journal article·2024-12Open access

Enhanced Direct Air Carbon Capture on NaX Zeolite by Electric‐Field Enhanced Physical Adsorption and In Situ CO2 Synergistic Effects of Cold Plasma

Minghai Shen, Fulin Kong, Wei Guo, Zhongqi Zuo, Chan Guo, Lige Tong, Shaowu Yin, Li Wang, Sibudjing Kawi, Paul K. Chu, Yulong Ding

Advanced Functional Materials· Volume 34· Issue 49

Abstract

Abstract Direct air carbon capture (DAC) is vital to achieving negative CO2 emissions, with physical adsorption offering a cost‐effective and energy‐efficient solution. an advanced zeolite modification technique is presented using cold plasma, which enhances the CO2 adsorption efficiency of NaX zeolite by 11.5% after just 60 min. This method utilizes the electric field to reorganize cation distribution and pore structure and significantly improve the adsorption capacity, efficiency, and selectivity. Compared to traditional methods, this technique is simpler and more effective, as demonstrated through first‐principles calculations, thermodynamics, kinetics, and adsorption equilibrium studies.
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Research context

OpenAlex topics: Catalytic Processes in Materials Science · Membrane Separation and Gas Transport · Carbon Dioxide Capture Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Beijing Key Laboratory of Energy Saving and Emission Reduction for Metallurgical Industry School of Energy and Environmental Engineering University of Science and Technology Beijing Beijing 100083 China

Department of Chemical and Biomolecular Engineering National University of Singapore Singapore 119260 Singapore

101 Research Institute of the Ministry of Civil Affairs Beijing 100070 China

Department of Physics Department of Materials Science and Engineering, and Department of Biomedical Engineering City University of Hong Kong Kowloon Hong Kong 999077 China

Birmingham Centre for Energy Storage & School of Chemical Engineering University of Birmingham Birmingham B15 2TT UK

Funding

National Key Research and Development Program of China · China Scholarship Council · Natural Science Foundation of Beijing Municipality

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