journal article·2022-09Open access

Real‐Time Mimicking the Electronic Structure of N‐Coordinated Ni Single Atoms: NiS‐Enabled Electrochemical Reduction of CO2 to CO (Adv. Energy Mater. 35/2022)

Man Ho Han, Dongjin Kim, Sangkuk Kim, Seung‐Ho Yu, Da Hye Won, Byoung Koun Min, Keun Hwa Chae, Woong Hee Lee, Hyung‐Suk Oh

Advanced Energy Materials· Volume 12· Issue 35

Abstract

CO2 Reduction Reaction In article number 2201843, Woong Hee Lee, Hyung-Suk Oh, and co-workers report that NiS nanoparticles mimicking Ni–NC in real-time, enhance the CO2 reduction reaction activity in a zero-gap electrolyzer. Just as Ni-NC was developed by mimicking the enzymes, NiS also mimics the electronic structure of Ni–NC under operating conditions. The cathodic potential and alkaline media in the device are thought to allow for the real-time electronic structure of the NiS catalyst to mimic that of the NiNC based catalyst.
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Research context

OpenAlex topics: CO2 Reduction Techniques and Catalysts · Electrocatalysts for Energy Conversion · Advanced Photocatalysis Techniques

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Affiliations

Clean Energy Research Center Korea Institute of Science and Technology (KIST) Hwarang‐ro 14‐gil 5, Seongbuk‐gu Seoul 02792 Republic of Korea

Department of Chemical and Biological Engineering Korea University 145 Anam‐ro, Seongbuk‐gu Seoul 02841 Republic of Korea

Department of Materials Science and Engineering Korea University Seoul 02841 Republic of Korea

KIST School Korea University of Science and Technology (UST) Seoul 02792 Republic of Korea

National Agenda Research Division Korea Institute of Science and Technology (KIST) Hwarang‐ro 14‐gil 5, Seonbuk‐gu Seoul 02792 Republic of Korea

Graduate School of Energy and Environment (KU‐KIST Green School) Korea University 145 Anam‐ro, Seongbuk‐gu Seoul 02841 Republic of Korea

Advanced Analysis and Data Center Korea Institute of Science and Technology (KIST) Hwarang‐ro 14‐gil 5, Seongbuk‐gu Seoul 02792 Republic of Korea

School of Advanced Materials Science & Engineering Sungkyunkwan University (SKKU) Suwon 16419 Republic of Korea

KIST‐SKKU Carbon‐Neutral Research Center Sungkyunkwan University (SKKU) Suwon 16419 Republic of Korea

References

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