journal article·2023-08Open access

Observation of Colossal Topological Hall Effect in Noncoplanar Ferromagnet Cr5Te6 Thin Films

Yequan Chen, Yingmei Zhu, Renju Lin, Wei Niu, Ruxin Liu, Wenzhuo Zhuang, Xu Zhang, Jinghua Liang, Wenxuan Sun, Zhongqiang Chen, Yongsheng Hu, Fengqi Song, Jian Zhou, Di Wu, Binghui Ge, Hongxin Yang, Rong Zhang, Xuefeng Wang

Advanced Functional Materials· Volume 33· Issue 33

Abstract

Abstract The topological Hall effect (THE) is critical to the exploration of the spin chirality generated by the real‐space Berry curvature, which has attracted worldwide attention for its prospective applications in spintronic devices. However, the prominent THE remains elusive at room temperature, which severely restricts the practical integration of chiral spin textures. Here, a colossal intrinsic THE is showed up to ≈1.6 µΩ cm in large‐area ferromagnet Cr5Te6 thin films epitaxially grown by pulsed laser deposition. Such a THE can be maintained until 270 K, which is attributed to the field‐stimulated noncoplanar spin textures induced by the interaction of the in‐plane ferromagnet and antiferromagnet infrastructures. The first‐principles calculations further verify the considerable Dzyaloshinskii‐Moriya interaction in Cr5Te6. This work not only paves the way for robust chiral spin textures near room temperature in large‐area low‐dimensional ferromagnetic films for practical applications, but also facilitates the development of high‐density and dissipationless spintronic devices.
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Research context

OpenAlex topics: Magnetic properties of thin films · Topological Materials and Phenomena · Multiferroics and related materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Jiangsu Provincial Key Laboratory of Advanced Photonic and Electronic Materials School of Electronic Science and Engineering Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China

National Laboratory of Solid State Microstructures School of Physics Nanjing University Nanjing 210093 China

Ningbo Institute of Materials Technology and Engineering Chinese Academy of Sciences Ningbo 315201 China

Information Materials and Intelligent Sensing Laboratory of Anhui Province Institutes of Physical Science and Information Technology Anhui University Hefei 230601 China

School of Science Nanjing University of Posts and Telecommunications Nanjing 210023 China

National Laboratory of Solid State Microstructures Department of Materials Science and Engineering Nanjing University Nanjing 210093 China

Department of Physics Xiamen University Xiamen 316005 China

Funding

National Natural Science Foundation of China · Fundamental Research Funds for the Central Universities

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