Nanoparticle‐Based Strain Gauges: Anisotropic Response Characteristics, Multidirectional Strain Sensing, and Novel Approaches to Healthcare Applications

Abstract Directional strain sensing is essential for advanced sensor applications in the field of human‐machine interfaces and healthcare. Here, the angle dependent anisotropic strain sensitivity caused by charge carriers percolating through cross‐linked gold nanoparticle (GNP) networks is studied and these versatile materials are used for the fabrication of wearable triaxial pulse and gesture sensors. More specifically, the anisotropic response of 1,9‐nonanedithiol cross‐linked GNP films is separated into geometric and piezoresistive contributions by fitting the measured data with an analytic model. Hereby, piezoresistive coefficients of g₁₁ ∼ 32 and g₁₂ ∼ 21 are extracted, indicating a slightly anisotropic response behavior of the GNP‐based material. To use the material for healthcare applications, arrangements of three GNP transducers are patterned lithographically and fully embedded into a highly flexible silicone polymer (Dragon Skin 30). The new encapsulation method ensures good and robust electrical contacts and enables facile handling and protection from external influences. A facile read‐out with wireless data transmission using off‐the‐shelf electrical components underlines the great potential of these devices for applications as skin‐wearable healthcare sensors.