journal article·2025-01Open access

Dimensional Self‐Assembled Magnetic Coupling via Embedding Ferromagnetic Nanoparticles in Multi‐Channel Fibers for Microwave Absorption

Xiangyu Wang, Xiaowei Lv, Ruixuan Zhang, XiaoFen Yang, Rong Dai, Wenbin You, Yuxiang Lai, Renchao Che

Advanced Functional Materials· Volume 35· Issue 3

Abstract

Abstract 1D magnetic fibers with significant morphological diversity and magnetic anisotropy are highly desirable for optimizing magnetic properties and electromagnetic responsiveness. However, it remains challenging for the precise control over internal magnetic interactions within each fiber. Herein, a strategy for self‐assembled magnetic coupling is taken to achieve the controllable reconstruction of continuous multiple coupling networks within a single fiber. High‐density ultrafine cobalt nanoparticles are uniformly embedded inside a carbon framework with a 1D multi‐channel structure (Co@MCF). This structure establishes a complex magnetic response system characterized by inherent inter‐fiber interactions and refined intra‐fiber self‐assembling coupling. The distinctive distribution of magnetic flux lines demonstrates enhanced magnetic sensitivity. This results in a minimum reflection loss of −57.65 dB and a broadband absorption frequency range of 7.28 GHz at 1.9 mm, effectively covers the entire Ku band and a substantial portion of the X band. The multi‐channel structure enhances the understanding of the relationship between microstructure and performance in magnetic fibers. Additionally, it positions Co@MCF as a highly competitive candidate for microwave absorption applications.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Electromagnetic wave absorption materials · Metamaterials and Metasurfaces Applications · Advanced Antenna and Metasurface Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative Materials Academy for Engineering & Technology Advanced Coatings Research Center of Ministry of Education of China Fudan University Shanghai 200438 China

Department of Physics Materials Genome Institute Shanghai Key Laboratory of High Temperature Superconductors International Centre of Quantum and Molecular Structures Shanghai University Shanghai 200444 China

Pico Electron Microscopy Center Innovation Institute for Ocean Materials Characterization Center for Advanced Studies in Precision Instruments Hainan University Haikou 570228 China

School of Materials Science & Engineering Tongji University Shanghai 201804 China

College of Physics Donghua University Shanghai 201620 China

Funding

National Natural Science Foundation of China

References (59)

Show source-provided references
1. 10.1002/adma.20140578810.1002/adma.201405788 ↗
2. 10.1002/adma.20231341110.1002/adma.202313411 ↗
3. 10.1021/acsnano.3c0217010.1021/acsnano.3c02170 ↗
4. 10.1002/adfm.20180739810.1002/adfm.201807398 ↗
5. 10.1002/adfm.20231672210.1002/adfm.202316722 ↗
6. 10.1002/adfm.20230037410.1002/adfm.202300374 ↗
7. 10.1007/s40820-021-00727-y10.1007/s40820-021-00727-y ↗
8. 10.1002/smll.20220632310.1002/smll.202206323 ↗
9. 10.1002/adfm.20180076110.1002/adfm.201800761 ↗
10. 10.1016/j.cej.2021.13130810.1016/j.cej.2021.131308 ↗
11. 10.1016/j.scib.2020.01.00910.1016/j.scib.2020.01.009 ↗
12. 10.1021/acsami.0c1183910.1021/acsami.0c11839 ↗
13. 10.1016/j.carbon.2019.06.04810.1016/j.carbon.2019.06.048 ↗
14. 10.1002/adfm.20180762410.1002/adfm.201807624 ↗
15. 10.1016/j.cej.2020.12431710.1016/j.cej.2020.124317 ↗
16. 10.1007/s12274-022-4401-810.1007/s12274-022-4401-8 ↗
17. 10.1016/j.cej.2019.12239310.1016/j.cej.2019.122393 ↗
18. 10.1016/j.carbon.2023.11835310.1016/j.carbon.2023.118353 ↗
19. 10.1016/j.cej.2021.13287810.1016/j.cej.2021.132878 ↗
20. 10.1016/j.carbon.2021.02.09210.1016/j.carbon.2021.02.092 ↗
21. 10.1016/j.carbon.2020.01.07310.1016/j.carbon.2020.01.073 ↗
22. 10.1002/sstr.20230015210.1002/sstr.202300152 ↗
23. Toulemon D. · Adv. Mater. · 2016 · 26 · 2454
24. 10.1021/acsnano.7b0176210.1021/acsnano.7b01762 ↗
25. 10.1038/s41565-021-01027-710.1038/s41565-021-01027-7 ↗
26. 10.1002/adfm.20231285610.1002/adfm.202312856 ↗
27. 10.1002/adma.20210213910.1002/adma.202102139 ↗
28. 10.1016/j.cej.2024.15307610.1016/j.cej.2024.153076 ↗
29. 10.1016/j.cej.2023.14631910.1016/j.cej.2023.146319 ↗
30. 10.1002/adma.20180121110.1002/adma.201801211 ↗
31. 10.1016/j.cej.2020.12715710.1016/j.cej.2020.127157 ↗
32. 10.1016/j.cej.2019.12305110.1016/j.cej.2019.123051 ↗
33. 10.1021/acsnano.8b0603910.1021/acsnano.8b06039 ↗
34. 10.1002/adma.20230253710.1002/adma.202302537 ↗
35. 10.1002/anie.20210839610.1002/anie.202108396 ↗
36. 10.1016/j.carbon.2020.10.06210.1016/j.carbon.2020.10.062 ↗
37. 10.1002/adfm.20240292310.1002/adfm.202402923 ↗
38. 10.1016/j.nanoen.2020.10548710.1016/j.nanoen.2020.105487 ↗
39. 10.1016/j.ensm.2019.10.02110.1016/j.ensm.2019.10.021 ↗
40. 10.1007/s40145-021-0520-z10.1007/s40145-021-0520-z ↗
41. 10.1016/j.carbon.2021.10.07710.1016/j.carbon.2021.10.077 ↗
42. 10.1016/j.cej.2019.12274310.1016/j.cej.2019.122743 ↗
43. 10.1002/adfm.20231354410.1002/adfm.202313544 ↗
44. 10.1002/adfm.20230678510.1002/adfm.202306785 ↗
45. 10.1007/s40820-021-00734-z10.1007/s40820-021-00734-z ↗
46. 10.1002/sstr.20230021010.1002/sstr.202300210 ↗
47. 10.1016/j.nantod.2023.10195810.1016/j.nantod.2023.101958 ↗
48. 10.1016/j.cej.2023.14658210.1016/j.cej.2023.146582 ↗
49. 10.1016/j.cej.2019.12298010.1016/j.cej.2019.122980 ↗
50. 10.1002/advs.20210198810.1002/advs.202101988 ↗
51. 10.1002/adfm.20231633810.1002/adfm.202316338 ↗
52. 10.1016/j.scib.2019.10.01110.1016/j.scib.2019.10.011 ↗
53. 10.1016/j.cej.2019.12309610.1016/j.cej.2019.123096 ↗
54. 10.1002/adfm.20240022010.1002/adfm.202400220 ↗
55. 10.1002/adfm.20240350810.1002/adfm.202403508 ↗
56. 10.1016/j.cej.2024.15072910.1016/j.cej.2024.150729 ↗
57. 10.1038/s41467-024-47537-510.1038/s41467-024-47537-5 ↗
58. 10.1002/adma.20230065910.1002/adma.202300659 ↗
59. 10.1007/s40820-021-00635-110.1007/s40820-021-00635-1 ↗