journal article·2026-01-17Open access

Al/Graphene Co-Doped ZnO Electrodes: Impact on CTS Thin-Film Solar Cell Efficiency

Done Ozbek, Meryem Cam, Guldone Toplu, Sevde Erkan, Serkan Erkan, Ali Altuntepe, Kasim Ocakoglu, Sakir Aydogan, Yavuz Atasoy, Mehmet Ali Olgar, Recep Zan

Crystals· Volume 16· Issue 1

Abstract

This study investigates pristine and doped ZnO thin films fabricated via the sol-gel technique, aiming to address efficiency challenges when used as transparent conductive oxide (TCO) layers in thin-film solar cells. ZnO was first doped with aluminum (Al), and subsequently with both Al and reduced graphene oxide (rGO), to evaluate the individual and combined effects of these dopants. The optimal pH value for the ZnO structure was initially determined, with the film produced at pH 9 exhibiting the most favorable characteristics. Al doping was then optimized at a ratio of Al/(Al + Zn) = 0.2, followed by optimization of the graphene content at 1.5 wt%. In this context, the structural, optical, and electrical properties of pristine ZnO, Al-doped ZnO (AZO), and Al and graphene co-doped ZnO (Gr:AZO) thin films were systematically investigated. These films were integrated as TCO layers into Cu2SnS3 (CTS)-based thin-film solar cells fabricated via physical vapor deposition (PVD). The cell architecture employed an 80 nm pristine ZnO window layer, while the doped ZnO films (300 nm) served as TCO layers. To assess the influence of the chemically deposited top layers, device performance was compared against a reference cell in which all layers were fabricated entirely using PVD. As expected, the reference cell exhibited superior performance compared to the cell whose AZO layer deposited chemically; however, the incorporation of both Al and graphene significantly enhanced the efficiency of the chemically modified cell, outperforming devices using only pristine or singly doped ZnO films. These results demonstrate the promising potential of co-doped solution-processed ZnO films as an alternative TCO layer in improving the performance of thin-film solar cell technologies.
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Research context

OpenAlex topics: Copper-based nanomaterials and applications · ZnO doping and properties · Chemical and Physical Properties of Materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Nanotechnology Application and Research Center, Niğde Ömer Halisdemir University, Nigde 51200, Türkiye

Optical Excellence Application and Research Center, Sivas University of Science and Technology, Sivas 58000, Türkiye

Department of Engineering Fundamental Sciences, Faculty of Engineering, Tarsus University, Tarsus 33400, Türkiye

Department of Physics, Science Faculty, Atatürk University, Erzurum 25240, Türkiye

Niğde Zübeyde Hanım Vocational School of Health Services, Niğde Ömer Halisdemir University, Nigde 51200, Türkiye

Department of Physics, Niğde Ömer Halisdemir University, Nigde 51200, Türkiye

Funding

Scientific and Technological Research Council of Türkiye

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