaction (CO2RR) have long been assumed to be solid silver, gold, and copper. However, there is an emerging body of data showing that molecular catalysts can operate at levels of performance commensurate with solid-state catalysts. These recent advances in deploying molecular catalysts present entirely new opportunities for understanding CO2RR in electrochemical reactors and tailoring active sites for the selective formation of CO2RR products. This Perspective highlights the recent advances and the opportunities for the implementation of molecular electrocatalysts into CO2RR electrolyzers.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: CO2 Reduction Techniques and Catalysts · Carbon dioxide utilization in catalysis · Ionic liquids properties and applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Université de Paris, Laboratoire d’Electrochimie Moléculaire, CNRS, F-75013 Paris, France

Department of Chemistry, University of British Columbia, Vancouver, British Columbia V6T 1Z1, Canada

Department of Chemical and Biological Engineering, The University of British Columbia, Vancouver, British Columbia V6T 1Z3, Canada

Stewart Blusson Quantum Matter Institute, The University of British Columbia, Vancouver, British Columbia V6T 1Z4, Canada

Canadian Institute for Advanced Research (CIFAR), Toronto, Ontario M5G 1M1, Canada

Institut Universitaire de France (IUF), F-75005 Paris, France

Funding

Air Liquide · China Scholarship Council · Institut Universitaire de France

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